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The manipulation of the motion of neutral molecules with electric or magnetic fields has seen tremendous progress over the last decade. Recently, these techniques have been extended to the manipulation of large and complex molecules. In…

Chemical Physics · Physics 2011-04-07 Frank Filsinger , Gerard Meijer , Henrik Stapelfeldt , Henry N. Chapman , Jochen Küpper

We report radiation pressure slowing of YbF molecules to low velocity. In YbF, laser slowing is hindered by leaks out of the optical cycle attributed to low-lying metastable electronic states arising from inner-shell excitation. We bring…

We produce SO_2 molecules with a centre of mass velocity near zero using a Stark decelerator. Since the initial kinetic energy of the supersonic SO_2 molecular beam is high, and the removed kinetic energy per stage is small, 326…

Atomic Physics · Physics 2009-11-13 O. Bucicov , M. Nowak , S. Jung , G. Meijer , E. Tiemann , Ch. Lisdat

We demonstrate the long-term ($<$ 1 minute) trapping of Stark-decelerated OH radicals in their $X~^{2}\Pi _{3/2}~(\nu = 0,~J = 3/2,~M_{J} = 3/2,~f)$ state in a permanent magnetic trap. The trap environment was cryogenically cooled to a…

Chemical Physics · Physics 2019-08-05 Dominik Haas , Claudio von Planta , Thomas Kierspel , Dongdong Zhang , Stefan Willitsch

We have designed and implemented a new Stark decelerator based on wire electrodes, which is suitable for ultrahigh vacuum applications. The 100 deceleration stages are fashioned out of 0.6 mm diameter tantalum and the array's total length…

Atomic Physics · Physics 2010-09-28 Adela Marian , Henrik Haak , Peter Geng , Gerard Meijer

We present a novel slowing scheme for beams of laser-coolable diatomic molecules reminiscent of Zeeman slowing of atomic beams. The scheme results in efficient compression of the 1-dimensional velocity distribution to velocities trappable…

Atomic Physics · Physics 2018-05-09 Maurice Petzold , Paul Kaebert , Philipp Gersema , Mirco Siercke , Silke Ospelkaus

A special class of molecules that are important to many subfields in molecular dynamics and chemical physics, namely free radical molecules, now enjoy a significant degree of center-of-mass motion control in the laboratory frame. The…

Atomic Physics · Physics 2009-11-10 J. R. Bochinski , Eric R. Hudson , H. J. Lewandowski , Jun Ye

We theoretically analyze the cooling dynamics of an atom which is tightly trapped inside a high-finesse optical resonator. Cooling is achieved by suitably tailored scattering processes, in which the atomic dipole transition either scatters…

Quantum Physics · Physics 2012-11-08 Marc Bienert , Giovanna Morigi

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

We present the design, construction, and characterisation of longitudinal- and transverse-field Zeeman slowers, based on arrays of permanent magnets, for slowing thermal beams of atomic Sr. The slowers are optimised for operation with…

Atomic Physics · Physics 2015-06-18 Ian R. Hill , Yuri B. Ovchinnikov , Elizabeth M. Bridge , E. Anne Curtis , Patrick Gill

The Stark deceleration of OH radicals in both low-field-seeking and high-field-seeking levels of the rovibronic ${}^2\Pi_{3/2},v=0,J=3/2$ ground state is demonstrated using a single experimental setup. Applying alternating-gradient…

Chemical Physics · Physics 2008-09-18 Kirstin Wohlfart , Frank Filsinger , Fabian Grätz , Jochen Küpper , Gerard Meijer

The possibility of a significant slowdown of particles by removing them from a localized state in an electromagnetic potential well with a fixed spatial distribution is shown with a sufficiently slow decrease in the depth of this well with…

General Physics · Physics 2022-09-22 Azad Izmailov

In this paper we describe the high-voltage generation system we have developed for a traveling-wave Stark decelerator (TWSD). The TWSD can reduce the forward velocity of a molecular beam of heavy neutral polar molecules such as strontium…

Atomic Physics · Physics 2026-02-12 Lucas van Sloten , Leo Huisman , Steven Hoekstra

We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…

Magneto-optical trapping forces for molecules are far weaker than for alkali atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further…

Atomic Physics · Physics 2021-12-14 M. R. Tarbutt , T. C. Steimle

High-precision hydrogen spectroscopy is an active field which helps to determine the Rydberg constant and proton charge radius, tests bound-state QED, and can search for Beyond Standard Model (BSM) Physics. Additionally, with recent…

Atomic Physics · Physics 2022-06-15 S. F. Cooper , C. Rasor , R. G. Bullis , A. D. Brandt , D. C. Yost

Cold, velocity-controlled molecular beams consisting of a single quantum state promise to be a powerful tool for exploring molecular scattering interactions. In recent years, Stark deceleration has emerged as one of the main methods for…

A pulsed beam of ground state OH radicals is slowed down using a Stark decelerator and is subsequently loaded into an electrostatic trap. Characterization of the molecular beam production, deceleration and trap loading process is performed…

Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the…

Atomic Physics · Physics 2015-06-18 A. M. Jayich , A. C. Vutha , M. T. Hummon , J. V. Porto , W. C. Campbell

We outline a method to slow paramagnetic atoms or molecules using pulsed magnetic fields. We also discuss the possibility of producing trapped particles by adiabatic deceleration of a magnetic trap. We present numerical simulation results…

Atomic and Molecular Clusters · Physics 2009-11-13 E. Narevicius , C. G. Parthey , A. Libson , M. F. Riedel , U. Even , M. G. Raizen