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Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the…

Mesoscale and Nanoscale Physics · Physics 2016-01-12 S. Dey , M. Banik , E. Hulkko , K. Rodriguez , V. A. Apkarian , M. Galperin , A. Nitzan

In order to model experimental non-resonant Raman optical activity, chemists must compute a host of second-order response tensors, (e.g. the electric-dipole magnetic-dipole polarizability) and their nuclear derivatives along a set of…

Chemical Physics · Physics 2025-12-12 Zhen Tao , Mansi Bhati , Joseph E. Subotnik

A new group-theory method to relate a spectrum of carbon nanotubes with that of a graphene monolayer is elaborated. The spectrum reconstruction is performed using a virtual intermediate planar periodic structure. Selected irreducible…

Materials Science · Physics 2015-06-05 M. V. Avramenko , S. B. Rochal , Yu. I. Yuzyuk

Using in-situ Raman scattering from phosphorene channel in an electrochemically top-gated field effect transistor, we show that its phonons with A$_g$ symmetry depend much more strongly on concentration of electrons than that of holes,…

Resonantly enhanced Raman scattering in dielectric nanostructures has been recently proven to be an effcient tool for developing nanothermometry and experimental determination of their mode- composition. In this paper, we develop a rigorous…

Optics · Physics 2018-02-14 Kristina Frizyuk , Mehedi Hasan , Alex Krasnok , Andrea Alu , Mihail Petrov

We show that the absorption spectrum in semiconducting nanotubes can be determined using the bosonization technique combined with mean-field theory and a harmonic approximation. Our results indicate that a multiple band semiconducting…

Mesoscale and Nanoscale Physics · Physics 2014-03-13 M. C. Sweeney , J. D. Eaves

We have theoretically investigated electromechanical properties of freely suspended carbon nanotubes when a current is injected into the tubes using a scanning tunneling microscope. We show that a shuttle-like electromechanical instability…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 L. M. Jonsson , L. Y Gorelik , R. I. Shekhter , M. Jonson

High quality InN nanoparticles are grown using atmospheric chemical vapour deposition technique via a self-seeded catalytic approach in the temperature range of 580 to 650 oC. In this temperature region, nucleation barrier of InN is…

Materials Science · Physics 2016-08-24 Kishore K. Madapu , S. R. Polaki , Sandip Dhara

We present a two-step procedure to probe hotspots of plasmon-enhanced Raman scattering with carbon nanotubes. Dielectrophoretic deposition places a small carbon nanotube bundle on top of plasmonic Au nanodimer. After 'pre-characterising'…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Sebastian Heeg , Nick Clark , Aravind Vijayaraghavan

We have performed first-principles calculations to study the lattice vibrational modes and their Raman activities in silicon nanowires (SiNWs). Two types of characteristic vibrational modes are examined: high-frequency optical modes and…

Mesoscale and Nanoscale Physics · Physics 2011-08-30 Li Yang , M. Y. Chou

The recently reported experimental optical spectra of double-walled carbon nanotubes exhibit more peaks than it could be expected based on the layers alone. The appearance of excess peaks has been attributed to the interlayer interaction.…

Mesoscale and Nanoscale Physics · Physics 2020-08-12 Valentin N. Popov

The multi-order Raman scattering is studied up to a fourth order for a detwinned LaMnO_3 crystal. Based on a comprehensive data analysis of the polarisation-dependent Raman spectra, we show that the anomalous features in the multi-order…

We study theoretically the electronic structure, transport and optical properties for a zigzag single-wall carbon nanotube connected to two normal conductor leads under the irradiation of an external electromagnetic field at low…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Wenhu Liao , Guanghui Zhou , Kai-He Ding

We propose and analyse a Raman spectroscopy technique for probing the properties of quantum degenerate bosons in the ground band of an optical lattice. Our formalism describes excitations to higher vibrational bands and is valid for deep…

Other Condensed Matter · Physics 2009-11-11 P. Blair Blakie

We calculate low-frequency Raman scattering from the confined acoustic phonon modes of CdS1-xSex nanoparticles embedded in borosilicate glass. The calculation of the Raman scattering by acoustic phonons in nanoparticles has been performed…

Mesoscale and Nanoscale Physics · Physics 2009-04-16 Sanjeev K. Gupta , Prafulla K. Jha , Satyaprakash Sahoo , A. K. Arora , Y. M. Azhniuk

A semiclassical model is used to investigate the possibility of selectively exciting one of two closely spaced, uncoupled Raman transitions. The duration of the intense pump pulse that creates the Raman coherence is shorter than the…

Chemical Physics · Physics 2009-11-10 S. A. Malinovskaya , P. H. Bucksbaum , P. R. Berman

We present a Raman spectroscopy study of iodine-intercalated (p-type-doped) double-walled carbon nanotubes. Double-walled carbon nanotubes (DWCNTs) are synthesized by catalytic chemical vapor deposition and characterized by Raman…

We present a first-principles study on lattice vibrational modes of Si/Ge core-shell nanowires (NWs). In addition to quantum confinement, the internal strain induced by the lattice mismatch between core and shell contributes to significant…

Mesoscale and Nanoscale Physics · Physics 2012-07-04 Shouting Huang , Li Yang

Carbyne, i.e. an infinitely long linear carbon chain (LCC), has been at the focus of a lot of research for quite a while, yet its optical, electronic, and vibrational properties have only recently started to become accessible experimentally…

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…

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