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We study the nonequilibrium dynamics of photoexcited electrons in the narrow-gap Mott insulator VO$_2$. The initial stages of relaxation are treated using a quantum Boltzmann equation methodology, which reveals a rapid ($\sim$ femtosecond…

Strongly Correlated Electrons · Physics 2016-03-23 Zhuoran He , Andrew J. Millis

We present a density-matrix embedding theory (DMET) study of the one-dimensional Hubbard-Holstein model, which is paradigmatic for the interplay of electron-electron and electron-phonon interactions. Analyzing the single-particle excitation…

Charge-transfer (CT) exciton effects are investigated for the optical absorption spectra of crosslinked C60 systems by using the intermediate exciton theory. We consider the C60-dimers, and the two (and three) molecule systems of the…

chem-ph · Physics 2008-02-03 K. Harigaya

The high flexibility of organic molecules offers great potential for designing the optical properties of light-active materials for the next generation of optoelectronic and photonic applications. However, despite successful implementations…

Employing the density-matrix renormalization group technique in the matrix-product-state representation, we investigate the photoexcited superconducting correlations induced by the $\eta$-pairing mechanism in the half-filled Hubbard chain.…

Strongly Correlated Electrons · Physics 2020-04-22 Satoshi Ejima , Tatsuya Kaneko , Florian Lange , Seiji Yunoki , Holger Fehske

We present a model for Desorption Induce by (Multiple) Electronic Transitions (DIET/DIMET) based on potential energy surfaces calculated with the Delta Self-Consistent Field extension of Density Functional Theory. We calculate potential…

Chemical Physics · Physics 2009-11-13 Thomas Olsen , Jeppe Gavnholt , Jakob Schiøtz

We study the optical response of a binary system of identical atoms in which one of them is excited by an incoherent pump. %We study the properties of photon scattering, absorption and emission, together with the time evolution of the…

Quantum Physics · Physics 2025-06-27 L. Acevedo , J. Sánchez-Cánovas , M. Donaire

Photo-doping of Mott insulators or correlated metals can create an unusual metallic state which simultaneously hosts hole-like and electron-like particles. We study the dynamics of this state up to long times, as it passes its kinetic…

Strongly Correlated Electrons · Physics 2021-05-26 Nagamalleswararao Dasari , Jiajun Li , Philipp Werner , Martin Eckstein

The Mott transistor is a paradigm for a new class of electronic devices---often referred to by the term Mottronics---, which are based on charge correlations between the electrons. Since correlation-induced insulating phases of most oxide…

Motivated by recent experimental studies of hydrogen-bonded molecular conductors $\kappa$-$X_3$(Cat-EDT-TTF)$_2$ [$X$=H, D], interplays of protons and correlated electrons, and their effects on magnetic, dielectric, and optical properties,…

Strongly Correlated Electrons · Physics 2018-06-13 Makoto Naka , Sumio Ishihara

Charge dynamics in a dimer Mott insulating system, where a non-polar dimer-Mott (DM) phase and a polar charge-ordered (CO) phase compete with each other, are studied. In particular, collective charge excitations are analyzed in the three…

Strongly Correlated Electrons · Physics 2015-06-11 Makoto Naka , Sumio Ishihara

The correlation-driven metal-insulator (Mott) transition at a solid surface is studied within the Hubbard model for a semi-infinite lattice by means of the dynamical mean-field theory. The transition takes place at a unique critical…

Strongly Correlated Electrons · Physics 2009-10-31 M. Potthoff , W. Nolting

In this work, we investigate the photoionization cross-section of an electron confined in a quantum dot, considering the position-dependent variation of the effective mass through the parameter $\gamma$. We used a theoretical model based on…

The temperature ($T$) dependent metal-insulator transition (MIT) in VO$_2$ is investigated using bulk sensitive hard x-ray ($\sim$ 8 keV) valence band, core level, and V 2$p-3d$ resonant photoemission spectroscopy (PES). The valence band…

In Peierls-distorted materials, photoexcitation leads to a strongly coupled transient response between structural and electronic degrees of freedom, always measured independently of each other. Here we use transient reflectivity in the…

Interacting many-body systems combining confined and extended dimensions, such as ladders and few layer systems are characterized by enhanced quantum fluctuations, which often result in interesting collective properties. Recently…

Strongly Correlated Electrons · Physics 2022-06-29 Annabelle Bohrdt , Lukas Homeier , Immanuel Bloch , Eugene Demler , Fabian Grusdt

The superfluid-insulator transitions of the fermionic atoms in optical lattices are investigated by the two-site dynamical mean-field theory. It is shown that the Mott transition occurs as a result of the multiband effects. The…

Other Condensed Matter · Physics 2009-11-13 Takuji Higashiyama , Kensuke Inaba , Sei-ichiro Suga

The problem of screening the Coulomb interaction between charge carriers in type II heterostructures based on transition metal dichalcogenides is Analytically solved. At a sufficiently high density of charge carriers, the density dependence…

Mesoscale and Nanoscale Physics · Physics 2022-05-11 Pavel V. Ratnikov

The physics of doping a Mott insulator is investigated in the presence of a solid-vacuum interface. Using the embedding approach for dynamical mean field theory we show that the change in surface spectral evolution in a doped Mott insulator…

Strongly Correlated Electrons · Physics 2011-07-12 Reza Nourafkan , Frank Marsiglio

We investigate the dynamics of correlated charge carriers in the vicinity of the Mott metal-to-insulator transition in various of the title quasi-two-dimensional organic charge-transfer salts by means of fluctuation (noise) spectroscopy.…

Strongly Correlated Electrons · Physics 2015-03-19 Jens Brandenburg , Jens Müller , Dieter Schweitzer , John A. Schlueter