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An application of the tight binding approximation is presented for the description of electronic structure and interatomic force in magnetic iron, both pure and containing hydrogen impurities. We assess the simple canonical d-band…

Materials Science · Physics 2015-05-19 A. T. Paxton , C. Elsaesser

A recent tight-binding scheme provides a method for extending the results of first principles calculations to regimes involving $10^2 - 10^3$ atoms in a unit cell. The method uses an analytic set of two-center, non-orthogonal tight-binding…

mtrl-th · Physics 2008-02-03 Michael J. Mehl , Dimitrios A. Papaconstantopoulos

The electronic structure, when restricted to the d-band approximation, is a computational model that is both efficient and useful for describing transition metals. In the absence of considering delocalized sp-states, this approximation…

Materials Science · Physics 2025-08-05 Jacques R. Eone

The rich novel materials class of iron based superconductors turned out to exhibit a very complex electronic structure, despite of the simplicity of their crystal structures. For various approaches to study the instability against magnetic…

Superconductivity · Physics 2013-05-29 H. Eschrig , K. Koepernik

We describe a self consistent magnetic tight-binding theory based in an expansion of the Hohenberg-Kohn density functional to second order, about a non spin polarised reference density. We show how a first order expansion about a density…

Materials Science · Physics 2009-11-13 A. T. Paxton , M. W. Finnis

Semiconducting transition metal dichalcogenides present a complex electronic band structure with a rich orbital contribution to their valence and conduction bands. The possibility to consider the electronic states from a tight-binding model…

Materials Science · Physics 2016-11-15 J. A. Silva-Guillén , P. San-Jose , R. Roldán

We present a tight-binding potential for transition metals, carbon, and transition metal carbides, which has been optimized through a systematic fitting procedure. A minimal basis, including the s, p electrons of carbon and the d electrons…

Tight-binding models provide great insight and are a low-cost alternative to \emph{ab initio} methods for calculation of a material's electronic structure. These models are used to calculate optical responses, including nonlinear optical…

Materials Science · Physics 2025-09-29 Andreas Ghosh , Aaron M. Schankler , Andrew M. Rappe

We propose a five-band tight-binding model for the Fe-As layers of iron pnictides with the hopping amplitudes calculated within the Slater-Koster framework. The band structure found in DFT, including the orbital content of the bands, is…

Superconductivity · Physics 2009-10-08 M. J. Calderon , B. Valenzuela , E. Bascones

It is shown that, an entire class of off-diagonally disordered linear lattices composed of two basic building blocks and described within a tight binding model can be tailored to generate absolutely continuous energy bands. It can be…

Disordered Systems and Neural Networks · Physics 2016-09-09 Atanu Nandy , Biplab Pal , Arunava Chakrabarti

For a previously published study of the titanium hcp (alpha) to omega (omega) transformation, a tight-binding model was developed for titanium that accurately reproduces the structural energies and electron eigenvalues from all-electron…

Materials Science · Physics 2008-07-24 D. R. Trinkle , M. D. Jones , R. G. Hennig , S. P. Rudin , R. C. Albers , J. W. Wilkins

We study the dependence of the electronic structure of iron pnictides on the angle formed by the arsenic-iron bonds. Within a Slater-Koster tight binding model which captures the correct symmetry properties of the bands, we show that the…

Strongly Correlated Electrons · Physics 2009-02-09 M. J. Calderon , B. Valenzuela , E. Bascones

Parameterized tight-binding models fit to first principles calculations can provide an efficient and accurate quantum mechanical method for predicting properties of molecules and solids. However, well-tested parameter sets are generally…

Materials Science · Physics 2023-04-28 Kevin F. Garrity , Kamal Choudhary

We employ a tight-binding parametrization based on the Slater Koster model in order to fit the band structures of single-layer, bilayer and bulk black phosphorus obtained from first-principles calculations. We find that our model, which…

Mesoscale and Nanoscale Physics · Physics 2017-12-13 Marcos G. Menezes , Rodrigo B. Capaz

We obtain parameters for non-orthogonal and orthogonal TB models from two-atomic molecules for all combinations of elements of period 1 to 6 and group 3 to 18 of the periodic table. The TB bond parameters for 1711 homoatomic and…

Materials Science · Physics 2021-02-17 Jan Jenke , Alvin N. Ladines , Thomas Hammerschmidt , David G. Pettifor , Ralf Drautz

The linear combination of atomic orbitals (LCAO) is a standard method for studying solids and molecules, it is also known as the tight$-$binding (TB) method. In most of the implementations only the basis set and the coupling constants are…

Materials Science · Physics 2024-01-18 Graziâni Candiotto

We propose an accurate tight-binding parametrization for the band structure of MoS$_2$ monolayers near the main energy gap. We introduce a generic and straightforward derivation for the band energies equations that could be employed for…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 E. Ridolfi , D. Le , T. S. Rahman , E. R. Mucciolo , C. H. Lewenkopf

Recent density functional theory (DFT) calculations by Foerst et al. have predicted that vacancies in both low and high carbon steels have a carbon dimer bound to them. This is likely to change the thinking of metallurgists in the kinetics…

Materials Science · Physics 2015-06-15 A. T. Paxton , C. Elsaesser

We propose to adapt the confined pseudo-atomic orbitals underpinning the precalculated Slater-Koster (SK) interaction tables in Density Functional Tight Binding (DFTB) to local atomic environments. We demonstrate significant improvement in…

Correlations derived through single-particle approximations of the many-body problem frequently result in erroneously inflated or diminished physical properties. In the context of transition metals, the impact of correlations can be…

Materials Science · Physics 2025-08-05 Jacques R. Eone
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