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We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

We report first direct experimental evidence of interspecies ion separation in direct-drive ICF experiments performed at the OMEGA laser facility via spectrally, temporally and spatially resolved imaging x-ray-spectroscopy data [S. C. Hsu…

We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…

Soft X-rays (90-173 eV) from the 3rd generation Canadian Light Source have been used in conjunction with a multi coincidence time and position sensitive detection apparatus to observe the dissociative ionization of OCS. By varying the X-ray…

We present the first high-resolution laboratory spectra of X-ray emission following L-shell charge exchange between nickel ions and neutral H2 and He. We employ the commonly used charge exchange models found in XSPEC and SPEX, ACX and…

An analysis of Lyman series lines arising from hydrogen-like oxygen and neon ions in the coronae of the active RS CVn-type binaries II Peg and IM Peg, observed using the {\it Chandra} High Resolution Transmission Grating Spectrograph, shows…

Astrophysics · Physics 2009-11-10 Paola Testa , Jeremy J. Drake , Giovanni Peres , Edward E. DeLuca

Resonant inelastic scattering measurements of poly(pyridine-2,5-diyl) have been performed at the N1s and C1s edges using synchrotron radiation. For comparison, molecular orbital calculations of the spectra have been carried out with the…

We establish the spectral line shape of orbital excitations created by resonant inelastic X-ray scattering for the model Mott insulator CoO. Improved experimental energy resolution reveals that the line shapes are strikingly different from…

Strongly Correlated Electrons · Physics 2015-06-18 L. Andrew Wray , J. Li , Z. Q. Qiu , Jinsheng Wen , Zhijun Xu , Genda Gu , Shih-Wen Huang , Elke Arenholz , Wanli Yang , Zahid Hussain , Yi-De Chuang

K-shell ionization and characteristic x-ray radiation (CXR) by high-energy electrons and positrons in oriented silicon crystals are studied using computer simulation. A method for this simulation has been developed and is described in…

Atomic Physics · Physics 2026-04-14 S. V. Trofymenko , I. V. Kyryllin

Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…

Resonant X-ray scattering (RXS) is a spectroscopy where both the power of site selective diffraction and the power of local absorption spectroscopy regarding atomic species are combined. By virtue of the dependence on the core level state…

Materials Science · Physics 2007-11-12 Yves Joly , Elena S. Nazarenko , José-Emilio Lorenzo , Sergio Di Matteo , Calogero R. Natoli

X-ray scattering spectra of Cu and Ni metals have been measured using monochromatic synchrotron radiation tuned from far above to more than 10 eV below threshold. Energy conservation in the scattering process is found to be sufficient to…

Materials Science · Physics 2012-01-04 M. Magnuson , J. -E. Rubensson , A. Föhlisch , N. Wassdahl , A. Nilsson , N. Mårtensson

Molecular iodine was photoexcited by a strong 800 nm laser, driving several channels of multiphoton excitation. The motion following photoexcitation was probed using time-resolved X-ray scattering, which produces a scattering map…

Chemical Physics · Physics 2020-03-25 Philip H. Bucksbaum , Matthew R. Ware , Adi Natan , James P. Cryan , James M. Glownia

We report a high-resolution resonant inelastic soft x-ray scattering study of the quantum magnetic spin-chain materials Li2CuO2 and CuGeO3. By tuning the incoming photon energy to the oxygen K-edge, a strong excitation around 3.5 eV energy…

High resolution spectroscopic observations of Seyfert galaxies with Chandra and XMM-Newton allows us to study the detailed ionization and thermal structures of the X-ray absorbing/emitting material in the circumnuclear environment. The vast…

We study the resonant x-ray scattering at Si and Al K-edges from chiral materials, $\alpha$-quartz and $\alpha$-berlinite. We derive the general form of the scattering matrix for the dipole transition by summing up the local scattering…

Materials Science · Physics 2012-10-03 Jun-ichi Igarashi , Manabu Takahashi

The massive X-ray binary Cen X-3 was observed over approximately one quarter of the system's 2.08 day orbit, beginning before eclipse and ending slightly after eclipse center with the Chandra X-ray Observatory using its High-Energy…

Core-excitation of water ice releases many different molecules and ions in the gas phase. Studying these desorbed species and the underlying mechanisms can provide useful information on the effects of X-ray irradiation in ice. We report a…

Chemical Physics · Physics 2020-10-20 R. Dupuy , G. Féraud , M Bertin , C. Romanzin , L. Philippe , T. Putaud , X. Michaut , R. Cimino , V. Baglin , J. -H. Fillion

Experimental cross sections for $m$-fold photodetachment ($m=3-6$) of silicon anions via $K$-shell excitation and ionization were measured in the photon-energy range of 1830-1900 eV using the photon-ion merged-beams technique at a…

We present a temperature and doping dependent resonant inelastic X-ray scattering experiment at the V L$_{2,3}$ and O K edges in La$_{1-x}$Sr$_x$VO$_3$ for $x=0$ and $x=0.1$. This material is a canonical example of a compound that exhibits…

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