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The magnetic and surface properties of some transition metals have been investigated within the tight-binding approximation, including Coulomb correlations. These surface properties are calculated after applying a charge neutrality rule…

Materials Science · Physics 2025-08-05 Jacques R. Eone

We present optimized tight-binding models with atomic orbitals to improve \textit{ab initio} tight-binding models constructed by truncating full density functional theory (DFT) Hamiltonian based on localized orbitals. Retaining qualitative…

Mesoscale and Nanoscale Physics · Physics 2024-02-20 Sejoong Kim

We extend a tight-binding total energy method to include f-electrons, and apply it to the study of the structural and elastic properties of a range of elements from Be to U. We find that the tight-binding parameters are as accurate and…

Materials Science · Physics 2009-11-07 Matthew D. Jones , R. C. Albers

Finite-temperature calculations are relevant for rationalizing material properties yet they are computationally expensive because large system sizes or long simulation times are typically required. Circumventing the need for performing many…

We investigate the electronic structure of the ternary iron selenide K$_{y}$% Fe$_{1.6}$Se$_{2}$ by considering the spatial symmetry of the $\sqrt{5}% \times \sqrt{5}$ vacancy ordered structure. Based on three orbitals of $% t_{2g}$, which…

Strongly Correlated Electrons · Physics 2011-11-28 Shin-Ming Huang , Chung-Yu Mou

The development of sensible microscopic models is essential to elucidate the normal-state and superconducting properties of the iron-based superconductors. Because these materials are mostly metallic, a good starting point is an effective…

Strongly Correlated Electrons · Physics 2017-01-05 Rafael M. Fernandes , Andrey V. Chubukov

We extend a tight-binding method to include the effects of spin-orbit coupling, and apply it to the study of the electronic properties of the actinide elements Th, U, and Pu. These tight-binding parameters are determined for the fcc crystal…

Materials Science · Physics 2013-05-29 M. D. Jones , R. C. Albers

The ideas of the linear combination of atomic orbitals (LCAO) method, well known from the study of electrons, is extended to the classical wave case. The Mie resonances of the isolated scatterer in the classical wave case, are analogous to…

Disordered Systems and Neural Networks · Physics 2009-10-31 E. Lidorikis , M. M. Sigalas , C. M. Soukoulis , E. N. Economou

We discuss how to construct a tight binding model Hamiltonan for the simplest possible solid, composed of hydrogen-like atoms. A single orbital per atom is not sufficient because the on-site electron-electron repulsion mixes in higher…

Strongly Correlated Electrons · Physics 2014-09-09 J. E. Hirsch

Motivated by the newly-discovered intercalated iron chalcogenide superconductors, we construct a single orbital tight-binding model for topological insulators on the square lattice with a perfect vacancy superstructure. We find that such…

Strongly Correlated Electrons · Physics 2015-03-19 Xiao-Yong Feng , Hua Chen , Chao Cao , Jianhui Dai

Harrison's tight-binding theory provides an excellent qualitative description of the electronic structure of the elements across the periodic table. However, the resulting band structures are in significant disagreement with those found by…

Materials Science · Physics 2009-11-10 L. Shi , D. A. Papaconstantopoulos

We provide a comprehensive analysis of the prominent tight-binding (TB) models for transition metal dichalcogenides (TMDs) available in the literature. We inspect the construction of these TB models, discuss their parameterization used and…

Materials Science · Physics 2024-06-25 Bert Jorissen , Lucian Covaci , Bart Partoens

We use the Gutzwiller Density Functional Theory to calculate ground-state properties and bandstructures of iron in its body-centered-cubic (bcc) and hexagonal-close-packed (hcp) phases. For a Hubbard interaction $U=9\, {\rm eV}$ and…

Strongly Correlated Electrons · Physics 2016-06-02 Tobias Schickling , Jörg Bünemann , Florian Gebhard , Lilia Boeri

An interacting lattice model describing the subspace spanned by a set of strongly-correlated bands is rigorously coupled to density functional theory to enable ab initio calculations of geometric and topological material properties. The…

Strongly Correlated Electrons · Physics 2019-03-26 Ryan Requist , E. K. U. Gross

Many of the important phases observed in twisted transition metal dichalcogenide homobilayers are driven by short-range interactions, which should be captured by a local tight binding description since no Wannier obstruction exists for…

Strongly Correlated Electrons · Physics 2024-10-02 Valentin Crépel , Andrew Millis

We demonstrate that variations in molecular chemisorption energy on different metals, different surface terminations, and different strain conditions can be accounted for by orbital-specific changes in the substrate electronic structure.…

Materials Science · Physics 2007-05-23 Sara E. Mason , Ilya Grinberg , Andrew M. Rappe

We describe an empirical, self-consistent, orthogonal tight-binding model for zirconia, which allows for the polarizability of the anions at dipole and quadrupole levels and for crystal field splitting of the cation d orbitals. This is…

Materials Science · Physics 2009-10-31 Stefano Fabris , Anthony T. Paxton , Michael W. Finnis

In this work we present a tight-binding model that allows to describe with a minimal amount of parameters the band structure of exciton-polariton lattices. This model based on $s$ and $p$ non-orthogonal photonic orbitals faithfully…

We present calculations of the free energy, and hence the melting properties, of a simple tight-binding model for transition metals in the region of d-band filling near the middle of a d-series, the parameters of the model being designed to…

Materials Science · Physics 2015-05-13 C. Cazorla , D. Alfè , M. J. Gillan

The tight binding model is a minimalistic electronic structure model for predicting properties of materials and molecules. For insulators at zero Fermi-temperature we show that the potential energy surface of this model can be decomposed…

Mathematical Physics · Physics 2020-04-21 Christoph Ortner , Jack Thomas , Huajie Chen