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A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

We study ultrafast population dynamics in the topological surface state of Sb$_2$Te$_3$ in two-dimensional momentum space with time- and angle-resolved two-photon photoemission. Linear polarized mid-infrared pump pulses are used to permit a…

Mesoscale and Nanoscale Physics · Physics 2023-04-26 J. Reimann , K. Sumida , M. Kakoki , K. A. Kokh , O. E. Tereshchenko , A. Kimura , J. Güdde , U. Höfer

Motivated by the recent rapid development of the field of quantum gases in optical lattices, we present a comprehensive study of the spectrum of ultracold atoms in a one-dimensional optical lattice subjected to a periodic lattice…

Quantum Gases · Physics 2011-10-11 Jia-Wei Huo , Fu-Chun Zhang , Weiqiang Chen , M. Troyer , U. Schollwöck

We investigate the effect of far-off-resonant trapping light on ultracold bosonic RbCs molecules. We use kHz-precision microwave spectroscopy to measure the differential AC Stark shifts between the ground and first excited rotational levels…

We study theoretically the quantum dynamics and spectroscopy of rovibrational polaritons formed in a model system composed of a single rovibrating diatomic molecule, which interacts with two degenerate, orthogonally polarized modes of an…

Chemical Physics · Physics 2023-01-11 Eric W. Fischer , Peter Saalfrank

Ultracold molecules offer entirely new possibilities for the control of quantum processes due to their rich internal structure. Recently, near quantum degenerate gases of molecules have been prepared in their rovibronic ground state. For…

Atomic Physics · Physics 2015-05-14 S. Ospelkaus , K. -K. Ni , G. Quemener , B. Neyenhuis , D. Wang , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

The population dynamics of a trapped Bose-Einstein condensate, subject to the action of an oscillatory field, is studied. This field produces a modulation of the trapping potential with the frequency close to the transition frequency…

Condensed Matter · Physics 2007-05-23 V. I. Yukalov , E. P. Yukalova , V. S. Bagnato

We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…

Atomic Physics · Physics 2026-01-14 Emanuel F. de Lima

We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…

Chemical Physics · Physics 2010-06-30 Xin Tong , Alexander H. Winney , Stefan Willitsch

Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…

Bare-state population inversion is demonstrated in a two-level system with all dipole matrix elements nonzero. A laser field is resonantly driving the sample whereas a second weaker and lower frequency coherent field additionally pumps it…

Quantum Physics · Physics 2015-07-31 Mihai Macovei , Mayank Mishra , Christoph H. Keitel

We demonstrate the direct formation of vibronic ground state RbCs molecules by photoassociation of ultracold atoms followed by radiative stabilization. The photoassociation proceeds through deeply-bound levels of the (2)^{3}\Pi_{0^{+}}…

Atomic Physics · Physics 2015-06-16 C. D. Bruzewicz , Mattias Gustavsson , Toshihiko Shimasaki , D. DeMille

We investigate magic-wavelength trapping of ultracold bialkali molecules in the vicinity of weak optical transitions from the vibrational ground state of the X$^1\Sigma^+$ potential to low-lying rovibrational states of the b$^3\Pi_0$…

Quantum Physics · Physics 2021-04-14 Q. Guan , S. L. Cornish , S. Kotochigova

The recent experimental realization of cold polar molecules in the rotational and vibrational ground state opens the door to the study of a wealth of phenomena involving long-range interactions. By applying an optical lattice to a gas of…

Quantum Gases · Physics 2015-03-13 J. R. Armstrong , N. T. Zinner , D. V. Fedorov , A. S. Jensen

We study theoretically the collective dynamics of rotational excitations of polar molecules loaded into an optical lattice in two dimensions. These excitations behave as hard-core bosons with a relativistic energy dispersion arising from…

Quantum Gases · Physics 2014-08-29 M. P. Kwasigroch , N. R. Cooper

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical…

Quantum Gases · Physics 2025-01-16 Siwei Zhang , Weijun Yuan , Niccolò Bigagli , Claire Warner , Ian Stevenson , Sebastian Will

We report here on the production of an ultracold gas of tightly bound Rb2 molecules in the ro-vibrational triplet ground state, close to quantum degeneracy. This is achieved by optically transferring weakly bound Rb2 molecules to the…

Quantum Physics · Physics 2009-11-13 F. Lang , K. Winkler , C. Strauss , R. Grimm , J. Hecker Denschlag

Recently, systems with strong coupling between electronic and vibrational degrees of freedom attract a great attention. In this work, we consider the transient dynamics of the system consisting of strongly coupled vibron and exciton driven…

Quantum Physics · Physics 2023-08-09 E. A. Tereshchenkov , V. Yu. Shishkov , E. S. Andrianov

The observation of significant dipolar effects in gases of ultra-cold polar molecules typically demands a strong external electric field to polarize the molecules. We show that even in the absence of a significant polarization, dipolar…

Quantum Gases · Physics 2011-12-20 A. Pikovski , M. Klawunn , A. Recati , L. Santos

Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…

Quantum Physics · Physics 2011-01-04 Svetlana Kotochigova , David DeMille