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We have synthesized epitaxial Sr2IrO4 thin-films on various substrates and studied their electronic structures as a function of lattice-strains. Under tensile (compressive) strains, increased (decreased) Ir-O-Ir bond-angles are expected to…

Strongly Correlated Electrons · Physics 2013-09-09 J. Nichols , J. Terzic , E. G. Bittle , O. B. Korneta , L. E. De Long , J. W. Brill , G. Cao , S. S. A. Seo

Cu$_2$IrO$_3$ has attracted recent interest due to its proximity to the Kitaev quantum spin liquid state and the complex structural response observed at high pressures. We use x-ray spectroscopy and scattering as well as electrical…

We present a combined oxygen $K$-edge x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) study of the bilayer ruthenate Ca$_3$Ru$_2$O$_7$. Our RIXS experiments on Ca$_3$Ru$_2$O$_7$ were carried out on the…

Strongly Correlated Electrons · Physics 2025-04-01 K. von Arx , F. Forte , M. Horio , V. Granata , Q. Wang , L. Das , Y. Sassa , R. Fittipaldi , C. G. Fatuzzo , O. Ivashko , Y. Tseng , E. Paris , A. Vecchione , T. Schmitt , M. Cuoco , J. Chang

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

Strongly Correlated Electrons · Physics 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux

Spin excitations in the overdoped high temperature superconductors Tl$_2$Ba$_2$CuO$_{6+\delta}$ and (Bi,Pb)$_2$(Sr,La)$_{2}$CuO$_{6+\delta}$ were investigated by resonant inelastic x-ray scattering (RIXS) as functions of doping and detuning…

The electronic structure of the heavy fermion compound CeB6 is probed by resonant inelastic soft X-ray scattering using photon energies across the Ce 3d and 4d absorption edges. The hybridization between the localized 4f orbitals and the…

Materials Science · Physics 2012-01-04 M. Magnuson , S. M. Butorin , J. -H. Guo , A. Agui , J. Nordgren , H. Ogasawara , A. Kotani , T. Takahashi , S. Kunii

We report new measurements and calculations of the non-resonant inelastic x-ray scattering (NRIXS) from Mg and Al for a wide range of momentum transfers, q. Extended oscillations in the dynamic structure factor S(q,w) due to scattering from…

Materials Science · Physics 2015-06-25 T. T. Fister , G. T. Seidler , C. Hamner , J. O. Cross , J. A. Soininen , J. J. Rehr

The electronic-structural modulations of Ir$_{1-x}$Pt$_x$Te$_2$ (0 $\leqq x\leqq$ 0.12) have been examined by resonant elastic x-ray scattering (REXS) and resonant inelastic x-ray scattering (RIXS) techniques at both the Ir and Te edges.…

Strongly Correlated Electrons · Physics 2018-07-04 K. Takubo , K. Yamamoto , Y. Hirata , H. Wadati , T. Mizokawa , R. Sutarto , F. He , K. Ishii , Y. Yamasaki , H. Nakao , Y. Murakami , G. Matsuo , H. Ishii , M. Kobayashi , K. Kudo , M. Nohara

We report the path from the charge density wave (CDW)-bearing superconductor CuIr2Te4 to the metal insulator transition (MIT)-bearing compound CuIr2S4 by chemical alloying with the gradual substitution of S for Te. The evolution of…

We investigated the temperature-dependent evolution of the electronic structure of the Jeff,1/2 Mott insulator Sr2IrO4 using optical spectroscopy. The optical conductivity spectra $\sigma(\omega)$ of this compound has recently been found to…

Strongly Correlated Electrons · Physics 2009-10-23 S. J. Moon , Hosub Jin , W. S. Choi , J. S. Lee , S. S. A. Seo , J. Yu , G. Cao , T. W. Noh , Y. S. Lee

We present a computation of Cu K-edge resonant inelastic x-ray scattering (RIXS) spectra for electron-doped cuprates which includes coupling to bosonic fluctuations. Comparison with experiment over a wide range of energy and momentum…

Strongly Correlated Electrons · Physics 2012-02-09 Susmita Basak , Tanmoy Das , Hsin Lin , M. Z. Hasan , R. S. Markiewicz , A. Bansil

We investigate mixed-valence oxide Co$_3$O$_4$ using Co $2p3d$ resonant inelastic X-ray scattering (RIXS). By setting resonant edges at Co$^{2+}$ and Co$^{3+}$ ions, the $dd$ excitations on the two Co sites are probed selectively, providing…

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

Strongly Correlated Electrons · Physics 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

Understanding quantum materials -- solids in which quantum-mechanical interactions among constituent electrons yield a great variety of novel emergent phenomena -- is a forefront challenge in modern condensed matter physics. This goal has…

Strongly Correlated Electrons · Physics 2026-03-13 M. Mitrano , S. Johnston , Young-June Kim , M. P. M. Dean

We investigate the excitation spectra of a spin-1/2 antiferromagnetic Heisenberg trimer spin chain by employing a combination of numerical and theoretical techniques. Utilizing the Krylov-space correction-vector method in density matrix…

Strongly Correlated Electrons · Physics 2025-01-17 Junli Li , Jun-Qing Cheng , Trinanjan Datta , Dao-Xin Yao

We report pressure-induced superconductivity in the spinel CuIr$_{2}$S$_{4}$ with a transition temperature ($T_{\text{c}}$) reaching \textbf{18.2 K}, establishing a new record for this class of materials and surpassing the decades-old limit…

The electronic structures of the Heusler type compounds Fe$_{3-x}V$_x$Si in the concentration range between x = 0 and x = 1 have been probed by photoemission spectroscopy (PES). The observed shift of Si 2p core- level and the main valence…

CuInP2S6 (CIPS) is an emerging layered material that exhibits ferrielectric ordering well above room temperature (Curie temperature TC ~ 315 K). When synthesized with Cu deficiencies, CIPS spontaneously segregates into CuInP2S6 and…

Materials Science · Physics 2021-11-02 Rahul Rao , Ryan Selhorst , Benjamin S. Conner , Michael A. Susner

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane.…

Systematic experimental data on resonant inelastic X-ray scattering (RIXS) in GaN near the N K-edge are presented for the first time. Excitation energy dependence of the spectral structures manifests the band structure effects originating…

Materials Science · Physics 2009-11-10 V. N. Strocov , T. Schmitt , J. -E. Rubensson , P. Blaha , T. Paskova , P. O. Nilsson