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Angle-resolved photoelectron spectroscopy of the unpaired electron in sodium-doped water, methanol, ammonia, and dimethyl ether clusters is presented. The experimental observations and the complementary calculations are consistent with…

Atomic and Molecular Clusters · Physics 2016-03-14 Adam H. C. West , Bruce L. Yoder , David Luckhaus , Clara-Magdalena Saak , Maximilian Doppelbauer , Ruth Signorell

Speed plot and time delay analysis confirms a two-pole S-matrix structure of the lowest 3/2+ level in 5He. Real parts of neutron-alpha elastic and 4He(n,d)3H reaction pole energies are 17.669+/-0.006 and 17.705+/-0.001 MeV n-4He c.m.,…

Nuclear Theory · Physics 2012-10-03 Bernard Hoop , Gerald M. Hale , Petr Navratil

Laser-assisted electron scattering (LAES), a light-matter interaction process that facilitates energy transfer between strong light fields and free electrons, has so far been observed only in gas phase. Here we report on the observation of…

Recoilless resonant capture of monoenergetic electron antineutrinos (Moessbauer antineutrinos) emitted in bound-state beta-decay in the system 3H - 3He is discussed. The recoilfree fraction including a possible phonon excitation due to…

High Energy Physics - Phenomenology · Physics 2008-12-18 W. Potzel

We report the measurement of broadening coefficients of pure rotational lines of methane at different pressure and temperature conditions. A total of 27 far-infrared spectra were recorded at the AILES beamline of the SOLEIL synchrotron at…

Earth and Planetary Astrophysics · Physics 2023-07-04 C. Richard , V. Boudon , L. Manceron , J. Vander Auwera , S. Vinatier , B. Bézard , M. Houelle

Using molecular dynamics simulations, we reveal emergent properties of hydrated electrode interfaces that while molecular in origin are integral to the behavior of the system across long times scales and large length scales. Specifically,…

Materials Science · Physics 2015-05-20 David T. Limmer , Adam P. Willard

Hydrogen arranges at dislocations in palladium to form nanoscale hydrides, changing the vibrational spectra. An ab initio hydrogen potential energy model versus Pd neighbor distances allows us to predict the vibrational excitations for H…

Materials Science · Physics 2011-06-01 Dallas R. Trinkle , Hyunsu Ju , Brent J. Heuser , Terrence J. Udovic

We report the preparation of sodium alanate, a promising hydrogen storage material, in a thin film form using co-sputtering in a reactive atmosphere of atomic hydrogen. We study the phase formation and distribution, and the hydrogen…

Materials Science · Physics 2009-10-14 M. Filippi , J. H. Rector , R. Gremaud , M. J van Setten , B. Dam

We theoretically and numerically analyze x-ray scattering from asymmetric-top molecules three-dimensionally aligned using elliptically polarized laser light. A rigid-rotor model is assumed. The principal axes of the polarizability tensor…

Atomic Physics · Physics 2010-05-07 Stefan Pabst , Phay J. Ho , Robin Santra

The dynamics of polarized fluorescence in reduced nicotinamide adenine dinucleotide (NADH) at 436~nm under two-photon excitation at 720~nm by femtosecond laser pulses in alcohol dehydrogenase (ADH)-containing buffer solution has been…

We have investigated sodium containing fullerene superconductors Na2AC60, A = Cs, Rb, and K, by Na-23 nuclear magnetic resonance (NMR) spectroscopy at 7.5 T in the temperature range of 10 to 400 K. Despite the structural differences from…

It is shown that if impurities in superfluid 3He have form of infinitely long non-magnetic strands, which are straight, parallel to each other and reflect quasi-particles specularly, the temperature of transition of liquid 3He from the…

Disordered Systems and Neural Networks · Physics 2019-04-22 I. A. Fomin

Noncontact Atomic Force Microscopy and synchrotron x-ray scattering measurements on dotriacontane (n-C32H66 or C32) films adsorbed on SiO2-coated Si(100) wafers reveal a narrow temperature range near the bulk C32 melting point Tb in which a…

Soft Condensed Matter · Physics 2007-05-23 M. Bai , K. Knorr , M. J. Simpson , S. Trogisch , H. Taub , S. N. Ehrlich , H. Mo , U. G. Volkmann , F. Y. Hansen

Ferroelectric phase transition in the semiconductor Sn2P2S6 single crystal has been studied by means of neutron scattering in the pressure-temperature range adjacent to the anticipated tricritical Lifshitz point (p=0.18GPa, T=296K). The…

Kinetics parameters for three anion exchange reactions - Zn-LDH-NO3 - Zn-LDH-Cl, Zn-LDH-NO3 - Zn-LDH-SO4 and Zn-LDH-NO3 - Zn-LDH-VOx - were obtained by in situ synchrotron study. The first and the second ones are two-stage reactions; the…

X-ray absorption and resonant inelastic x-ray scattering measurements are carried out on lithium nitrate LiNO$_3$. The $\sigma$ orbitals around the nitrogen atoms exhibit a large lifetime effect. Experimentally, this is manifest as an…

Materials Science · Physics 2019-09-04 John Vinson , Terrence Jach , Matthias Müller , Rainer Unterumsberger , Burkhard Beckhoff

We theoretically study the influence of laser polarization in inelastic scattering of electrons by hydrogen atoms in the presence of a circularly polarized laser field in the domain of field strengths below $10^{7}$ V/cm and high projectile…

Atomic Physics · Physics 2023-06-16 Gabriela Buică

Using helium-3 atom scattering, we have studied the adsorption kinetics, the structure and the diffusional dynamics of atomic hydrogen on the surface of a graphene monolayer on Ni(111). Diffraction measurements reveal a 4$^\circ$ rotated…

Mesoscale and Nanoscale Physics · Physics 2022-12-15 Emanuel Bahn , Anton Tamtögl , John Ellis , William Allison , Peter Fouquet

Absorption spectra of closed-shell Na_2, Na_3+, Na_4, Na_5+, Na_6, Na_7+, and Na_8 clusters are calculated using a recently implemented conserving linear response method. In the framework of a quasiparticle approach, we determine…

Materials Science · Physics 2015-05-14 George Pal , Georgios Lefkidis , Hans Christian Schneider , Wolfgang Huebner

Quasielastic neutron scattering (QENS) measurements combined with first principles based moleculardynamics calculations were conducted to study the dynamics of Li$^+$ ions in a solid-state electrolyte La$_{2/3-x}$Li$_{3x}$TiO$_{3}$ (LLTO)…

Materials Science · Physics 2021-10-01 Masato Matsuura , Yasuyuki Fujiwara , Hiroki Moriwake , Koji Ohara , Yukinobu Kawakita