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We consider a model of Raman scattering for a two--dimensional $S=1/2$ Heisenberg Anti-Ferromagnet which includes a {\it dynamical} spin--phonon interaction. We observe a broadening of the line shape due to increased coupling with excited…

Condensed Matter · Physics 2009-10-28 Matthew J. Reilly , A. G. Rojo

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

In FeSc2S4 spin-orbital exchange competes with strong spin-orbit coupling, suppressing long-range spin and orbital order and, hence, this material represents one of the rare examples of a spin-orbital liquid ground state. Moreover, it is…

Strongly Correlated Electrons · Physics 2015-06-22 L. Mittelstädt , M. Schmidt , Zhe Wang , F. Mayr , V. Tsurkan , P. Lunkenheimer , D. Ish , L. Balents , J. Deisenhofer , A. Loidl

Inelastic neutron scattering is used to investigate the collective magnetic excitations of the high-temperature superconductor parent antiferromagnet La2CuO4. We find that while the lower energy excitations are well described by spin-wave…

Strongly Correlated Electrons · Physics 2010-12-13 N. S. Headings , S. M. Hayden , R. Coldea , T. G. Perring

Transformation of Coulomb interaction terms to the pseudo-orbital basis constituted by $J=1/2$ and $3/2$ states arising from spin-orbit coupling provides a versatile tool. This formalism is applied to investigate magnetic anisotropy effects…

Strongly Correlated Electrons · Physics 2019-03-11 Shubhajyoti Mohapatra , Avinash Singh

We report the first observation of soft-x-ray scattering from spin fluctuations in a high-Tc parent compound. An antiferromagnetic charge transfer insulator, CaCuO2, was irradiated by Cu M-edge soft x-rays. Ultra-high resolution…

Raman scattering in the spin-crossover system [Fe(pmd)(H2O){Au(CN)2}2]*H2O reveals a complex three-phase spin-state transition in contrast to earlier observations in magnetization measurements. We observe different spin state phases as…

Strongly Correlated Electrons · Physics 2010-03-09 V. Gnezdilov , P. Lemmens , P. Scheib , M. Ghosh , Yu. G. Pashkevich , H. Paulsen , V. Schuenemann , J. A. Wolny , G. Agusti , J. A. Real

The strongly correlated insulator Ca$_{2}$RuO$_4$ is considered as a paradigmatic realization of both spin-orbital physics and a band-Mott insulating phase, characterized by orbitally selective coexistence of a band and a Mott gap. We…

The two-magnon (2M) excitation at 3000 cm-1 in Sr_14Cu_24O_41 two-leg ladder is studied by Raman scattering. A slight anisotropy of the superexchange coupling J_{\perp}/J_{||} \approx 0.8 with J_{||} = 110 \pm 20 meV is proposed from the…

Strongly Correlated Electrons · Physics 2009-11-07 A. Gozar , G. Blumberg , B. S. Dennis , B. S. Shastry , N. Motoyama , H. Eisaki , S. Uchida

We present a microscopic model for the anisotropic exchange interactions in Sr$_{2}$IrO$_{4}$. A direct construction of Wannier functions from first-principles calculations proves the $j_{\mathrm{eff}}$=1/2 character of the spin-orbit…

Strongly Correlated Electrons · Physics 2013-05-29 Hosub Jin , Hogyun Jeong , Taisuke Ozaki , Jaejun Yu

Two-magnon Raman scattering intensity is obtained for two-dimensional spin-1/2 antiferromagnets in presence of hopping disorder. A consistent mode assignment scheme is prescribed which essentially establishes a correspondence between the…

Condensed Matter · Physics 2007-05-23 Saurabh Basu

Spin excitations of layered copper oxide show various characteristic features, depending on the carrier concentration. In this study, we conducted inelastic neutron scattering (INS) measurements on La$_{2-x}$Sr$_{x}$CuO$_4$ (LSCO), with $x$…

Superconductivity · Physics 2022-01-26 K. Ikeuchi , S. Wakimoto , M. Fujita , T. Fukuda , R. Kajimoto , M. Arai

We report Raman scattering measurements on iron-pnictide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals with varying cobalt $x$ content. The electronic Raman continuum shows a strong spectral weight redistribution upon…

Superconductivity · Physics 2011-10-07 L. Chauvière , Y. Gallais , M. Cazayous , M. A. Méasson , A. Sacuto , D. Colson , A. Forget

The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…

Astrophysics · Physics 2007-05-23 Jacques Moret-Bailly

The low-temperature magnetic excitations of the two-dimensional spin-5/2 square-lattice Heisenberg antiferromagnet Rb2MnF4 have been probed using pulsed inelastic neutron scattering. In addition to dominant sharp peaks identified with…

Strongly Correlated Electrons · Physics 2009-11-11 T. Huberman , R. Coldea , R. A. Cowley , D. A. Tennant , R. L. Leheny , R. J. Christianson , C. D. Frost

Lack of inversion symmetry in metals breaks SU(2) symmetry which results in spin-splitting of the electronic states at the Fermi level due to various types of spin-orbit coupling (SOC) such as Dresselhaus, Rashba, or Ising (also called…

Mesoscale and Nanoscale Physics · Physics 2026-04-02 Mojdeh Saleh , Saurabh Maiti

We study the resonance fluorescence properties of an optically active spin 1/2 system, elucidating the effects of a magnetic field on the coherence of the scattered light. We derive a master equation model for this system that reproduces…

By performing time-of-flight neutron scattering measurements on a large amount of single crystals of Sr$_2$RuO$_4$, we studied detailed structure of the imaginary part of the dynamic spin susceptibility over a wide range of phase space. In…

Strongly Correlated Electrons · Physics 2015-05-28 K. Iida , M. Kofu , N. Katayama , J. Lee , R. Kajimoto , Y. Inamura , M. Nakamura , M. Arai , Y. Yoshida , M. Fujita , K. Yamada , S. -H. Lee

Clusters of single spins form the relevant spin entities in the formation of long-range magnetic order in spin cluster Mott insulators. Such type of spin order bears resemblance to molecular crystals, and we therefore may expect a…

Strongly Correlated Electrons · Physics 2020-01-08 R. B. Versteeg , C. Boguschewski , P. Becker , P. H. M. van Loosdrecht

We calculate the reflection and transmission probabilities in a one-dimensional Fermi gas with an equal mixing of the Rashba and Dresselhaus spin-orbit coupling (RD-SOC) produced by an external Raman laser field. These probabilities are…

Quantum Physics · Physics 2016-12-07 Su-Ju Wang , Chris H. Greene