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Organic solar cells have the potential for widespread usage due to their promise of low cost, roll-to-roll manufacturability, and mechanical flexibility. However, deployment is impeded by their relatively low power conversion efficiencies.…

Materials Science · Physics 2015-03-19 Olga Wodo , Srikanta Tirthapura , Sumit Chaudhary , Baskar Ganapathysubramanian

Polymer based organic photovoltaic (OPV) technology offers a relatively inexpensive option for solar energy conversion provided its efficiency increases beyond the current level (6-7%) along with significant improvements in operational…

Materials Science · Physics 2015-03-17 Biswajit Ray , Pradeep R. Nair , Muhammad A. Alam

In numerous solution-processed thin films, a complex morphology resulting from liquid-liquid phase separation (LLPS) or from polycrystallization arises during the drying or subsequent processing steps. The morphology has a strong influence…

Applied Physics · Physics 2022-06-28 Olivier J. J. Ronsin , Jens Harting

Film formation from solvent evaporation in polymer ternary solutions is relevant for several technological applications, such as the fabrication of organic solar cells. The performance of the final device will strongly depend on the…

Soft Condensed Matter · Physics 2025-03-18 Emilio N. M. Cirillo , Nicklas Jävergård , Rainey Lyons , A. Muntean , S. A. Muntean

The performance of solution-processed solar cells strongly depends on the geometrical structure and roughness of the photovoltaic layers formed during film drying. During the drying process, the interplay of crystallization and…

We develop a mesoscopic lattice model to study the morphology formation in interacting ternary mixtures with evaporation of one component. As concrete application of our model, we wish to capture morphologies as they are typically arising…

Understanding the morphology formation process of solution-cast photoactive layers (PALs) is crucial to derive design rules for optimized and reliable third generation solar cell fabrication. For this purpose, a Phase-Field (PF)…

Materials Science · Physics 2023-10-19 Maxime Siber , Olivier J. J. Ronsin , Jens Harting

We use a Convolutional Recurrent Neural Network approach to learn morphological evolution driven by surface diffusion. To this aim we first produce a training set using phase field simulations. Intentionally, we insert in such a set only…

Computational Physics · Physics 2024-05-07 Daniele Lanzoni , Marco Albani , Roberto Bergamaschini , Francesco Montalenti

Understanding the relationship between morphology and performance in organic solar cells is essential for developing devices that are both high performing and resilient to aging. This work introduces a unique method capable of calculating…

Materials Science · Physics 2026-05-20 Yasin Ameslon , Larry Lüer , Jens Harting , Olga Wodo , Olivier J. J. Ronsin

We present a model for the morphology evolution of printed organic solar cells which occurs during the drying of a mixture of polymer, the non-fullerene acceptor and the solvent. Our model uses a phase field approach coupled to a…

Numerical Analysis · Mathematics 2026-01-26 Pelin Çiloğlu , Carmen Tretmans , Roland Herzog , Jan-F. Pietschmann , Martin Stoll

We study a nonlinear coupled parabolic system with non-local drift terms modeling at the continuum level the inter-species interaction within a ternary mixture that allows the evaporation of one of the species. In the absence of…

Analysis of PDEs · Mathematics 2023-11-17 Rainey Lyons , Emilio N. M. Cirillo , Adrian Muntean

Solvent evaporation in soft matter solutions (solutions of colloidal particles, polymers and their mixtures) is an important process in material making and in printing and coating industries. The solvent evaporation process determines the…

Soft Condensed Matter · Physics 2018-01-11 Jiajia Zhou , Xingkun Man , Ying Jiang , Masao Doi

Tailoring the nanomorphology of organic photoactive layers through a specialized chain of processing steps is an imperative challenge on the path towards reliable and performant organic electronic manufacturing. This hurdle generally proves…

Materials Science · Physics 2025-12-19 Maxime Siber , Olivier J. J. Ronsin , Gitti L. Frey , Jens Harting

The evaporation of droplets occurs in a large variety of natural and technological processes such as medical diagnostics, agriculture, food industry, printing, and catalytic reactions. We study the different droplet morphologies adopted by…

Soft Condensed Matter · Physics 2020-02-11 Jose M. Encarnacion Escobar , Diana Garcia-Gonzalez , Ivan Devic , Xuehua Zhang , Detlef Lohse

A machine learning approach is presented to accelerate the computation of block polymer morphology evolution for large domains over long timescales. The strategy exploits the separation of characteristic times between coarse-grained…

Chemical Physics · Physics 2023-09-01 Hyun Park , Boyuan Yu , Juhae Park , Ge Sun , Emad Tajkhorshid , Juan J. de Pablo , Ludwig Schneider

The active layer in a perovskite solar cell is usually composed of a polycrystalline thin film. Fabrication of this layer by solution processing is a promising candidate for up-scaling to the mass market. However, the evolution of an…

Materials Science · Physics 2025-09-05 M. Majewski , O. J. J. Ronsin , J. Harting

Mollusk shells are an ideal model system for understanding the morpho-elastic basis of morphological evolution of invertebrates' exoskeletons. During the formation of the shell, the mantle tissue secretes proteins and minerals that calcify…

Quantitative Methods · Quantitative Biology 2019-08-12 Shiva Rudraraju , Derek E. Moulton , Régis Chirat , Alain Goriely , Krishna Garikipati

Modeling the spontaneous evolution of morphology in natural systems and its preservation by proportionate growth remains a major scientific challenge. Yet, it is conceivable that if the basic mechanisms of growth and the coupled kinetic…

Soft Condensed Matter · Physics 2020-12-30 Virginia von Streng , Rami Abi-Akl , Bianca Giovanardi , Tal Cohen

The internal structure of adhesive tapes determines the effective mechanical properties. This holds true especially for blended systems, here consisting of acrylate and rubber phases. In this note, we propose a lattice-based model to study…

Soft Condensed Matter · Physics 2023-05-30 Vi Cecilia Erik Kronberg , Stela Andrea Muntean , Nils Hendrik Kröger , Adrian Muntean

A computer simulation is used to predict the effects of membrane morphology on the thermal efficiency of direct contact membrane distillation. The mass transfer through the porous microstructure and the heat conduction through the membrane…

Computational Physics · Physics 2019-03-06 Gavin A. Buxton
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