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In this study we investigated by means of density functional theory calculations the adsorption geometry and bonding mechanism of a single thymine (C$_5$H$_6$N$_2$O$_2$) molecule on Cu(110) surface. In the most stable energetic…

Materials Science · Physics 2008-11-20 V. Caciuc , N. Atodiresei , P. Lazic , Y. Morikawa , S. Blugel

Exploring the role of van der Waals (vdW) forces on the adsorption of molecules on extended metal surfaces has become possible in recent years thanks to exciting developments in density functional theory (DFT). Among these newly developed…

Materials Science · Physics 2015-06-19 Javier Carrasco , Wei Liu , Angelos Michaelides , Alexandre Tkatchenko

In this work, we have studied theoretically the effects of gold adsorption on the Al(001) surface, using {\it ab initio} pseudo-potential method in the framework of the density functional theory. Having found the hollow sites at the Al(001)…

Materials Science · Physics 2009-11-13 N. Zare Dehnavi , M. Payami

The dissociative adsorption of methane on variously oxidized Pd, Pt and Pd-Pt surfaces is investigated using density-functional theory, as a step towards understanding the combustion of methane on these materials. For Pd-Pt alloys, models…

Several dissociated and two non-dissociated adsorption structures of the phenol molecule on the Si(001)-(2 \times 1) surface are studied using density functional theory with various exchange and correlation functionals. The relaxed…

Computational Physics · Physics 2015-05-19 Karen Johnston , Andris Gulans , Tuukka Verho , Martti J. Puska

Extensive density-functional calculations are performed to understand atomic chemisorption on the TiC(111) and TiN(111) surfaces, in particular the calculated pyramid-shaped trends in the adsorption energies for second- and third-period…

Materials Science · Physics 2009-11-11 Carlo Ruberto , Aleksandra Vojvodic , Bengt I. Lundqvist

We use density functional theory to investigate adsorption of liquid mixtures on solid surfaces modified with end-grafted chains. The chains are modelled as freely joined spheres. The fluid molecules are spherical. All spherical species…

Soft Condensed Matter · Physics 2016-03-08 M. Borówko , T. Staszewski

Metal nanoparticle surfaces comprise of multiple planes with various atomic arrangements that interact with gases differently1,2. Identification of gas adsorption properties on all facets is an essential prerequisite for rational design of…

Materials Science · Physics 2015-07-28 Pin Ann Lin , Jonathan Winterstein , John Kohoutek , Henri Lezec , Renu Sharma

We use density functional theory (DFT) with the generalized gradient approximation (GGA) and our first-principles extrapolation method for accurate chemisorption energies {[Mason {\em et al.}, Phys. Rev. B {\bf 69}, 161401R (2004)]} to…

Materials Science · Physics 2007-05-23 Sara E. Mason , Ilya Grinberg , Andrew M. Rappe

Theory of adsorption on a surface with nanolocal defects is proposed. Two efficacy parameters of surface modification for nanotechnological purposes are introduced, where the modification is a creation of nanolocal artificial defects. The…

Chemical Physics · Physics 2009-10-31 Yu. E. Lozovik , A. M. Popov

The adsorption of the chiral molecule lactic acid on chiral Pt surfaces is studied by Density Functional Theory calculations. First we study the adsorption of L-lactic acid on the flat Pt(111) surface. Using the oPBE-vdW functional which…

Materials Science · Physics 2013-10-04 Jörn-Holger Franke , Daniel S. Kosov

Puzzling trends in surface stress were reported experimentally for Ni/W(110) as a function of Ni coverage. In order to explain this behavior, we have performed a density-functional-theory study of the surface stress and atomic structure of…

Materials Science · Physics 2015-06-04 Natasa Stojic , Nadia Binggeli

We report results of the first computer simulation studies of a physically adsorbed gas on a quasicrystalline surface, Xe on decagonal Al-Ni-Co. The grand canonical Monte Carlo method is employed, using a semi-empirical gas-surface…

Materials Science · Physics 2009-11-11 Stefano Curtarolo , Wahyu Setyawan , Nicola Ferralis , Renee D. Diehl , Milton W. Cole

The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

The spin-density functional theory (DFT) and DFT+$U$ with Hubbard $U$ term accounting for on-site Coulomb interactions were applied to investigate structure, stability, and electronic properties of different terminations of the…

Materials Science · Physics 2015-06-03 Adam Kiejna , Tomasz Ossowski , Tomasz Pabisiak

We have investigated the initial growth of Fe on GaAs(110) by means of density functional theory. In contrast to the conventionally used (001)-surface the (110)-surface does not reconstruct. Therefore, a flat interface and small diffusion…

Materials Science · Physics 2009-09-01 A. Grünebohm , H. C. Herper , P. Entel

Electronic and atomic structures of the clean, and As and Te covered Si(211) surface are studied using pseudopotential density functional method. The clean surface is found to have (2 X 1) and rebonded (1 X 1) reconstructions as stable…

Materials Science · Physics 2009-11-10 Prasenjit Sen , Inder P. Batra , S. Sivananthan , C. H. Grein , Nibir Dhar , S. Ciraci

We study the three-dimensional structure formation when atoms are deposited onto a substrate with a decagonal quasicrystalline order. Molecular-dynamicscalculations show that the adsorbate layer consists of ordered nano-scale domains with…

Materials Science · Physics 2007-11-29 Muhittin Mungan , Yves Weisskopf , Mehmet Erbudak

In the X-ray spectra of most X-ray dim isolated neutron stars (XDINSs) absorption features with equivalent widths (EWs) of 50 -- 200 eV are observed. We theoretically investigate different models to explain absorption features and compare…

High Energy Astrophysical Phenomena · Physics 2010-12-17 V. Suleimanov , V. V. Hambaryan , A. Y. Potekhin , M. van Adelsberg , R. Neuhaeuser , K. Werner

Using the atomic density function theory (ADFT), we examine the point defect absorption at [110] symmetrical tilt grain boundaries in body-centered cubic iron. It is found that the sink strength strongly depends on misorientation angle. We…

Materials Science · Physics 2015-12-18 O. Kapikranian , H. Zapolsky , R. Patte , C. Pareige , B. Radiguet , P. Pareige