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Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

High harmonic spectroscopy has the potential to combine attosecond temporal with sub-Angstrom spatial resolution of the early nuclear and multielectron dynamics in molecules. It involves strong field ionization of the molecule by the IR…

Atomic Physics · Physics 2013-08-08 Valeria Serbinenko , Olga Smirnova

The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as…

Optics · Physics 2013-12-06 Michael Chini , Kun Zhao , Zenghu Chang

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

A new method for efficiently generating an isolated single-cycle attosecond pulse is proposed. It is shown that the ultraviolet (UV) attosecond pulse can be utilized as a robust tool to control the dynamics of electron wave packets (EWPs).…

Atomic Physics · Physics 2009-11-13 Pengfei Lan , Peixiang Lu , Wei Cao , Xinlin Wang

In many areas of imaging science, it is difficult to measure the phase of linear measurements. As such, one often wishes to reconstruct a signal from intensity measurements, that is, perform phase retrieval. In several applications the…

Information Theory · Computer Science 2015-06-16 Afonso S. Bandeira , Dustin G. Mixon

The present work focuses on the characterisation of the amount of orbital angular momentum (OAM) encoded in the twisted attosecond pulses via energy- and angle-resolved attosecond streaking in pump-probe setup. It is found that the…

Atomic Physics · Physics 2020-06-03 Irfana N. Ansari , Deependra S. Jadoun , Gopal Dixit

Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…

Optics · Physics 2019-05-15 Martin Kozák , Norbert Schönenberger , Peter Hommelhoff

The demanding experimental access to the ultrafast dynamics of materials challenges our understanding of their electronic response to applied strong laser fields. For this purpose, trapped ultracold atoms with highly controllable potentials…

Fascinating developments in optical pulse engineering over the last 20 years lead to the generation of laser pulses as short as few femtosecond, providing a unique tool for high resolution time domain spectroscopy. However, a number of the…

General Physics · Physics 2008-06-03 M Kozlowski , J Marciak-Kozlowska , M Pelc

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Phase retrieval is in general a non-convex and non-linear task and the corresponding algorithms struggle with the issue of local minima. We consider the case where the measurement samples within typically very small and disconnected subsets…

Signal Processing · Electrical Eng. & Systems 2022-06-28 Jonas Kornprobst , Alexander Paulus , Josef Knapp , Thomas F. Eibert

Various schemes are presented for the generation of circularly polarized molecular high-order harmonic generation (MHOHG) from molecules. In particular it is shown that combinations of counter-rotating circularly polarized pulses produce…

Optics · Physics 2015-12-15 Andre D. Bandrauk , Kai-Jun Yuan

Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…

Chemical Physics · Physics 2022-11-07 Lorenzo Restaino , Deependra Jadoun , Markus Kowalewski

The attosecond streaking technique is normally utilized to characterize the attosecond pulses in extreme ultraviolet spectrum, while the pulse simulation and reconstruction schemes turn out to be unreliable for extremely short sub-100as…

Optics · Physics 2018-09-05 Renzhi Shao , Bin Li

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

In this paper we consider the nonlinear inverse problem of phase retrieval in the context of dynamical sampling. Where phase retrieval deals with the recovery of signals & images from phaseless measurements, dynamical sampling was…

Numerical Analysis · Mathematics 2021-02-02 Robert Beinert , Marzieh Hasannasab

Characterizing an isolated attosecond pulse (IAP) is essential for its potential applications. A complete characterization of an IAP ultimately requires the determination of its electric field in both time and space domains. However,…

Optics · Physics 2022-10-05 Lixin He , Jianchang Hu , Siqi Sun , Yanqing He , Yu Deng , Pengfei Lan , Peixiang Lu

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan