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Giant strides in ultrashort laser pulse technology have enabled real-time observation of dynamical processes in complex molecular systems. Specifically, the discovery of oscillatory transients in the two-dimensional electronic spectra of…

Chemical Physics · Physics 2021-03-08 Akihito Ishizaki , Graham R. Fleming

The synchronization of charge oscillations after photoexcitation that has been realized through the emergence of an electronic breathing mode on dimer lattices is studied here from the viewpoint of the competition between interactions and…

Strongly Correlated Electrons · Physics 2020-07-03 Toshiya Shimada , Kenji Yonemitsu

We develop a theory of polarized photoluminescence of interface excitons localized at lateral heterojunctions between transition metal dichalcogenide monolayers. We show that the circular selection rules governing interband optical…

Mesoscale and Nanoscale Physics · Physics 2026-03-26 M. V. Durnev , D. S. Smirnov

One-particle interchain hopping in a system of coupled Luttinger liquids is investigated by use of exact diagonalizations techniques. Firstly, the two chain problem of spinless fermions is studied in order to see the behaviour of the band…

Strongly Correlated Electrons · Physics 2009-10-30 S. Capponi , D. Poilblanc

We study effects of relaxation/decoherence processes on quantum transport of non-interacting Fermi particles across the tight-binding chain, where we distinguish between relaxation processes in the contacts (external decoherence) and those…

Mesoscale and Nanoscale Physics · Physics 2024-07-11 Andrey R. Kolovsky

We present a study on the evolution of the Fenna-Matthews-Olson bacterial photosynthetic pigment-protein complex. This protein complex functions as an antenna. It transports absorbed photons - excitons - to a reaction center where…

In this work, we theoretically investigate the optical orientation and alignment of excitons in quantum dots with weak electron-hole exchange interaction and long exciton radiative lifetimes. This particular regime is realized in…

Mesoscale and Nanoscale Physics · Physics 2023-08-30 D. S. Smirnov , E. L. Ivchenko

We discuss coherent exciton-polariton states in long molecular chains that are formed due to the interaction of molecular excitations with both vacuum photons and surface excitations of the neighboring reflecting substrate. The resonance…

Other Condensed Matter · Physics 2009-11-13 Yu. N. Gartstein , V. M. Agranovich

We present photoluminescence measurements in monolayer WSe$_2$, which point to the importance of the interaction between charged particles and excitonic complexes. The theoretical analysis highlights the key role played by exchange…

Materials Science · Physics 2022-02-15 Min Yang , Lei Ren , Cedric Robert , Dinh Van Tuan , Laurent Lombez , Bernhard Urbaszek , Xavier Marie , Hanan Dery

We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron and electron-phonon interactions, and captures exciton formation as well as the transition…

Materials Science · Physics 2025-02-13 Zhenlin Zhang , Wei Hu , Enrico Perfetto , Gianluca Stefanucci

Transport phenomena at the nanoscale are of interest due to the presence of both quantum and classical behavior. In this work, we demonstrate that quantum transport efficiency can be enhanced by a dynamical interplay of the system…

Quantum Physics · Physics 2009-05-22 Patrick Rebentrost , Masoud Mohseni , Ivan Kassal , Seth Lloyd , Alán Aspuru-Guzik

Energy transfer between chromophores in photosynthesis proceeds with near unity quantum efficiency. Understanding the precise mechanisms of these processes is made difficult by the complexity of the electronic structure and interactions…

Chemical Physics · Physics 2015-03-03 Gethin H. Richards , Krystyna E. Wilk , Paul M. G. Curmi , Jeffrey A. Davis

The idea that excitonic state (electronic) coherences are of fundamental importance to natural photosynthesis gained popularity when, a decade ago, slowly dephasing quantum beats were observed in the two-dimensional electronic spectra of…

We show that finite-size, disordered molecular networks can mediate highly efficient, coherent excitation transfer which is robust against ambient dephasing and associated with strong multi-site entanglement. Such optimal, random molecular…

Light-harvesting and excitation energy transfer in photosynthesis generally involve chlorophyll-molecules, maintained by their host proteins at short distances from each other, this resulting in excitonic coupling. The transfer of…

We investigate the role of quantum coherence in modulating the energy transfer rate between two independent energy donors and a single acceptor participating in an excitonic energy transfer process. The energy transfer rate depends…

Chemical Physics · Physics 2015-07-13 Sreenath K. Manikandan , Anil Shaji

In superlattices of twisted semiconductor monolayers, tunable moir\'e potentials emerge, trapping excitons into periodic arrays. In particular, spatially separated interlayer excitons are subject to a deep potential landscape and they…

Mesoscale and Nanoscale Physics · Physics 2023-06-02 Samuel Brem , Ermin Malic

We employ five {\pi}-conjugated model materials of different molecular shape --- oligomers and cyclic structures --- to investigate the extent of exciton self-trapping and torsional motion of the molecular framework following optical…

Equations of motion for weakly coupled excitonic complexes are derived. The description allows to treat the system in the basis of electronic states localized on individual chromophores, while at the same time accounting for experimentally…

Chemical Physics · Physics 2012-01-30 Tomas Mancal , Vytautas Balevicius , Leonas Valkunas

Understanding the transport mechanism of electronic excitations in conjugated polymers is key to advancing organic optoelectronic applications, such as solar cells, OLEDs and flexible electronics. While crystalline polymers can be studied…

Materials Science · Physics 2021-12-13 Francesco Campaioli , Jared H. Cole
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