Related papers: Ultrafast absorption of intense x rays by nitrogen…
Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied…
The total photo-absorption cross section of $^4$He is evaluated microscopically using two- (NN) and three-nucleon (NNN) interactions based upon chiral effective field theory ($\chi$EFT). The calculation is performed using the Lorentz…
The present manuscript considers the application of the method of the near-edge X-ray absorption spectroscopy (NEXAFS) for the investigation of the graphene-based systems (from free-standing graphene to the metal-intercalation-like…
Attosecond transient absorption spectroscopy (ATAS) is becoming an indispensable and powerful tool in the emerging field of attochemistry, while the interpretation of measurements often requires full considerations of the coupling among…
The interaction of swift, free-space electrons with confined optical near fields has recently sparked much interest. It enables a new type of photon-induced near-field electron microscopy, mapping local optical near fields around…
Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…
We present measurements of K-shell x-ray emission following charge exchange of fully ionized argon with various neutral gaseous targets at small collision energies inside an electron beam ion trap. We also resolve the principal quantum…
Resonance fluorescence of laser-driven highly charged ions is studied in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for…
X-ray scattering at the carbon absorption edge is uniquely sensitive to local molecular bond identity and orientation in organic nanostructures, encoded as a function of photon energy and polarization. However, quantitative analysis is…
Absorption of infrared and visible radiation from stellar emission spectra by the negatively charged hydrogen ions H$^{-}$ is considered. The explicit formula for the photodetachment cross-section of the negatively charged hydrogen ion(s)…
Nearly one third of all nitrogen oxides are removed from the atmosphere through the reactive uptake of N$_2$O$_5$ into aqueous aerosol. The primary step in reactive uptake is the rapid hydrolysis of N$_2$O$_5$, yet despite significant…
We describe a novel technique to characterize ultrashort electron bunches in X-ray Free-Electron Lasers. Namely, we propose to use coherent Optical Transition Radiation to measure three-dimensional (3D) electron density distributions. Our…
Determination of optical absorption cross-section is always among the central importance of understanding a material. However its realization on individual nanostructures, such as carbon nanotubes, is experimentally challenging due to the…
We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…
We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor…
We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in…
A number of emission and absorption features are expected to be visible in high energy resolution X-ray spectra of type 1 AGN with ionized gas along the line of sight (so called "warm absorbers"). Emission strongly depends on the…
Isotope effects associated with gas phase N2 photolysis are used to interpret Martian atmospheric evolution, icy satellite atmospheric chemistry and meteorite isotopic anomalies from nebular N2 photochemistry. To interpret observations at…
Electron energy loss near edge spectra (ELNES) has been calculated for two different Fe based superconducting material FeSe and FeTe using density functional theory (DFT). Fe K-edge absorption spectra consist of several features, origins of…
X-ray free-electron lasers (FELs) are promising tools for structural determination of macromolecules via coherent x-ray scattering. During ultrashort and ultraintense x-ray pulses with an atomic scale wavelength, samples are subject to…