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We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

Strongly Correlated Electrons · Physics 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd$_2$Zr$_2$O$_7$ by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out"…

Strongly Correlated Electrons · Physics 2021-07-22 M. Léger , E. Lhotel , M. Ciomaga Hatnean , J. Ollivier , A. R. Wildes , S. Raymond , E. Ressouche , G. Balakrishnan , S. Petit

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

Strongly Correlated Electrons · Physics 2022-04-06 Sheetal , C. S. Yadav

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

Using neutron diffraction, 170Yb Mossbauer and muSR spectroscopies, we have examined the pyrochlore Yb2Ti2O7 where the Yb3+ S'=1/2 ground state has planar anisotropy. Below ~0.24K, the temperature of the known specific heat lambda…

We report the X-ray study for the pyrochlore oxide Cd2Re2O7. Two symmetry-lowering structural transitions were observed at Ts1=200K and Ts2=120K. The former is of the second order from the ideal cubic pyrochlore structure with space group…

Strongly Correlated Electrons · Physics 2009-11-07 Jun-Ichi Yamaura , Zenji Hiroi

Recent neutron scattering and specific heat studies on the pyrochlore Yb2Ti2O7 have revealed variations in its magnetic behavior below 265mK. In the best samples, a sharp anomaly in the specific heat is observed at T=265mK. Other samples,…

Strongly Correlated Electrons · Physics 2013-02-01 K. A. Ross , Th. Proffen , H. A. Dabkowska , J. A. Quilliam , L. R. Yaraskavitch , J. B. Kycia , B. D. Gaulin

Intensity distribution of the neutron magnetic scattering has been taken in the reciprocal space of a single crystal of the "spin ice" system Ho2Ti2O7 at the elastic energy position in the temperature (T) region between 0.4 K and 50 K. The…

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Remarkably, the spin ices provide one of very few…

Strongly Correlated Electrons · Physics 2014-07-29 Michel J. P. Gingras , Paul A. McClarty

By measurements of specific heat, we have investigated the magnetic field ($H$) induced spin-structural change in Nd$_2$Mo$_2$O$_7$ that shows spin-chirality-related magneto-transport phenomena. A broad peak around 2 K caused by the…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Onose , Y. Taguchi , T. Ito , Y. Tokura

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

We have investigated the kagom\'{e} ice behavior of the dipolar spin-ice compound Dy_{2}Ti_{2}O_{7} in magnetic field along a [111] direction using neutron scattering and Monte Carlo simulations. The spin correlations show that the…

Disordered Systems and Neural Networks · Physics 2007-05-23 Y. Tabata , H. Kadowaki , K. Matsuhira , Z. Hiroi , N. Aso , E. Ressouche , B. Fak

The spin glass behavior of Y2Mo2O7 has puzzled physicists for nearly three decades. Free of bulk disorder within the resolution of powder diffraction methods, it is thought that this material is a rare realization of a spin glass resulting…

In this work, we show that the zero field excitation spectra in the quantum spin ice candidate pyrochlore compound \ybti\ is a continuum characterized by a very broad and almost flat dynamical response which extends up to $1-1.5$ meV,…

Strongly Correlated Electrons · Physics 2015-09-30 J. Robert , E. Lhotel , G. Remenyi , S. Sahling , I. Mirebeau , C. Decorse , B. Canals , S. Petit

Neutron scattering from high-quality YBa2Cu3O6.33 (YBCO6.33) single crystals with a Tc of 8.4 K shows no evidence of a coexistence of superconductivity with long-range antiferromagnetic order at this very low, near-critical doping of…

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

Spin correlations in the pyrochlore antiferromagnet Y_2Ru_2O_7 with Curie-Weiss temperature $\Theta_{CW}=-1100$ K and critical temperature T_N=77 K were examined through neutron scattering. For $T_N<T<\Theta_{CW}/3$ the data show spin…

Strongly Correlated Electrons · Physics 2014-07-03 J. van Duijn , N. Hur , J. W. Taylor , Y. Qiu , Q. Z. Huang , S. -W. Cheong , C. Broholm , T. G. Perring