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The wide-band limit is a commonly used approximation to analyze transport through nanoscale devices. In this work we investigate its applicability to the study of charge and heat transport through molecular break junctions exposed to…

Mesoscale and Nanoscale Physics · Physics 2018-05-15 F. Covito , F. G. Eich , R. Tuovinen , M. A. Sentef , A. Rubio

Molecular electronics break-junction experiments are widely used to investigate fundamental physics and chemistry at the nanoscale. Reproducibility in these experiments relies on measuring conductance on thousands of freshly formed…

Chemical Physics · Physics 2024-01-29 Leopoldo Mejía , Pilar Cossio , Ignacio Franco

The heat conduction behavior of one dimensional momentum conserving lattice systems with asymmetric interparticle interactions is numerically investigated. It is found that with certain degree of interaction asymmetry, the heat conductivity…

Statistical Mechanics · Physics 2015-05-28 Yi Zhong , Yong Zhang , Jiao Wang , Hong Zhao

Boltzmann transport theory, the standard framework for predicting thermal conductivity, assumes that every vibrational mode eventually scatters, acquiring a finite lifetime that yields a convergent, length-independent thermal conductivity:…

Mesoscale and Nanoscale Physics · Physics 2026-05-22 P. M. Martinez , O. Mateos-Lopez , J. C. Cuevas , J. G. Vilhena

Nanoscale solid-solid contacts define a wealth of material behaviours from the electrical and thermal conductivity in modern electronic devices to friction and losses in micro- and nanoelectromechanical systems. For modern ultra-high…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 B. J. Robinson , M. E. Pumarol , O. V. Kolosov

A method for the calculation of the conductance of nanoscale electrical junctions is extended to ab-initio electronic structure methods and applied to realistic models of metallic wires and break-junctions of sodium and gold. The method is…

Materials Science · Physics 2014-05-13 Matthieu J. Verstraete , P. Bokes , R. W. Godby

The thermal conductivity of nanoparticles colloidal suspensions, submitted to the action of an external force field has been calculated by non equilibrium molecular dynamics simulations. For driven forces in the radio frequency and…

Mesoscale and Nanoscale Physics · Physics 2008-01-25 Clément Le Goff , Philippe Ben-Abdallah , Gilberto Domingues , Ahmed Ould El Moctar

We demonstrate switching behavior and quantized conductance at room temperature in percolating films of nanoparticles. Our experiments and complementary simulations show that switching and quantization result from formation of atomic scale…

Mesoscale and Nanoscale Physics · Physics 2015-07-29 Abdul Sattar , Shawn Fostner , Simon A. Brown

We present a rigorous approach that leads, from a many-particle description, to a nonlinear, stochastic constitutive relation for the modeling of transient heat conduction processes at nanoscale. By enforcing statistical consistency, in…

Statistical Mechanics · Physics 2018-04-02 Weiqi Chu , Xiantao Li

Thermal conductivities are routinely calculated in molecular dynamics simulations by keeping the boundaries at different temperatures and measuring the slope of the temperature profile in the bulk of the material, explicitly using Fourier's…

Statistical Mechanics · Physics 2021-04-13 Yuanyang Ren , Kai Wu , David Cubero

Colloidal particles or nanoparticles, with equal affinity for two fluids, are known to adsorb irreversibly to the fluid-fluid interface. We present large-scale computer simulations of the demixing of a binary solvent containing such…

Soft Condensed Matter · Physics 2007-05-23 K. Stratford , R. Adhikari , I. Pagonabarraga , J. -C. Desplat , M. E. Cates

Atomic and single-molecule junctions represent the ultimate limit to the miniaturization of electrical circuits. They are also ideal platforms to test quantum transport theories that are required to describe charge and energy transfer in…

Mesoscale and Nanoscale Physics · Physics 2013-08-01 Woochul Lee , Kyeongtae Kim , Wonho Jeong , Linda Angela Zotti , Fabian Pauly , Juan Carlos Cuevas , Pramod Reddy

The thermal conductivity of nanometric objects or nanostructured materials can be determined using non equilibrium molecular dynamics (NEMD) simulations. The technique is simple in its principle, and resembles a numerical guarded hot plate…

Materials Science · Physics 2007-05-23 Patrice Chantrenne , Jean-Louis Barrat

Two aspects of conductive heat are focused here (i) the nature of conductive heat, defined as that form of energy that is transferred as a result of a temperature difference and (ii) the nature of the intermolecular potentials that induces…

General Physics · Physics 2016-08-08 Christopher Gunaseelan Jesudason

In the past few decades, great efforts have been devoted to studying heat transfer on the nanoscale due to its importance in multiple technologies such as thermal control and sensing applications. Heat conduction through the nanoconfined…

Computational Physics · Physics 2022-06-03 Reza Rabani , Samy Merabia , Ahmadreza Pishevar

We analytically study heat conduction in a chain with interparticle interaction V(x)=lambda[1-cos(x)] and harmonic on-site potential. We start with each site of the system connected to a Langevin heat bath, and investigate the case of small…

Statistical Mechanics · Physics 2007-05-23 Emmanuel Pereira , Ricardo Falcao

The simplicity of single-molecule junctions based on direct bonding of a small molecule between two metallic electrodes make them an ideal system for the study of fundamental questions related to molecular electronics. Here we study the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 O. Tal , M. Kiguchi , W. H. A. Thijssen , D. Djukic , C. Untiedt , R. H. M. Smit , J. M. van Ruitenbeek

We study heat conduction in a one-dimensional chain of particles with longitudinal as well as transverse motions. The particles are connected by two-dimensional harmonic springs together with bending angle interactions. Using equilibrium…

Statistical Mechanics · Physics 2009-11-10 Jian-Sheng Wang , Baowen Li

Understanding and controlling the flow of heat is a major challenge in nanoelectronics. When a junction is driven out of equilibrium by light or the flow of electric charge, the vibrational and electronic degrees of freedom are, in general,…

Mesoscale and Nanoscale Physics · Physics 2011-06-29 Daniel R. Ward , David A. Corley , James M. Tour , Douglas Natelson

Proper design and manufacturing thermal bridges based on molecular junctions at the contact between graphene platelets or other thermally conductive nanoparticles would provide a fascinating way to produce efficient heat transport networks…

Materials Science · Physics 2017-11-07 Alessandro Di Pierro , Guido Saracco , Alberto Fina