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We study the electronic structure of diluted F atoms chemisorbed on graphene using density functional theory calculations. We show that the nature of the chemical bonding of a F atom adsorbed on top of a C atom in graphene strongly depends…

Mesoscale and Nanoscale Physics · Physics 2015-03-18 J. O. Sofo , A. M. Suarez , Gonzalo Usaj , P. S. Cornaglia , A. D. Hernández-Nieves , C. A. Balseiro

The next-nearest neighbor interaction (NNN) is included in a tight-binding calculation of the electronic spectrum and conductivity of doped graphene. As a result, we observe a wide variation of the conductivity behavior, since the Fermi…

Materials Science · Physics 2015-10-12 J. E. Barrios-Vargas , Gerardo G Naumis

Polyyne, a sp1-hybridized linear allotrope of carbon, has a tunable quasiparticle energy gap, which depends on the terminated chemical ending groups as well as the chain length. Previously, nitrogen doping was utilized to tailor the…

Materials Science · Physics 2022-11-15 Kan Zhang , Jiling Li , Peitao Liu , Guowei Yang , Lei Shi

The significant electron-electron interactions that characterize the {\pi}-electrons of graphene nanoribbons (GNRs) necessitate going beyond one-electron tight-binding description. Existing theories of electron-electron interactions in GNRs…

Strongly Correlated Electrons · Physics 2016-07-27 V. M. L. Durga Prasad Goli , Suryoday Prodhan , Sumit Mazumdar , S. Ramasesha

Based on first-principles density-functional theory calculations, we present a comparative study of the elec- tronic structures of ultranarrow zigzag graphene nanoribbons (ZGNRs) embedded in hexagonal boron nitride (BN) sheet and fully…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 Sun-Woo Kim , Hyun-Jung Kim , Jin-Ho Choi , Ralph H. Scheicher , Jun-Hyung Cho

Undoped graphene is semi-metallic and thus not suitable for many electronic and optoelectronic applications requiring gapped semiconductor materials. However, a periodic array of holes (antidot lattice) renders graphene semiconducting with…

Mesoscale and Nanoscale Physics · Physics 2008-06-24 Thomas G. Pedersen , Christian Flindt , Jesper Pedersen , Antti-Pekka Jauho , Niels Asger Mortensen , Kjeld Pedersen

We present a theoretical study of the structural and electronic properties of graphene monolayer functionalized with boron and nitrogen atoms substituting carbon atoms. Our study is based on the ab initio calculations in the framework of…

Materials Science · Physics 2013-07-29 Magdalena Woinska , Karolina Z. Milowska , Jacek A. Majewski

Graphene-based sponges doped with atomic nitrogen and boron were applied for the electrochemical degradation of persistent organic contaminants in one-pass, flow-through mode, and in a low-conductivity supporting electrolyte. The B-doped…

Chemical Physics · Physics 2021-09-30 Luis Baptista-Pires , Giannis-Florjan Norra , Jelena Radjenovic

We have theoretically investigated the electronic and magnetic properties of graphene whose zigzag edges are oxidized. The alteration of these properties by adsorption of $\mathrm{H_{2}O}$ and $\mathrm{NH_3}$ molecules have been considered.…

Chemical Physics · Physics 2015-05-14 Julia Berashevich , Tapash Chakraborty

Chemically synthesized "cove"-type graphene nanoribbons (cGNRs) of different widths were brought into dispersion and drop-cast onto exfoliated hexagonal boron nitride (hBN) on a Si/SiO2 chip. With AFM we observed that the cGNRs form ordered…

We propose a class of graphene nanoribbons showing strong intrinsic ferromagnetic behavior due to their asymmetry. Such ribbons are based on a zig-zag edged backbone surmounted by a periodic, triangular notched region of variable size. The…

Having access to the chemical environment at the atomic level of a dopant in a nanostructure is crucial for the understanding of its properties. We have performed atomically-resolved electron energy-loss spectroscopy to detect individual…

In this study, we investigate the electronic and magnetic properties of graphane nanoribbons. We find that zigzag and armchair graphane nanoribbons with H-passivated edges are nonmagnetic semiconductors. While bare armchair ribbons are also…

Materials Science · Physics 2010-05-20 Hasan Sahin , Can Ataca , Salim Ciraci

The formation of graphen-nanotube composites addresses a few basic problems. First, both partners are good donors and acceptors of electrons, which significantly complicates the intermolecular interaction between them leading to a two-well…

Materials Science · Physics 2009-01-26 Elena F. Sheka , Leonid A. Chernozatonskii

In this communication, we report a theoretical attempt to understand the electronic and optical properties of germagraphene, a two-dimensional graphene analogue. We study two different structures, C$_{17}$Ge and C$_{16}$Ge. In the…

Computational Physics · Physics 2019-07-02 Sujoy Datta , Debnarayan Jana , Chhanda Basu Chaudhuri , Abhijit Mookerjee

Graphene nanostructures can be engineered with atomic precision to display customized electronic states with application in spintronics or quantum technologies. In order to take advantage of their full potential, their charge and spin state…

Armchair graphene nanoribbons with different proportions of edge oxygen atoms are investigated by using crystal orbital method based on density functional theory. All the nanoribbons are energetically favorable, although buckled edges are…

Materials Science · Physics 2014-11-07 Hongyu Ge , Guo Wang , Yi Liao

It was recently shown that nitrogen-doped graphene (NG) can exhibit both p- and n-type characters depending on the C-N bonding nature, which represents a significant bottleneck for the development of graphene-based electronics. Based on…

Mesoscale and Nanoscale Physics · Physics 2015-03-10 Hyo Seok Kim , Han Seul Kim , Seong Sik Kim , Yong-Hoon Kim

We present an ab initio study of the structural, electronic, and quantum transport properties of B-N-complex edge-doped graphene nanoribbons (GNRs). We find that the B-N edge codop-ing is energetically a very favorable process and…

Mesoscale and Nanoscale Physics · Physics 2015-03-10 Seong Sik Kim , Han Seul Kim , Hyo Seok Kim , Yong-Hoon Kim

Nitrogen doping of the carbon is an important method to improve the performance and durability of catalysts for proton exchange membrane fuel cells by platinum-nitrogen and carbon-nitrogen bonds. This study shows that p-phenyl groups and…