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Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…

We investigate photoinization, energy deposition, plasma formation and the ultrafast optical breakdown in crystalline silicon irradiated by intense near-infrared laser pulses with pulse duration $\tau \le $ 100 fs. The occurrence of…

Materials Science · Physics 2021-11-24 Tzveta Apostolova , Boyan Obreshkov

Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and…

We apply the coupled dynamics of time-dependent density functional theory and Maxwell equations to the interaction of intense laser pulses with crystalline silicon. As a function of electromagnetic field intensity, we see several regions in…

Other Condensed Matter · Physics 2015-06-03 K. Yabana , T. Sugiyama , Y. Shinohara , T. Otobe , G. F. Bertsch

Ionization and excitation of water molecules in intense laser pulses is studied theoretically by solving the three-dimensional time-dependent electronic Schr\"odinger equation within the single-active-electron approximation. The possibility…

Atomic Physics · Physics 2011-12-13 Simon Petretti , Alejandro Saenz , Alberto Castro , Piero Decleva

Time-resolved X-ray Emission/Absorption Spectroscopy (Tr-XES/XAS) is an informative experimental tool sensitive to electronic dynamics in materials, widely exploited in diverse research fields. Typically, Tr-XES/XAS requires X-ray pulses…

A circularly polarized laser pulse can induce persistent intra-molecular currents by either exciting or ionizing molecules. These two cases are identified as electron currents and hole currents, respectively, and up to now they have been…

Chemical Physics · Physics 2024-10-18 Tennesse Joyce , Agnieszka Jaron

Intense few cycle terahertz pulses exhibit complex non-linear behavior under interaction with heavily n-doped Si. Fast increase in the transmission of a 700 fs pulse (central frequency 1.5 THz) through the Si sample (low field transmission…

Using a three-dimensional quasiclassical technique we explore the double ionization pathways of a diatomic molecule driven by an intense infrared (800nm) ultrashort laser pulse. For intensities corresponding to the tunneling regime, we find…

Atomic Physics · Physics 2009-02-26 Agapi Emmanouilidou

Ultrafast pump-probe technique is a powerful tool to understand and manipulate properties of materials for designing novel quantum devices. An intense, single cycle terahertz pulse can change the intrinsic properties of semiconductor…

Mesoscale and Nanoscale Physics · Physics 2020-07-13 Chen-Yen Lai , D. A. Yarotski , Jian-Xin Zhu

The physics of strong-field applications requires driver laser pulses that are both energetic and extremely short. Whereas optical amplifiers, laser and parametric, boost the energy, their gain bandwidth restricts the attainable pulse…

Generation of collimated, quasi-monoenergetic electron beams (peak energy ~17-22MeV, divergence ~10mrad, energy spread ~20%) by interaction of Ti:sapphire laser pulse of 200fs duration, focussed to an intensity of ~ 2.1x10^18 W/cm^2,with an…

Plasma Physics · Physics 2019-08-09 D. Hazra , A. Moorti , B. S. Rao , A. Upadhyay , J. A. Chakera , P. A. Naik

A new regime in the interaction of a two-colour ($\omega$,$2\omega$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For…

Plasma Physics · Physics 2020-04-22 Y. X. Zhang , S. Rykovanov , Mingyuan Shi , C. L. Zhong , X. T. He , B. Qiao , M. Zepf

Semi-heavy water (HOD) is one of the simplest molecules in which the bonds are labelled by isotope. We demonstrate that a pair of intense few-femtosecond infrared laser pulses can be used to selectively tunnel ionize along one of the two…

Polyatomic molecules provide complex internal structures that are ideal for applications in quantum information science, quantum simulation, and precision searches for physics beyond the Standard Model. A key feature of polyatomic molecules…

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

Materials Science · Physics 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…

Atomic Physics · Physics 2017-05-25 R. E. F. Silva

Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the…

Atomic Physics · Physics 2020-12-18 Konrad Wenz , Ivan Kozyryev , Rees L. McNally , Leland Aldridge , Tanya Zelevinsky

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein
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