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Resonant inelastic (Raman) light scattering off neutral GaAs quantum dots which contain a mean number, N=42, of electron-hole pairs is computed. We find Raman amplitudes corresponding to strongly collective final states (charge-density…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Alain Delgado , Augusto Gonzalez , Eduardo Menendez-Proupin

Inelastic light scattering from Dirac-type electrons in graphene is shown to be dominated by the generation of the inter-band electronic modes which are odd in terms of time-inversion symmetry and belong to the irreducible representation…

Mesoscale and Nanoscale Physics · Physics 2010-01-25 Oleksiy Kashuba , Vladimir I. Fal'ko

We exploit the near field enhancement of nano-antennas to investigate the Raman spectra of otherwise not optically detectable carbon nanotubes (CNTs). We demonstrate that a top-down fabrication approach is particularly promising when…

Mesoscale and Nanoscale Physics · Physics 2015-07-01 Nicola Paradiso , Fatemeh Yaghobian , Christoph Lange , Tobias Korn , Christian Schüller , Rupert Huber , Christoph Strunk

The vibrational properties of a series of push-pull polyynes have been studied by infrared and Raman spectroscopy. The simultaneous activation of a strong infrared and Raman mode, i.e. the collective vibration of CC bonds of the sp carbon…

Recent optical absorption/emission experiments showed that the lower energy optical transitions in carbon nanotubes are excitonic in nature, as predicted by theory. These experiments were based on the symmetry aspects of free electron-hole…

Hyper-Raman scattering has been measured on vitreous boron oxide, $v-$B$_2$O$_3$. This spectroscopy, complemented with Raman scattering and infrared absorption, reveals the full set of vibrations that can be observed with light. A mode…

Disordered Systems and Neural Networks · Physics 2009-11-13 G. Simon , B. Hehlen , R. Vacher , E. Courtens

We present a resonance Raman study of the disorder-induced D mode in a sample highly enriched with semiconducting (9,7) single-walled carbon nanotubes in the excitation energy range of 1.49 - 2.05 eV. The intensity of the D mode shows a…

Materials Science · Physics 2015-06-12 Jan Laudenbach , Frank Hennrich , Hagen Telg , Manfred Kappes , Janina Maultzsch

We used tip-enhanced Raman spectroscopy to study the diameter-dependent Raman modes in a contacted carbon nanotube rope. We show that with the near-field tip enhancement a large number of nanotubes within a rope can be identified, even if…

Mesoscale and Nanoscale Physics · Physics 2012-08-30 Karin Goß , Niculina Peica , Christian Thomsen , Janina Maultzsch , Claus M. Schneider , Carola Meyer

In this paper, we investigate the low frequency Raman spectra of multi-wall carbon nanotubes (MWNT) prepared by the electric arc method. Low frequency Raman modes are unambiguously identified on purified samples thanks to the small internal…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. M. Benoit , J. P. Buisson , O. Chauvet , C. Godon , S. Lefrant

We present it ab-initio calculations of the non-resonant Raman spectra of zigzag and armchair BN nanotubes. In comparison, we implement a generalized bond-polarizability model where the parameters are extracted from first-principles…

Materials Science · Physics 2013-08-07 Ludger Wirtz , Michele Lazzeri , Francesco Mauri , Angel Rubio

The vibrational modes of some single wall carbon nanotube (SWNT) intramolecular junctions (IMJs) have been calculated using the newest Brenner reactive empirical bond order (REBO) potential, based upon which their nonresonant Raman spectra…

Mesoscale and Nanoscale Physics · Physics 2007-07-31 Gang Wu , Jinming Dong

Resonance Raman scattering, which probes electrons, phonons and their interplay in crystals, is extensively used in two-dimensional materials. Here we investigate Raman modes in MoSe$_2$ at different laser excitation energies from 2.33 eV…

We study, numerically and analytically, a model of a one-dimensional array of carbon nanotube resonators in a two-terminal configuration. The system is brought into resonance upon application of an AC-signal superimposed on a DC-bias…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 A. Isacsson , J. M. Kinaret

The vibrational spectroscopy of semiconductor nanostructures can provide important information on their structure. In this work, experimental Raman and infrared spectra are compared with vibrational spectra of CdSe/CdS core/shell…

We study the scattering of electromagnetic waves in anisotropic energetic materials. Nonlinear light-matter interactions in molecular crystals result in frequency-conversion and polarization changes. Applied electromagnetic fields of…

Computational Physics · Physics 2016-01-20 M. A. Wood , D. A. R. Dalvit , D. S. Moore

In terms of lattice dynamics theory, we study the vibrational properties of the oxygen-functionalized single wall carbon nanotubes (O-SWCNs). Due to the C-O and O-O interactions, many degenerate phonon modes are split and even some new…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Z. X. Guo , J. W. Ding , Y. Xiao , D. Y. Xing

From resonant Raman scattering on isolated nanotubes we obtained the optical transition energies, the radial breathing mode frequency and Raman intensity of both metallic and semiconducting tubes. We unambiguously assigned the chiral index…

Materials Science · Physics 2009-11-10 H. Telg , J. Maultzsch , S. Reich , F. Hennrich , C. Thomsen

A consistent calculation of resonant inelastic (Raman) scattering amplitudes for relatively large quantum dots, which takes account of valence-band mixing, discrete character of the spectrum in intermediate and final states, and…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez

The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…

Quantum Physics · Physics 2021-10-04 Sho Tamaki , Tomohiro Yokoyama , Hajime Ishihara

The purpose of this work is to calculate the vibrational modes of an elastically anisotropic sphere embedded in an isotropic matrix. This has important application to understanding the spectra of low-frequency Raman scattering from…

Mesoscale and Nanoscale Physics · Physics 2010-09-29 L. Saviot , D. B. Murray , E. Duval , A. Mermet , S. Sirotkin , M. C. Marco de Lucas