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Engineering and harnessing coherent excitonic transport in organic nanostructures has recently been suggested as a promising way towards improving man-made light harvesting materials. However, realising and testing the dissipative…

Quantum Physics · Physics 2018-06-19 A. W. Chin , E. Mangaud , O. Atabek , M. Desouter-Lecomte

The spin echo approach is extended to include bio-complexes for which the interaction with dynamical noise is strong. Significant restoration of the free induction decay signal due to homogeneous (decoherence) and inhomogeneous (dephasing)…

Biological Physics · Physics 2015-05-13 Alexander I. Nesterov , Gennady P. Berman

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery

Excitonic transport in photosynthesis exhibits a wide range of time scales. Absorption and initial relaxation takes place over tens of femtoseconds. Excitonic lifetimes are on the order of a nanosecond. Hopping rates, energy differences…

Quantum Physics · Physics 2011-11-22 Seth Lloyd , Masoud Mohseni , Alireza Shabani , Herschel Rabitz

The recent accessibility of high quality, charge neutral monolayer transition metal dichalcogenides with narrow exciton linewidths at the homogeneous limit provides an ideal platform to study excitonic many-body interactions. In particular,…

The molecular photo cell, i.e., a single molecule donor-acceptor complex, beside being technologically important, is a paradigmatic example of a many-body system operating in strong non-equilibrium. The quantum transport and the…

Mesoscale and Nanoscale Physics · Physics 2020-07-06 Subhajit Sarkar , Yonatan Dubi

Transport phenomena in organic, self-assembled molecular J-aggregates have long attracted a great deal of attention due to its potential role in designing novel organic photovoltaic devices. A large number of theoretical and experimental…

Chemical Physics · Physics 2020-02-21 Luis Felipe Morales-Curiel , Roberto de J. León-Montiel

Photosystem I is a protein-pigment complex that performs photosynthesis in plants, green algae, and cyanobacteria. It contains an aggregate of chlorophylls that absorbs light and delivers the resulting electronic excitation to the special…

Biological Physics · Physics 2007-05-23 Sanghyun Park , Melih K. Sener , Deyu Lu , Klaus Schulten

We expose a new excitation transport channel in FMO, consisting of the 7 intramonomeric pigments and their 2nd nearest intermonomeric counterpart. Such a channel outcompetes the standard alternative, where intramonomeric pigments partner…

Chemical Physics · Physics 2022-01-13 Daniel López Díaz , Gabriel Gil , Augusto González

The strong coherent coupling of quantum emitters to vacuum fluctuations of the light field offers opportunities for manipulating the optical and transport properties of nanomaterials, with potential applications ranging from ultrasensitive…

Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why…

Quantum Physics · Physics 2022-09-14 S. Ali Hassani Gangaraj , Lei Ying , Francesco Monticone , Zongfu Yu

Excitation transfer through interacting systems plays an important role in many areas of physics, chemistry, and biology. The uncontrollable interaction of the transmission network with a noisy environment is usually assumed to deteriorate…

Quantum Physics · Physics 2009-09-12 Filippo Caruso , Alex W. Chin , Animesh Datta , Susana F. Huelga , Martin B. Plenio

A mass transport directed from low to high density region in an inhomogeneous medium is modeled as a limiting case of a two-component lattice gas with excluded volume constraint and one of the components fixed. In the long-wavelength…

Disordered Systems and Neural Networks · Physics 2012-10-05 Sergei P. Lukyanets , Oleksandr V. Kliushnychenko

Employing tight-binding approximation we derive a transfer matrix formalism for one-dimensional single photon transport through a composite scattering center, which consists of parallel connected resonator optical waveguides. By solving the…

Quantum Physics · Physics 2017-03-29 Yu Jiang , M. Lozada-Cassou

We examine the dynamics of entanglement entropy of all parts in an open system consisting of a two-level dimer interacting with an environment of oscillators. The dimer-environment interaction is almost energy conserving. We find the…

Quantum Physics · Physics 2018-05-09 M. Merkli , G. P. Berman , R. T. Sayre , X. Wang , A. I. Nesterov

Lead halide perovskites show remarkable performance when used in photovoltaic and optoelectronic devices. However, the peculiarities of light-matter interactions in these materials in general are far from being fully explored experimentally…

Other Condensed Matter · Physics 2022-02-24 A. V. Trifonov , S. Grisard , A. N. Kosarev , I. A. Akimov , D. R. Yakovlev , J. Höcker , V. Dyakonov , M. Bayer

Although coherent light is usually required for the self-organization of regular spatial patterns from optical beams, we show that peculiar light matter interaction can break this evidence. In the traditional method to record laser-induced…

Quantum interference between one- and two-photon absorption pathways allows coherent control of interband transitions in unbiased bulk semiconductors; carrier population, carrier spin polarization, photocurrent injection, and spin current…

Other Condensed Matter · Physics 2007-05-23 R. D. R. Bhat , J. E. Sipe

We discuss our recent theoretical work on vibronic coupling mechanisms in a model energy transfer system in the context of previous 2DEV experiments on a natural light-harvesting system, light-harvesting complex II (LHCII), where vibronic…

Chemical Physics · Physics 2021-09-22 Eric A. Arsenault , Addison J. Schile , David T. Limmer , Graham R. Fleming

Exciton transfer along a polymer is essential for many biological processes, for instance light harvesting in photosynthetic biosystems. Here we apply a new witness of non-classicality to this phenomenon, to conclude that, if an exciton can…

Quantum Physics · Physics 2024-09-12 Giuseppe Di Pietra , Vlatko Vedral , Chiara Marletto