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We present a calculation of a fourth-order, time-dependent density correlation function that measures higher-order spatiotemporall correlations of the density of a liquid. From molecular dynamics simulations of a glass-forming Lennard-Jones…

Statistical Mechanics · Physics 2009-11-07 N. Lacevic , F. W. Starr , T. B. Schroder , V. N. Novikov , S. C. Glotzer

The formation, growth, structure and cluster size distribution (CSD) properties in a two-dimensional system of particles interacting with Lennard-Jones (LJ) potential under controlled cooling condition have been studied using Monte-Carlo…

Soft Condensed Matter · Physics 2018-01-18 Barnana Pal

We present a finite-size scaling analysis of the droplet condensation-evaporation transition of a lattice gas (in two and three dimensions) and a Lennard-Jones gas (in three dimensions) at fixed density. Parallel multicanonical simulations…

Soft Condensed Matter · Physics 2015-08-04 Johannes Zierenberg , Wolfhard Janke

The slow down of dynamics in glass forming liquids as the glass transition is approached has been characterised through the Adam-Gibbs relation, which relates relaxation time scales to the configurational entropy. The Adam-Gibbs relation…

Soft Condensed Matter · Physics 2018-05-24 Anshul D. S. Parmar , Shiladitya Sengupta , Srikanth Sastry

Wetting and drying of a rigid substrate by a Lennard-Jones fluid in molecular dynamics simulations is reported. The size of the substrate particles, being smaller than the fluid particles in former simulations, is now taken to be equal to,…

Soft Condensed Matter · Physics 2015-06-25 C. Bruin

We consider the Kob-Andersen model, a cooperative lattice gas with kinetic constraints which has been widely analyzed in the physics literature in connection with the study of the liquid/glass transition. We consider the model in a finite…

Probability · Mathematics 2020-09-02 Fabio Martinelli , Assaf Shapira , Cristina Toninelli

We address a recent conjecture according to which the relaxation time $\tau$ of a viscous liquid obeys density scaling ($\tau=F(\rho^\gamma/T)$ where $\rho$ is density) if the liquid is ``strongly correlating,'' i.e., has almost 100%…

Soft Condensed Matter · Physics 2012-03-27 Thomas B. Schrøder , Ulf R. Pedersen , Jeppe C. Dyre

The relationship between excess entropy and diffusion is revisited by means of large-scale computer simulation combined to supervised learning approach to determine the excess entropy for the Lennard-Jones potential. Results reveal that it…

Statistical Mechanics · Physics 2021-11-03 Anthony Saliou , Philippe Jarry , Noel Jakse

We study low-Reynolds-number fluid flow through a two-dimensional porous medium modeled as a Lorentz gas. Using extensive finite element simulations we fully resolve the flow fields for packing fractions approaching the percolation…

Fluid Dynamics · Physics 2024-05-22 Mirko Residori , Suvendu Mandal , Axel Voigt , Christina Kurzthaler

Dynamical quantities such as the diffusion coefficient and relaxation times for some glass-formers may depend on density and temperature through a specific combination, rather than independently, allowing the representation of data over…

Statistical Mechanics · Physics 2013-09-27 Shiladitya Sengupta , Thomas B. Schröder , Srikanth Sastry

In this paper, a formalism for the activation volume of glass forming materials is suggested. An isothermal equation of state for the activation volume is formulated, which is extended to a generalized equation of state that describes the…

Fundamental thermodynamics and an earlier elastic solid-state point defect model [P. Varotsos and K. Alexopoulos, Phys. Rev B 15, 4111 (1977); 18, 2683 (1978)] are employed to formulate an analytical second-order polynomial function…

Soft Condensed Matter · Physics 2009-03-31 A. N. Papathanassiou

We study supercooled dynamics in quantum hard-sphere liquid using quantum mode-coupling formulation. In the moderate quantum regime, classical cage effects lead to slower dynamics compared to strongly quantum regime, where tunneling…

Statistical Mechanics · Physics 2021-02-03 Ankita Das , Eran Rabani , Kunimasa Miyazaki , Upendra Harbola

In this third paper of the series, which started with [N. P. Bailey et al., J. Chem. Phys. 129, 184507 and 184508 (2008)], we continue the development of the theoretical understanding of strongly correlating liquids - those whose…

Soft Condensed Matter · Physics 2013-01-29 Thomas B. Schrøder , Nicholas P. Bailey , Ulf R. Pedersen , Nicoletta Gnan , Jeppe C. Dyre

Given the right set of circumstances, ultracold quantum gases are able to change character and condense into a liquid state of quantum droplets. The size distribution of the droplets is determined dynamically in the condensation process. A…

Quantum Gases · Physics 2025-05-20 Ian G. Moss

Strongly correlated amorphous solids are a class of glass-formers whose inter-particle potential admits an approximate inverse power-law form in a relevant range of inter-particle distances. We study the steady-state plastic flow of such…

Materials Science · Physics 2015-05-13 Edan Lerner , Itamar Procaccia

We use molecular dynamics simulations in two dimensions to investigate the possibility that a core-softened potential can reproduce static and dynamic anomalies found experimentally in liquid water: (i) the increase in specific volume upon…

Soft Condensed Matter · Physics 2009-10-31 A. Scala , M. Reza Sadr-Lahijany , N. Giovambattista , S. V. Buldyrev , H. E. Stanley

Glass-forming liquids have only a modest tendency to crystallize and hence their dynamics can be studied even below the melting temperature. The relaxation dynamics of most of these liquids shows at a temperature $T_c$, somewhat above the…

Soft Condensed Matter · Physics 2025-01-17 Francesco Rusciano , Raffaele Pastore , Francesco Greco , Walter Kob

Recent analyses of high pressure measurement data suggest that the degree of the dynamic heterogeneity ({\chi}_4)^max cannot be in general a single variable function of the structural relaxation time {\tau}. For a wide class of real and…

The properties of liquid water are known to change drastically in confined geometries. A most interesting and intriguing phenomenon is that the diffusion of water is found to be strongly enhanced by the proximity of a hydrophobic confining…

Soft Condensed Matter · Physics 2024-12-06 Lorenzo Agosta , Kersti Hermansson , Mikhail Dzugutov