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We study heat conduction in (n, 0)/(2n, 0) intramolecular junctions by using molecular dynamics method. It is found that the heat conduction is asymmetric, namely, heat transports preferably in one direction. This phenomenon is also called…

Mesoscale and Nanoscale Physics · Physics 2007-08-18 Gang Wu , Baowen Li

The realization of single-molecule thermal conductance measurements has driven the need for theoretical tools to describe conduction processes that occur over atomistic length scales. In macroscale systems, the principle that is typically…

Mesoscale and Nanoscale Physics · Physics 2023-05-17 Galen T. Craven , Abraham Nitzan

Motivated by recent experiments [Lee et al. Nature 498, 209 (2013)], we present here a detailed theoretical analysis of the Joule heating in current-carrying single-molecule junctions. By combining the Landauer approach for quantum…

The energy dependent thermoelectric response of a single molecule contains valuable information about its transmission function and its excited states. However, measuring it requires devices that can efficiently heat up one side of the…

This mini review focuses on conductance measurements through molecular junctions containing few tens of molecules, which are fabricated along two approaches: (i) conducting atomic force microscope contacting a self-assembled monolayers on…

Applied Physics · Physics 2019-11-12 Dominique Vuillaume

We present an exact solution for the heat conductance along a harmonic chain connecting two reservoirs at different temperatures. In this model, the end points correspond to Brownian particles with different damping coefficients. Such…

Statistical Mechanics · Physics 2020-09-09 G. A. Weiderpass , Gustavo M. Monteiro , A. O. Caldeira

We compute the thermal conductance between two nanoparticles in contact based on the Molecular Dynamics technique. The contact is generated by letting both particles stick together under van der Waals attractions. The thermal conductance is…

Materials Science · Physics 2008-12-18 Gilberto Domingues , D. Rochais , Sebastian Volz

In the present Letter we present an analytical and numerical solution of the self-consistent mode-coupling equations for the problem of heat conductivity in one-dimensional systems. Such a solution leads us to propose a different scenario…

Statistical Mechanics · Physics 2009-11-11 L. Delfini , S. Lepri , R. Livi , A. Politi

We present the computer simulation results of a chain of hard point particles with alternating masses interacting on its extremes with two thermal baths at different temperatures. We found that the system obeys Fourier's law at the…

Statistical Mechanics · Physics 2009-11-07 Pedro L. Garrido , Pablo I. Hurtado , Bjoern Nadrowski

We present a theoretical analysis of heat transport through a single-molecule junction with two possible transport channels for electrons where interactions between electrons on the molecule and phonons in the nuclear environment is strong…

Mesoscale and Nanoscale Physics · Physics 2023-07-13 Natalya A. Zimbovskaya

We study heat transfer from a heated nanoparticle into surrounding fluid, using molecular dynamics simulations. We show that the fluid next to the nanoparticle can be heated well above its boiling point without a phase change. Under…

Materials Science · Physics 2009-12-17 Samy Merabia , Pawel Keblinski , Laurent Joly , Laurent Lewis , Jean-Louis Barrat

We derive rigorous quantum mechanical bounds for the heat current through a nanojunction connecting two thermal baths at different temperatures. Based on exact sum rules, these bounds compliment the well-known quantum of thermal conductance…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Edward Taylor , Dvira Segal

We report a numerical investigation on the heat transfer through one dimensional arrays of metallic nanoparticles closely spaced in a host material. Our simulations show that the multipolar interactions play a crucial role in the heat…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Philippe Ben-Abdallah , Karl Joulain , Jérémie Drevillon , Clément Le Goff

We have developed an efficient scalable kernel method for thermal transport in open systems, with which we have computed the thermal conductance of a junction between bulk silicon and silicon nanowires with diameter up to 10 nm. We have…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Ivan Duchemin , Davide Donadio

Electrically connected and plasmonically enhanced molecular junctions combine the optical functionalities of high field confinement and enhancement (cavity function), and of high radiative efficiency (antenna function) with the electrical…

Thermal convection in nanofluids is investigated by means of a continuum model for binary-fluid mixtures, with a thermal conductivity depending on the local concentration of colloidal particles. The applied temperature difference between…

Soft Condensed Matter · Physics 2015-05-20 Martin Glässl , Markus Hilt , Walter Zimmermann

We study full counting statistics for classical heat transport through anharmonic/nonlinear molecular junctions formed by interacting oscillators. Analytical result of the steady state heat flux for an overdamped anharmonic junction with…

Statistical Mechanics · Physics 2013-03-13 Sha Liu , Bjiay Kumar Agarwalla , Jian-Sheng Wang , Baowen Li

We present an original method to estimate the conductivity of a single molecule anchored to nanometric-sized metallic electrodes, using a Mechanically Controlled Break Junction (MCBJ) operated at room temperature in liquid. We record the…

Mesoscale and Nanoscale Physics · Physics 2018-03-16 M. Gil , T. Malinowski , M. Iazykov , H. Klein

Heating and heat conduction in molecular junctions are considered within a general NEGF formalism. We obtain a unified description of heating in current carrying molecular junctions as well as the electron and phonon contributions to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Mark A. Ratner , Abraham Nitzan

In this contribution, we study situations in which nanoparticles in a fluid are strongly heated, generating high heat fluxes. This situation is relevant to experiments in which a fluid is locally heated using selective absorption of…

Materials Science · Physics 2009-11-16 Samy Merabia , Serguei Shenogin , Laurent Joly , Pawel Keblinski , J. -L. Barrat