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We investigate the effect of photodesorption on the snow line position at the surface of a protoplanetary disk around a Herbig Ae/Be star, motivated by the detection of water ice particles at the surface of the disk around HD142527 by Honda…

Earth and Planetary Astrophysics · Physics 2012-02-27 Akinori Oka , Akio K. Inoue , Taishi Nakamoto , Mitsuhito Honda

The desorption dynamics of rubidium dimers (Rb_2) off the surface of helium nanodroplets induced by laser excitation is studied employing both nanosecond and femtosecond ion imaging spectroscopy. Similarly to alkali metal atoms, we find…

Atomic and Molecular Clusters · Physics 2017-02-08 A. Sieg , J. von Vangerow , F. Stienkemeier , O. Dulieu , M. Mudrich

In this study, we investigated the physisorption mechanisms of O2, H2O, CH4, and CO2 molecules on alumina and their effect on electronic properties. We employed quantum-classical molecular dynamics simulations and the self-consistent-charge…

In this work, we determine the dissociation temperature of the hydrogen (H$_2$) hydrate by computer simulation using two different methods. In both cases, the molecules of water and H$_2$ are modeled using the TIP4P/Ice and a modified…

Soft Condensed Matter · Physics 2026-01-27 Miguel J. Torrejon , S. Blazquez , Jesus Algaba , M. M. Conde , F. J. Blas

We propose a new simple computational model to estimate adsorption energies of atoms and molecules to low-temperature amorphous water ice, and we present the adsorption energies of carbon (3P), nitrogen (4S), and oxygen (3P) atoms based on…

Astrophysics of Galaxies · Physics 2018-03-14 Takashi Shimonishi , Naoki Nakatani , Kenji Furuya , Tetsuya Hama

To explain grain growth and destruction in warm media, ice mantle formation and sublimation in cold media, and gas line emission spectroscopy, astrochemical models must mimic the gas--solid abundance ratio. Ice-sublimation mechanisms…

Astrophysics of Galaxies · Physics 2024-04-04 F. Kruczkiewicz , F. Dulieu , A. V. Ivlev , P. Caselli , B. M. Giuliano , C. Ceccarelli , P. Theulé

Context. Sulfur is used as a tracer of the evolution from interstellar clouds to stellar systems. However, most of the expected sulfur in molecular clouds remains undetected. Sulfur disappears from the gas phase in two steps. One first…

Astrophysics of Galaxies · Physics 2022-01-19 S. Cazaux , H. Carrascosa , G. M. Munoz Caro , P. Caselli , A. Fuente , D. Navarro-Almaida , P. Riviére-Marichalar

Water ice covers the surface of various objects in the outer Solar system. Within the heliopause, surface ice is constantly bombarded and sputtered by energetic particles from the solar wind and magnetospheres. We report a laboratory…

Fragments from organic molecule dissociation (such as reactive ions and radicals) can form interstellar complex molecules like amino acids. The goal of this work is to experimentally study photoionization and photodissociation processes of…

Astrophysics · Physics 2007-05-23 S. Pilling , A. C. F. Santos , H. M. Boechat-Roberty

Molecular hydrogen is the most abundant molecular species in the Universe. While no doubts exist that it is mainly formed on the interstellar dust grain surfaces, many details of this process remain poorly known. In this work, we focus on…

In the previous works the significance of the symmetric and non-symmetric ion-atom absorption processes in far UV and EUV regions within a model of the quiet Sun atmosphere, has been studied. The considered processes were the processes of…

Solar and Stellar Astrophysics · Physics 2013-12-03 V. A. Sreckovic , A. A. Mihajlov , Lj. M. Ignjatovic , M. S. Dimitrijevic

Radiative cooling by molecules is a crucial process for hydrodynamic escape, as it can efficiently remove the thermal energy driving the outflow, acquired through X-ray and extreme UV absorption. Carbon oxides, such as CO and CO2, and their…

Earth and Planetary Astrophysics · Physics 2024-11-26 Tatsuya Yoshida , Naoki Terada , Kiyoshi Kuramoto

Water absorption and dissociation processes on pristine low-index TiO$_2$ interfaces are important but poorly understood outside the well-studied anatase (101) and rutile (110). To understand these, we construct three sets of machine…

Materials Science · Physics 2023-03-15 Zezhu Zeng , Felix Wodaczek , Keyang Liu , Frederick Stein , Jürg Hutter , Ji Chen , Bingqing Cheng

The interaction of hydrogen with many transition metal surfaces is characterized by a coexistence of activated with non-activated paths to adsorption with a broad distribution of barrier heights. By performing six-dimensional quantum…

mtrl-th · Physics 2016-09-07 Axel Gross , Matthias Scheffler

Two dimensional transition metal dichalcogenides appear as good candidates for gas sensing and catalysis. Here, by means of density functional theory, we characterize the adsorption and dissociation of selected diatomic molecules (CO,…

Materials Science · Physics 2022-01-06 Raúl Bombín , Maite Alducin , Iñaki Juaristi

Ultraslow radiative cooling lifetimes and adiabatic detachment energies for three astrochemically relevant anions, C$_n^-$ ($n=3-5$), are measured using the Double ElectroStatic Ion Ring ExpEriment (DESIREE) infrastructure at Stockholm…

The photo-induced desorption and oxidation of CO on Ru(0001) is simulated using ab initio molecular dynamics with electronic friction that accounts for the non-equilibrated excited electrons and phonons. Different (O,CO) coverages are…

Materials Science · Physics 2023-07-06 Auguste Tetenoire , J. Iñaki Juaristi , Maite Alducin

Two-pulse correlation experiments performed using pulses of different intensities on Pd(111) with different CO coverages showed that the CO photodesorption probability depends on whether the strong or the weak pulse arrives first to the…

We determine the impact of electron solvation on D$_2$O structures adsorbed on Cu(111) with low temperature scanning tunneling microscopy, two-photon photoemission, and ab initio theory. UV photons generating solvated electrons lead not…

The urgent need to mitigate rising atmospheric CO2 levels motivates the search for stable, efficient, and tunable adsorbent materials. In this study, we employ first-principles density functional theory to investigate the adsorption of CO2…

Materials Science · Physics 2026-02-16 Jakkapat Seeyangnok , Rungkiat Nganglumpoon , Joongjai Panpranot , Udomsilp Pinsook