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Resonant inelastic X-ray scattering (RIXS) is a powerful probe of elementary excitations in solids. It is now widely applied to study magnetic excitations. However, its complex cross-section means that RIXS has been more difficult to…

Strongly Correlated Electrons · Physics 2021-06-30 H. C. Robarts , M. Garcia-Fernandez , J. Li , A. Nag , A. C. Walters , N. E. Headings , S. M. Hayden , Ke-Jin Zhou

The anisotropy of the magnetic incommensurate fluctuations in Sr2RuO4 has been studied by inelastic neutron scattering with polarized neutrons. We find a sizeable enhancement of the out of plane component by a factor of two for intermediate…

Strongly Correlated Electrons · Physics 2009-11-10 M. Braden , P. Steffens , Y. Sidis , J. Kulda , S. Hayden , N. Kikugawa , Y. Maeno

When strong spin-orbit coupling removes orbital degeneracy, it would at the same time appear to render the Jahn-Teller mechanism ineffective. We discuss such a situation, the t_2g manifold of iridates, and show that, while the Jahn-Teller…

Strongly Correlated Electrons · Physics 2016-03-08 Ekaterina M. Plotnikova , Maria Daghofer , Jeroen van den Brink , Krzysztof Wohlfeld

The effect of the Doppler shift is studied in a model for the $\alpha$-$\beta$ bands of Sr$_2$RuO$_4$ consisting of two hybridized 1D bands. Assuming a superconducting gap with nodes in the diagonal directions, we examine the oscillation of…

Superconductivity · Physics 2009-11-10 Y. Tanaka , K. Kuroki , Y. Tanuma , S. Kashiwaya

We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…

We have investigated the electronic structure of Sr2IrO4 using core level resonant inelastic x-ray scattering. The experimental spectra can be well reproduced using ab initio density functional theory based multiplet ligand field theory…

Polarized and unpolarized neutron inelastic scattering has been used to measure the spin excitations in the spin-charge-ordered stripe phase of La5/3Sr1/3NiO4. At high energies, sharp magnetic modes are observed characteristic of a static…

Strongly Correlated Electrons · Physics 2009-11-07 A. T. Boothroyd , D. Prabhakaran , P. G. Freeman , S. J. S. Lister , M. Enderle , A. Hiess , J. Kulda

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

We study dynamical properties of the anisotropic triangular quantum antiferromagnet Cs_2CuCl_4. Inelastic neutron scattering measurements have established that the dynamical spin correlations cannot be understood within a linear spin wave…

Strongly Correlated Electrons · Physics 2007-05-23 Martin Y. Veillette , Andrew J. A. James , Fabian H. L. Essler

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

Strongly Correlated Electrons · Physics 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson

We investigated the low-energy incommensurate (IC) magnetic fluctuations in Sr$_2$RuO$_4$ by the high-resolution inelastic neutron scattering measurements and random phase approximation (RPA) calculations. We observed a spin resonance with…

The low energy spin excitations of La(2-x)Sr(x)NiO(4), x = 0.275 and 1/3, have been investigated by unpolarized- and polarized-inelastic neutron scattering from single crystals. A pattern of magnetic diffuse scattering is observed in both…

Strongly Correlated Electrons · Physics 2011-03-17 P. G. Freeman , D. Prabhakaran , K. Nakajima , A. Stunault , M. Enderle , C. Niedermayer , C. Niedermayer , K. Yamada , A. T. Boothroyd

The charge transfer reaction Ar+ + N2 --> Ar + N2+ has been investigated in a crossed beam experiment in combination with three-dimensional velocity map imaging. Angular differential state-to-state cross sections were determined as a…

Chemical Physics · Physics 2015-06-12 S. Trippel , M. Stei , J. A. Cox , R. Wester

Although correlated electronic-structure calculations explain very well the normal state of Sr$_2$RuO$_4$, its superconducting symmetry is still unknown. Here we construct the spin and charge fluctuation pairing interactions based on its…

Superconductivity · Physics 2019-11-27 Olivier Gingras , Reza Nourafkan , André-Marie S. Tremblay , Michel Côté

The spin fluctuations in the normal state of the unconventional superconductor Sr2RuO4 have been studied using inelastic neutron scattering with polarization analysis on single crystals. We find that the spin fluctuations are anisotropic…

Strongly Correlated Electrons · Physics 2007-05-23 B. Fak , S. Raymond , F. Servant , P. Lejay , J. Flouquet

We report a neutron scattering study of the instantaneous spin correlations in the two-dimensional spin S=5/2 square-lattice Heisenberg antiferromagnet Rb_2MnF_4. The measured correlation lengths are quantitatively described, with no…

Strongly Correlated Electrons · Physics 2009-10-31 Y. S. Lee , M. Greven , B. O. Wells , R. J. Birgeneau , G. Shirane

Magnetic Raman scattering from a frustrated spin-1/2 Heisenberg-chain is considered with a focus on the uniform phase of the spin-Peierls compound CuGeO_3. The Raman intensity is analyzed in terms of a Loudon-Fleury scattering process using…

Strongly Correlated Electrons · Physics 2016-08-31 Wolfram Brenig

With octahedrally coordinated $t_{\rm 2g}$ orbitals which are active at filling $n=2$, the $\rm Sr_2CrO_4$ compound exhibits rich interplay of spin-orbital physics with tetragonal distortion induced crystal field tuning by external agent…

Strongly Correlated Electrons · Physics 2022-10-20 Shubhajyoti Mohapatra , Dheeraj Kumar Singh , Avinash Singh

We use the symmetry constrained low energy effective Hamiltonian of iron based superconductors to study the Raman scattering in the normal state of underdoped iron-based superconductors. The incoming and scattered Raman photons couple…

Strongly Correlated Electrons · Physics 2015-07-01 M. Khodas , A. Levchenko

We use resonant inelastic x-ray scattering (RIXS) at the Ir L3 edge to study the effect of hole doping upon the Jeff=1/2 Mott-insulating state in Sr2IrO4, via Rh replacement of the Ir site. The spin-wave gap, associated with XY-type…

Strongly Correlated Electrons · Physics 2020-03-24 J. Bertinshaw , J. K. Kim , J. Porras , K. Ueda , N. H. Sung , A. Efimenko , A. Bombardi , Jungho Kim , B. Keimer , B. J. Kim