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The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

We report low temperature specific heat and muon spin relaxation/rotation ($\mu$SR) measurements on both polycrystalline and single crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. This system is believed to possess a spin…

We present the results of zero-field muon-spin relaxation measurements made on the double perovskite insulators Sr$_{2}B$OsO$_6$ ($B={\rm Fe, Y, In}$). Spontaneous muon-spin precession indicative of quasistatic long range magnetic ordering…

Strongly Correlated Electrons · Physics 2016-01-27 R. C. Williams , F. Xiao , I. O. Thomas , S. J. Clark , T. Lancaster , G. A. Cornish , S. J. Blundell , W. Hayes , A. K. Paul , C. Felser , M. Jansen

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Muon spin relaxation measurements on some quantum spin ice candidate materials, the insulating pyrochlores Pr2B2O7 (B = Sn, Zr, Hf), have been performed for temperatures in the range 0.05-280 K. The results are indicative of a static…

Strongly Correlated Electrons · Physics 2015-06-22 F. R. Foronda , F. Lang , J. S. Möller , T. Lancaster , A. T. Boothroyd , F. L. Pratt , S. R. Giblin , D. Prabhakaran , S. J. Blundell

The magnetic ground state of oxynitride pyrochlore Lu$_2$Mo$_2$O$_{5-y}$N$_2$, a candidate compound for the quantum spin liquid ($S=1/2$, Mo$^{5+}$), was studied by muon spin rotation/relaxation experiment. In contrast to Lu$_2$Mo$_2$O$_7$…

Strongly Correlated Electrons · Physics 2023-01-11 S. K. Dey , K. Ishida , H. Okabe , M. Hiraishi , A. Koda , T. Honda , J. Yamaura , H. Kageyama , R. Kadono

The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…

Statistical Mechanics · Physics 2015-06-24 Adrian G. Del Maestro , Michel J. P. Gingras

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Ohta , Y. Machida , S. Nakatsuji , G. M. Luke , K. Ishida , R. H. Heffner , Lei Shu , O. O. Bernal

Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose electronic properties within a localized ion picture are characterized by non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical frustration, has…

Strongly Correlated Electrons · Physics 2015-03-17 M. Miyazaki , R. Kadono , K. H. Satoh , M. Hiraishi , S. Takeshita , A. Koda , A. Yamamoto , H. Takagi

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

Strongly Correlated Electrons · Physics 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

Geometrical frustration and spin-orbit coupling effect together play vital role to influence properties in pyrochlore based iridium oxides. Here we have investigated detailed structural, magnetic, thermodynamic and transport properties of…

Strongly Correlated Electrons · Physics 2017-02-06 Harish Kumar , A. K. Pramanik

Slow spin fluctuations ($\nu < 10^{12}$ s$^-1$) observed by the muon spin relaxation technique in Y$_{1-x}$Sc$_x$Mn$_2$ exhibits a power law dependence on temperature ($\nu \propto T^\alpha$), where the power converges asymptotically to…

Strongly Correlated Electrons · Physics 2011-06-13 M. Miyazaki , R. Kadono , M. Hiraishi , T. Masuda , A. Koda , K. M. Kojima , T. Yamazaki , Y. Tabata , H. Nakamura

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

Strongly Correlated Electrons · Physics 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

We report study of magnetization, resistivity, magnetoresistance and specific heat of the pyrochlore Iridate (Eu1-xNdx)2Ir2O7 with x=0.0, 0.5 and 1.0, where spin orbit coupling, electronic correlation, magnetic frustration and Kondo…

Strongly Correlated Electrons · Physics 2020-12-02 Sampad Mondal , M. Modak , B. Maji , M. K. Ray , S. Mandal , Swapan K. Mandal , M. Sardar , S. Banerjee

Longitudinal-field muon spin relaxation experiments have been carried out in the paramagnetic state of single-crystal Gd_2Ti_2O_7 just above the phase transition at T_m = 1.0 K. At high applied fields the exponential relaxation time T_1 is…

Strongly Correlated Electrons · Physics 2009-11-11 D. E. MacLaughlin , M. S. Rose , J. E. Anderson , Lei Shu , R. H. Heffner , T. Kimura , G. D. Morris , O. O. Bernal