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Resonant x-ray scattering shows that the bulk structure of the twist-bend liquid crystal phase, recently discovered in bent molecular dimers, has spatial periodicity without electron density modulation, indicating a lattice-free heliconical…

Experimental cross sections for m-fold photodetachment (m=2-5) of oxygen anions via K-shell excitation and ionization were measured in the photon-energy range of 525-1500 eV using the photon-ion merged-beams technique at a synchrotron light…

Core-level spectra of liquids can be difficult to interpret due to the presence of a range of local environments. We present computational methods for investigating core-level spectra based on the idea that both local structural parameters…

Soft Condensed Matter · Physics 2017-08-09 Johannes Niskanen , Christoph J. Sahle , Keith Gilmore , Frank Uhlig , Jens Smiatek , Alexander Föhlisch

The structural, magnetic and electronic properties of transition metal oxides reflect in atomic charge, spin and orbital degrees of freedom. Resonant x-ray scattering (RXS) allows us to perform an accurate investigation of all these…

Strongly Correlated Electrons · Physics 2015-05-14 G. Subías , Joaquín García , Blasco Javier , Javier Herrero-Martin , María Concepción Sanchez

We study the scattering of infrared light by small dielectric core-shell particles taking a sapphire sphere with a CaO core as an example. The extinction efficiency of such a particle shows two intense series of resonances attached,…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 E. Thiessen , F. X. Bronold , R. L. Heinisch , H. Fehske

In this work, we report X-ray photoelectron (XPS) and valence band (VB) spectroscopy measurements of surfactant-free silver nanoparticles and silver/linear carbon chains (Ag@LCC) structures prepared by pulse laser ablation (PLA) in water.…

Mesoscale and Nanoscale Physics · Physics 2017-11-21 D. W. Boukhvalov , I. S. Zhidkov , E. Z. Kurmaev , E. Fazio , S. O. Cholakh , L. D'Urso

The electronic structure of CoO is studied by resonant inelastic soft X-ray scattering spectroscopy using photon energies across the Co 2p absorption edges. The different spectral contributions from the energy-loss structures are identified…

Materials Science · Physics 2012-01-04 M. Magnuson , S. M. Butorin , J. -H. Guo , J. Nordgren

A recent and unexpected discrepancy between \textit{ab initio} simulations and the interpretation of a laser shock experiment on aluminum, probed by X-ray Thomson scattering (XRTS), is addressed. The ion-ion structure factor deduced from…

Plasma Physics · Physics 2020-11-19 J. Clerouin , P. Arnault , G. Robert , C. Ticknor , J. Kress , L. Collins

We present high resolution laboratory spectra of K-shell X-ray lines from inner-shell excited and ionized ions of oxygen, obtained with a reflection grating spectrometer on the electron beam ion trap (EBIT-I) at the Lawrence Livermore…

We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

Materials Science · Physics 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

The experimental characterization of scattering resonances in low energy collisions has proven to be a stringent test for quantum chemistry calculations. Previous measurements on the NO-H$_2$ system at energies down to $10$ cm$^{-1}$…

Soft x-ray resonant scattering has been used to examine the charge and magnetic interactions in the cycloidal antiferromagnetic compound \dyfeal. By tuning to the Dy $M_4$ and $M_5$ absorption edges and the Fe L(2) and L(3) absorption edges…

Strongly Correlated Electrons · Physics 2007-05-23 T. A. W. Beale , S. B. Wilkins , P. D. Hatton , P. Abbamonte , S. Stanescu , J. A. Paixao

Synchrotron X-ray diffraction experiments and molecular dynamics simulations have been performed on simple aliphatic aldehydes, from propanal to nonanal. The performance of the OPLS all-atom interaction potential model for aldehydes has…

Chemical Physics · Physics 2018-11-27 Ildikó Pethes , László Temleitner , Matija Tomšič , Andrej Jamnik , László Pusztai

We present the first optical images of scattered light from large, detached gas/dust shells around two carbon stars, R Scl and U Ant, obtained in narrow band filters centred on the resonance lines of neutral K and Na, and in a Str. b filter…

Astrophysics · Physics 2009-11-06 D. Gonzalez Delgado , H. Olofsson , H. E. Schwarz , K. Eriksson , B. Gustafsson

X-ray emissions from cometary atmospheres were modeled from first principles using the charge-exchange interaction with solar wind ions as well as coherent scattering of solar X-rays from dust and ice grains. Scattering cross-sections were…

High Energy Astrophysical Phenomena · Physics 2018-01-31 Bradford Snios , Jack Lichtman , Vasili Kharchenko

The most important processes for the creation of S12+ to S14+ ions excited states from the ground configurations of S9+ to S14+ ions in an electron cyclotron resonance ion source, leading to the emission of K X-ray lines, are studied.…

By simulating the dissociation of O2 molecules on the Be(0001) surface using the first-principles molecular dynamics approach, we propose a new atomistic model for the surface oxidation of sp metals. In our model, only the dissociation of…

Materials Science · Physics 2015-05-18 Yu Yang , Ping Zhang

In existing theoretical approaches to core-level excitations of transition-metal ions in solids relaxation and polarization effects due to the inner core hole are often ignored or described phenomenologically. Here we set up an ab initio…

Soft X-ray resonant scattering studies at the Mn $L_{\texttt{II, III}}$- and the La $M_{\texttt{IV, V}}$- edges of single-crystal LaSr$_2$Mn$_2$O$_7$ are reported. At low temperatures, below $T_\texttt{N} \approx 160$ K, energy scans with a…

Strongly Correlated Electrons · Physics 2014-07-08 H. -F. Li , Y. Su , Tapan Chatterji , A. Nefedov , J. Persson , P. Meuffels , Y. Xiao , Th. Brückel