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We propose a new mechanism to produce ultracold polar molecules with microwave fields. The proposed mechanism converts trapped ultracold atoms of different species into vibrationally excited molecules by a single microwave transition and…

Quantum Physics · Physics 2009-11-13 Svetlana Kotochigova

We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where…

Atomic Physics · Physics 2012-11-13 I. Manai , R. Horchani , H. Lignier , A. Fioretti , M. Allegrini , P. Pillet , D. Comparat

We determine trapping conditions for ultracold polar molecules, where pairs of internal states experience identical trapping potentials. Such conditions could ensure that detrimental effects of inevitable inhomogeneities across an ultracold…

Atomic Physics · Physics 2015-06-12 Alexander Petrov , Constantinos Makrides , Svetlana Kotochigova

Population dynamics in weakly-excited clouds of ultracold $^{87}$Rb Rydberg atoms were studied by means of trap loss, fluorescence detection, and state dependent stimulated emission. Rydberg atoms were excited to various nl Rydberg states…

Quantum Physics · Physics 2009-11-13 J. O. Day , E. Brekke , T. G. Walker

We study a simple model consisting of an atomic ion and a polar molecule trapped in a single setup, taking into consideration their electrostatic interaction. We determine analytically their collective modes of excitation as a function of…

Atomic Physics · Physics 2016-08-11 Jordi Mur-Petit , Juan José García-Ripoll

We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…

Atomic Physics · Physics 2008-10-28 Christiane P. Koch , Robert Moszynski

Ultracold polar molecules trapped on an optical lattice is a many-body system that, under appropriate conditions, may support collective excitations reminiscent of excitons in solid state crystals. Here, we discuss the rotational…

Atomic Physics · Physics 2017-08-23 Marina Litinskaya , Roman V. Krems

We investigate cooperative phenomena and superradiance for vibrational transitions in polar molecule spectroscopy when a high optical-depth (OD) sample is studied. Such cooperativity comes from the build-up of inter-particle coherence…

Atomic Physics · Physics 2015-06-15 Guin-Dar Lin , Susanne F. Yelin

We discuss the production of ultracold molecules in their electronic ground state by photoassociation employing electronically excited states with ion-pair character and strong spin-orbit interaction. A short photoassociation laser pulse…

We theoretically investigate how population can be trapped in the excited doublet in presence of vacuum-induced coherence (VIC). We employ delayed pulses to transfer population from a metastable state to the excited states. Subsequently,…

Quantum Physics · Physics 2018-02-14 Babu Lal Kumawat , Pardeep Kumar , Shubhrangshu Dasgupta

The transfer of weakly bound KRb molecules from levels just below the dissociation threshold into the vibrational ground state with shaped laser pulses is studied. Optimal control theory is employed to calculate the pulses. The complexity…

Atomic Physics · Physics 2011-04-15 Mamadou Ndong , Christiane P. Koch

We produce ultracold dense trapped samples of 87Rb133Cs molecules in their rovibrational ground state, with full nuclear hyperfine state control, by stimulated Raman adiabatic passage (STIRAP) with efficiencies of 90%. We observe the onset…

Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…

We propose a method for achieving highly efficient transfer between the vibrational states in a diatomic molecule. The process is mediated by strong laser pulses and can be understood in terms of light-induced potentials. In addition to…

Quantum Physics · Physics 2009-11-06 M. Rodriguez , K. -A. Suominen , B. M. Garraway

We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…

Quantum Gases · Physics 2012-05-15 Sebastian D. Huber , Hans Peter Büchler

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

We consider the effect of the long range dipole-dipole interaction on the excitation exchange dynamics of cold two-level atomic gase in the conditions where the size of the atomic cloud is large as compared to the wavelength of the dipole…

Quantum Physics · Physics 2015-05-13 A. Mandilara , V. M. Akulin , P. Pillet

Ultra-cold RbCs molecules in high-lying vibrational levels of the a$^3\Sigma^+$ ground electronic state are confined in an optical trap. Inelastic collision rates of these molecules with both Rb and Cs atoms are determined for individual…

We demonstrate efficient transfer of ultracold molecules into a deeply bound rovibrational level of the singlet ground state potential in the presence of an optical lattice. The overall molecule creation efficiency is 25%, and the transfer…

Molecular hydrogen ions in weakly bound states close to the first dissociation threshold are attractive quantum sensors for measuring the proton-to-electron mass ratio and hyperfine-induced ortho-para mixing. The experimental accuracy of…

Atomic Physics · Physics 2022-09-23 A. D. Ochoa Franco , M. Beyer