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Two-pulse correlation experiments performed using pulses of different intensities on Pd(111) with different CO coverages showed that the CO photodesorption probability depends on whether the strong or the weak pulse arrives first to the…

We bring forth a consistent theory for the electron-mediated vibrational intermode coupling that clarifies the microscopic mechanism behind the vibrational relaxation of adsorbates on metal surfaces. Our analysis points out the inability of…

Materials Science · Physics 2018-04-16 Dino Novko , Maite Alducin , Joseba Iñaki Juaristi

We study hot-electron cooling by acoustic and optical phonons in monolayer MoS$_2$. The cooling power $P$ ($P_e = P/n$) is investigated as a function of electron temperature $T_e$ (0-500 $\mathrm{K}$) and carrier density $n$…

Mesoscale and Nanoscale Physics · Physics 2014-11-04 Kristen Kaasbjerg , K. S. Bhargavi , S. S. Kubakaddi

We study the electron-phonon relaxation (dephasing) rate in disordered semiconductors and low-dimensional structures. The relaxation is determined by the interference of electron scattering via the deformation potential and elastic electron…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 A. Sergeev , M. Yu. Reizer , V. Mitin

We show how coupling to an Einstein phonon $\omega_E$ affects the absorption peaks seen in the optical conductivity of graphene under a magnetic field $B$. The energies and widths of the various lines are shifted, and additional peaks arise…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Adam Pound , J. P. Carbotte , E. J. Nicol

We propose a mechanism of energy relaxation for carriers confined in a non-polar quantum dot surrounded by an amorphous polar environment. The carrier transitions are due to their interaction with the oscillating electric field induced by…

Mesoscale and Nanoscale Physics · Physics 2008-08-08 A. N. Poddubny , S. V. Goupalov , V. I. Kozub , I. N. Yassievich

Inelastic electron scattering by the adsorbate covered Pt(100) single crystal surface is studied by Disappearance Potential Spectroscopy and density of states (DOS) calculations. Two peculiar channels of elastic electron consumption are…

Materials Science · Physics 2012-09-17 A. R. Cholach , V. M. Tapilin

Manipulating energy levels while controlling the electron localization is an essential step for many applications of confined systems. In this paper we demonstrate how to achieve electron localization and induce energy level oscillation in…

Mesoscale and Nanoscale Physics · Physics 2015-05-25 Fahhad H. Alharbi , Pablo Serra , Marcelo Carignano , Sabre Kais

A model calculation is given for the energy relaxation of a non-equilibrium distribution of hot electrons prepared in a metallic sample that has been subjected to homogeneous photo-excitation by a femtosecond laser pulse. The model assumes…

Statistical Mechanics · Physics 2009-11-11 Navinder Singh

Battery electrode surfaces are generally coated with electronically insulating solid films of thickness 1-50 nm. Both electrons and Li+ can move at the electrode-surface film interface in response to the voltage, which adds complexity to…

Materials Science · Physics 2015-07-10 Kevin Leung , Andrew Leenheer

Electron relaxation is studied in endofullerene Mg@C60, after an initial localized photoexcitation in Mg, by nonadiabtic molecular dynamics simulations. To ensure reliability, two methods are used: i) an independent particle approach with a…

Atomic and Molecular Clusters · Physics 2021-06-08 Mohamed El-Amine Madjet , Esam Ali , Marcelo Carignano , Oriol Vendrell , Himadri S. Chakraborty

A thorough understanding of the energy transfer mechanism from the electric field to electrons is of utmost importance for optimization and control of different plasma sources and processes. This mechanism, called electron power absorption,…

Understanding how photoexcited electron dynamics depend on electron-electron (e-e) and electron-phonon (e-p) interaction strengths is important for many fields, e.g. ultrafast magnetism, photocatalysis, plasmonics, and others. Here, we…

Materials Science · Physics 2020-10-23 Richard Wilson , Sinisa Coh

Electron-electron interactions in general lead to both ground state and excited state confinement. We show, however, that in phenyl-substituted polyacetylenes electron-electron interactions cause enhanced delocalization of quasiparticles in…

Strongly Correlated Electrons · Physics 2009-10-31 Haranath Ghosh , Alok Shukla , Sumit Mazumdar

Molecular adsorption on surfaces plays a central role in catalysis, corrosion, desalination, and many other processes of relevance to industry and the natural world. Few adsorption systems are more ubiquitous or of more widespread…

We examine the intrinsic energy dissipation steps in electrically biased graphene channels. By combining in-situ measurements of the spontaneous optical emission with a Raman spectroscopy study of the graphene sample under conditions of…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Stéphane Berciaud , Melinda Y. Han , Louis E. Brus , Philip Kim , Tony F. Heinz

Electron-stimulated desorption (ESD) of cryosorbed molecules on surfaces is a process of relevance to fields as varied as vacuum dynamics in accelerators and astrochemistry. While desorption from such molecular systems induced by keV…

Chemical Physics · Physics 2020-11-05 Rémi Dupuy , Michal Haubner , Bernard Henrist , Jean-Hugues Fillion , Vincent Baglin

We study theoretically the piezoelectric interaction of a surface acoustic wave (SAW) with a two-dimensional electron gas confined to an isolated quantum dot. The electron motion in the dot is diffusive. The electron-electron interaction is…

Condensed Matter · Physics 2008-02-03 Andreas Knaebchen , Yehoshua Levinson , Ora Entin-Wohlman

We investigate charge relaxation rates due to acoustic phonons in weakly-confined quantum dot systems, including both deformation potential and piezoelectric field interactions. Single-electron excited states lifetimes are calculated for…

Mesoscale and Nanoscale Physics · Physics 2007-10-30 J. I. Climente , A. Bertoni , G. Goldoni , E. Molinari

We study the dynamics of an electron weakly coupled to a phonon gas. The initial state of the electron is the superposition of two spatially localized distant bumps moving towards each other, and the phonons are in a thermal state. We…

Mathematical Physics · Physics 2009-11-13 Riccardo Adami , Laszlo Erdos