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Optical excitations in hexagonal nanonetwork materials, for example, Boron-Nitride (BN) sheets and nanotubes, are investigated theoretically. The bonding of BN systems is positively polarized at the B site, and is negatively polarized at…

Materials Science · Physics 2016-08-31 Kikuo Harigaya

We use resonant soft X-ray diffraction to track the photo-induced dynamics of the antiferromagnetic structure in a NdNiO$_{3}$ thin film. Femtosecond laser pulses with a photon energy of 0.61 eV, resonant with electron transfer between…

We report on the demonstration of a femtosecond all-optical modulator providing, without nonlinearity and therefore at arbitrarily low intensity, ultrafast light-by-light control. The device engages the coherent interaction of optical waves…

Ultrafast manipulation of vibrational coherence is an emergent route to control the structure of solids. However, this strategy can only induce long-range correlations and cannot modify atomic structure locally, which is required in many…

Two-dimensional moir\'e materials are formed by artificially stacking atomically thin monolayers. A wealth of correlated and topological quantum phases can be engineered via precise choice of stacking geometry. These designer electronic…

We carry out first-principles calculations for CaTiO$_3$/BaTiO$_3$ superlattices with epitaxial strain corresponding to growth on a SrTiO$_3$ substrate, and consider octahedral rotations as well as ferroelectric distortions. The…

Materials Science · Physics 2015-05-19 Xifan Wu , Karin M. Rabe , David Vanderbilt

Nanophotonics and metamaterials have revolutionised the way we think about optical space (epsilon, mu), enabling us to engineer the refractive index almost at will, to confine light to the smallest of the volumes, and to manipulate optical…

Heterostructure engineering provides an efficient way to obtain several unconventional phases of LaNiO3, which is otherwise paramagnetic, metallic in bulk form. In this work, a new class of short periodic superlattices, consisting of LaNiO3…

Strongly Correlated Electrons · Physics 2019-10-18 S. Middey , Ranjan Kumar Patel , D. Meyers , Xiaoran Liu , M. Kareev , P. Shafer , J. -W. Kim , P. J. Ryan , J. Chakhalian

The control of optically driven high-frequency strain waves in nanostructured systems is an essential ingredient for the further development of nanophononics. However, broadly applicable experimental means to quantitatively map such…

Instrumentation and Detectors · Physics 2018-01-29 Armin Feist , Nara Rubiano da Silva , Wenxi Liang , Claus Ropers , Sascha Schäfer

The conditions whereby epitaxy is achieved are commonly believed to be mostly governed by misfit strain. We report on a systematic investigation of growth and interface structure of single crystalline tungsten thin films on two different…

The mechanism underlying femtosecond laser pulse induced ultrafast magnetization dynamics remains elusive despite two decades of intense research on this phenomenon. Most experiments focused so far on characterizing magnetization and charge…

We synthesized crystalline films of neodymium nickel oxide (NdNiO3), a perovskite quantum material, switched the films from a metal phase (intrinsic) into an insulator phase (electron-doped) by field-driven lithium-ion intercalation, and…

We fabricated ultrathin ferroelectric/correlated electron oxide heterostructures composed of the ferroelectric Pb(Zr0.2Ti0.8)O3 and the correlated electron oxide (CEO) La0.8Sr0.2MnO3 on SrTiO3 substrates by pulsed laser epitaxy. The hole…

Materials Science · Physics 2012-07-25 Lu Jiang , Woo Seok Choi , Hyoungjeen Jeen , Takeshi Egami , Ho Nyung Lee

Controlling the strain level in nanowire heterostructures is critical for obtaining coherent interfaces of high crystalline quality and for the setting of functional properties such as photon emission, carrier mobility or piezoelectricity.…

Materials Science · Physics 2020-08-05 D. V. Beznasyuk , P. Stepanov , J. L. Rouvière , F. Glas , M. Verheijen , J. Claudon , M. Hocevar

We report the lattice dynamics of transition metal thin films by using the ultrafast electron diffraction. We observe a suppression of the diffraction intensity in a few picosecond after the photoexcitation, which is directly interpreted as…

Materials Science · Physics 2016-01-19 A. Nakamura , T. Shimojima , M. Nakano , Y. Iwasa , K. Ishizaka

Simultaneous measurements of transient transmission and reflectivity were performed in the unintentionally doped InN film to reveal ultrafast optical bleaching and its recovery behavior under intense laser irradiation. The optical bleaching…

Optics · Physics 2021-02-16 Junjun Jia , Takashi Yagi , Toshiki Makimoto

The electronic and magnetic properties of NdNiO$_3$ (NNO) thin films are very sensitive to epitaxial strain and to the proximity to ferromagnetic oxides. In this work, we investigate the structural, electronic, and magnetic properties of…

Materials Science · Physics 2024-09-20 Henrique M. M. Cardoso , Maria C. O. Aguiar , Cinthia Piamonteze , Walber H. Brito

Long regarded as a model system for studying insulator-to-metal phase transitions, the correlated electron material vanadium dioxide (VO$_2$) is now finding novel uses in device applications. Two of its most appealing aspects are its…

Mesoscale and Nanoscale Physics · Physics 2016-04-18 M. A. Huber , M. Plankl , M. Eisele , R. E. Marvel , F. Sandner , T. Korn , C. Schüller , R. F. Haglund, , R. Huber , T. L. Cocker

Using oxide substrates for functional ceramic thin film deposition beyond their usual application as chemical inert, lattice-matched support for the films represents a novel concept in ceramic thin film research. The substrates are applied…

Strongly Correlated Electrons · Physics 2009-11-10 H. -U. Habermeier

We present a direct comparison between resonant terahertz (THz) and nonresonant impulsive stimulated Raman scattering (ISRS) excitation of phonon-polaritons in ferroelectric lithium niobate. THz excitation offers advantages of selectively…

Materials Science · Physics 2017-02-01 Blake S. Dastrup , Jacob R. Hall , Jeremy A. Johnson
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