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Related papers: Dynamic transition in an atomic glass former: a mo…

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We present molecular dynamics results for a two component, two-dimensional Lennard-Jones supercooled liquid near the glass transition. We find that the supercooled liquid is spatially heterogeneous and that there are long-lived clusters…

Disordered Systems and Neural Networks · Physics 2009-10-31 Gregory Johnson , Andrew I. Melcuk , Harvey Gould , W. Klein , Raymond D. Mountain

We simulate the compression of a two-component Lennard-Jones liquid at a variety of constant temperatures using a molecular dynamics algorithm in an isobaric-isothermal ensemble. The viscosity of the liquid increases with pressure,…

chem-ph · Physics 2009-10-22 Shelly L. Shumway , Andrew S. Clarke , Hannes Jónsson

We show that the dynamics of kinetically constrained models of glass formers takes place at a first-order coexistence line between active and inactive dynamical phases. We prove this by computing the large-deviation functions of suitable…

Statistical Mechanics · Physics 2009-11-13 J. P. Garrahan , R. L. Jack , V. Lecomte , E. Pitard , K. van Duijvendijk , F. van Wijland

We use molecular dynamics simulation to study the relationship between structure and dynamics in supercooled binary Lennard--Jones nanoparticles over a range of particle sizes. The glass transition temperature of the nanoparticles is found…

Soft Condensed Matter · Physics 2025-05-15 Weikai Qi , Shreya Tiwary , Richard K. Bowles

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

Statistical Mechanics · Physics 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

The interplay of slow dynamics and thermodynamic features of dense liquids is studied by examinining how the glass transition changes depending on the presence or absence of Lennard-Jones-like attractions. Quite different thermodynamic…

Materials Science · Physics 2009-11-13 Th. Voigtmann

In two recent interesting letters evidence was presented for the existence of a growing dynamic correlation length when we approach the glass transition from the liquid phase (a similar divergence is present also in the off-equilibrium…

Statistical Mechanics · Physics 2007-05-23 S. Franz , G. Parisi

Whether the glass transition is caused by an underlying singularity or is a purely kinetic phenomenon is a significant outstanding question. Studying an atomistic glass former, we introduce a sampling method to access temperatures…

Statistical Mechanics · Physics 2017-09-20 Thomas Speck , C. Patrick Royall , Stephen R. Williams

In recent years, a second fluid-fluid phase transition has been reported in several materials at pressures far above the usual liquid-gas phase transition. In this paper, we introduce a new model of this behavior based on the Lennard-Jones…

Statistical Mechanics · Physics 2009-11-07 H. K. Lee , R. H. Swendsen

Dynamical properties of a Lennard-Jones binary mixture embedded in an off lattice matrix of soft spheres are studied in the direct space upon supercooling by molecular dynamics simulations. On lowering temperature the smaller particles tend…

Soft Condensed Matter · Physics 2009-11-10 P. Gallo , R. Pellarin , M. Rovere

Recently the supercooled Wahnstrom binary Lennard-Jones mixture was partially crystallized into ${\rm MgZn_2}$ phase crystals in lengthy Molecular Dynamics simulations. We present Molecular Dynamics simulations of a modified Kob-Andersen…

Soft Condensed Matter · Physics 2012-10-01 Søren Toxvaerd , Ulf R. Pedersen , Thomas B. Schrøder , Jeppe C. Dyre

A simple model to investigate the long time dynamics of glass-formers is presented and applied to study a Lennard-Jones system in supercooled and glassy phases. According to our model, the point representing the system in the…

Disordered Systems and Neural Networks · Physics 2009-10-31 Luca Angelani , Giorgio Parisi , Giancarlo Ruocco , Gabriele Viliani

We investigate experimentally the dynamic phase transition of a two-dimensional active nematic layer interfaced with a passive liquid crystal. Under a temperature ramp that leads to the transition of the passive liquid into a highly…

We investigate the calorimetric liquid-glass transition by performing simulations of a binary Lennard-Jones mixture in one through four dimensions. Starting at a high temperature, the systems are cooled to T=0 and heated back to the ergodic…

Disordered Systems and Neural Networks · Physics 2009-01-01 Ralf Brüning , Denis A. St-Onge , Steve Patterson , Walter Kob

It is established that liquid metals exhibit surface layering at the liquid-vapor interface, while dielectric simple systems, like those interacting through Lennard-Jones potentials, show a monotonic decay from the liquid density to that of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Luis E. Gonzalez , David J. Gonzalez

We study the relaxation dynamics of a binary Lennard-Jones liquid in the presence of an amorphous wall generated from equilibrium particle configurations. In qualitative agreement with the results presented in Nature Phys. {\bf 8}, 164…

Statistical Mechanics · Physics 2014-06-16 Glen M Hocky , Ludovic Berthier , Walter Kob , David R. Reichman

Molecular dynamics simulations are performed for a finite non-relativistic system of particles with Lennard-Jones potential. We study the effect of liquid-gas mixed phase on particle number fluctuations in coordinate subspace. A metastable…

High Energy Physics - Phenomenology · Physics 2023-05-30 Volodymyr A. Kuznietsov , Oleh Savchuk , Roman V. Poberezhnyuk , Volodymyr Vovchenko , Mark I. Gorenstein , Horst Stoecker

We investigate the dynamics of kinetically constrained models of glass formers by analysing the statistics of trajectories of the dynamics, or histories, using large deviation function methods. We show that, in general, these models exhibit…

Statistical Mechanics · Physics 2009-01-21 J. P. Garrahan , R. L. Jack , V. Lecomte , E. Pitard , K. van Duijvendijk , F. van Wijland

Among the key insights into the glass transition has been the identification of a non-equilibrium phase transition in trajectory space which reveals phase coexistence between the normal supercooled liquid (active phase) and a glassy state…

Soft Condensed Matter · Physics 2017-07-19 Rattachai Pinchaipat , Matteo Campo , Francesco Turci , James Hallett , Thomas Speck , C. Patrick Royall

We investigate by Molecular Dynamics simulation a system of $N$ particles moving on the surface of a two-dimensional sphere and interacting by a Lennard-Jones potential. We detail the way to account for the changes brought by a nonzero…

Statistical Mechanics · Physics 2015-06-18 Julien-Piera Vest , Gilles Tarjus , Pascal Viot
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