Related papers: Water Molecules in Ultrashort Intense Laser Fields
We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…
Liquid water at ambient temperature displays ultrafast molecular motions and concomitant fluctuations of very strong electric fields originating from the dipolar H2O molecules. We show that such random intermolecular fields induce tunnel…
A time-dependent bond-hardening process is discovered in a polyatomic molecule (tetramethyl silane, TMS) using few-cycle pulses of intense 800 nm light. In conventional mass spectrometry, symmetrical molecules like TMS do not exhibit a…
The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent…
Photoelectron angular distributions (PADs) of oriented polar molecules in response to different polarized lasers are systematically investigated. It is found that the PADs of polar CO molecules show three distinct styles excited by…
The ion-induced long-range orientational order between water molecules recently observed in second harmonic scattering experiments and illustrated with large scale molecular dynamics simulations is quantitatively explained using the…
We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…
We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…
This paper reviews recent observations of water in Galactic interstellar clouds and nearby galactic nuclei. Two results are highlighted: (1) Multi-line H$_2$O mapping of the Orion Bar shows that the water chemistry in PDRs is driven by…
We propose a laser-based method for the preparation of high-energy polarized electrons, from the ionization of isolated spin-polarized hydrogen (SPH) atoms. The SPH atoms are prepared from the photodissociation of HCl, using two consecutive…
The spin-dependent density of states and the density of spin polarization of an InAs-based two-dimensional electron gas with the Rashba spin-orbit coupling under an intense terahertz laser field are investigated by utilizing the Floquet…
The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…
The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…
We investigate two-photon double ionization of helium by intense ($10^{15} W/cm^2$) ultrashort ($\approx 300$ as) soft X-ray pulses (E = 91.6 eV). The time-dependent two-electron Schr\"odinger equation is solved using a coupled channel…
We study the interaction of strong femtosecond laser pulses with the C$_{60}$ molecule employing time-dependent density functional theory with the ionic background treated in a jellium approximation. The laser intensities considered are…
This research demonstrates high-repetition-rate laser-accelerated ion beams via dual, intersecting, counterpropagating laser-driven blast waves to precisely shape underdense gas into long-lived near-critical density targets. The collision…
The employment of ultrashort laser sources at the mid-IR spectral region for transparent materials is designed to open new routes for laser patterning and a wealth of exciting applications in optics and photonics. To elucidate the material…
We show, both classically and quantum mechanically, enantioselective orientation of gas phase chiral molecules excited by laser fields with twisted polarization. Counterintuitively, the induced orientation, whose direction is laser…
The subject of this paper is the scattering of a very intense laser pulse (intensity $I\sim10^{21}\;{\mathrm{W/cm^2}}$) on relativistic electrons with Lorentz factor between 10 and 45. The laser pulse is modeled by a plane wave with finite…
Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…