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Modern theories of quantum magnetism predict exotic multipolar states in weakly interacting strongly frustrated spin-1/2 Heisenberg chains with ferromagnetic nearest neighbor (NN) inchain exchange in high magnetic fields. Experimentally…

We report a single-crystal study on the magnetism of the rare-earth compound PrTiNbO$_6$ that experimentally realizes the zigzag pseudospin-$\frac{1}{2}$ quantum antiferromagnetic chain model. Random crystal electric field caused by the…

Strongly Correlated Electrons · Physics 2018-06-05 Yuesheng Li , Sebastian Bachus , Yoshifumi Tokiwa , Alexander A. Tsirlin , Philipp Gegenwart

Single crystals of a new silver and-cobalt based vanadate AgCo2V3O10 were grown from a melted mixture. The crystal structure determination reveals that this new vanadate crystallizes in triclinic system with space group P-1. The structure…

Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus…

Strongly Correlated Electrons · Physics 2018-01-19 K. Morita , T. Sugimoto , S. Sota , T. Tohyama

We report a new peculiar effect of the interaction between a sublattice of frustrated quantum spin-1/2 chains and a sublattice of pseudospin-1/2 centers (quantum electric dipoles) uniquely co-existing in the complex oxide Li2ZrCuO4. 7Li…

Strongly Correlated Electrons · Physics 2015-05-13 E. Vavilova , A. S. Moskvin , Y. Arango , A. Sotnikov , V. Kataev , S. -L. Drechsler , R. Klingeler , O. Volkova , A. Vasiliev , B. Büchner

The strong corrugation of the V4O9 layer in the spin gap system CaV4O9 is examined for its impact on the exchange coupling constants between the spin 1/2 V ions. Local spin density (LSD) calculations show that the V spin occupies a…

Strongly Correlated Electrons · Physics 2008-02-03 W. E. Pickett

We report $^{63}$Cu nuclear magnetic resonance and muon spin rotation measurements on the S=1/2 antiferromagnetic Heisenberg spin chain compound Sr$_{1.9}$Ca$_{0.1}$CuO$_3$. An exponentially decreasing spin-lattice relaxation rate 1/T$_1$…

Strongly Correlated Electrons · Physics 2014-05-21 F. Hammerath , E. M. Brüning , S. Sanna , Y. Utz , N. S. Beesetty , R. Saint-Martin , A. Revcolevschi , C. Hess , B. Büchner , H. -J. Grafe

Electron spin resonance experiments in the quasi-1D S=1/2 antiferromagnet K$_2$CuSO$_4$Cl$_2$ reveal opening of a gap in absence of magnetic ordering, as well as an anisotropic shift of the resonance magnetic field. These features of…

Strongly Correlated Electrons · Physics 2018-11-14 T. A. Soldatov , A. I. Smirnov , K. Yu. Povarov , M. Hälg , W. E. A. Lorenz , A. Zheludev

In a frustrated J_1-J_2 chain with the nearest-neighbor ferromagnetic interaction J_1 and the next-nearest-neighbor antiferromagnetic interaction J_2, novel magnetic states such as a spin-nematic state are theoretically expected. However,…

NaOsO3 hosts a rare manifestation of a metal-insulator transition driven by magnetic correlations, placing the magnetic exchange interactions in a central role. We use resonant inelastic x-ray scattering to directly probe these magnetic…

We study the spin gap of the S=1/2 Heisenberg model on the distorted diamond chain, which is recently proposed to represent magnetic properties of Cu_3 Cl_6 (H_2 O)_2 2H_8 C_4 SO_2. This model is composed of stacked trimers and has three…

Strongly Correlated Electrons · Physics 2009-10-31 Kazuhiro Sano , Ken'ichi Takano

The temperature dependent ac and dc magnetization and heat capacity data of Ca$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derived rhombohedral structure, show the features due to magnetic ordering of a…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

We present a detailed investigation of the magnetic properties of the spin-$\frac{3}{2}$ system Li$_2$Co(WO$_4$)$_2$ by means of magnetic susceptibility and specific heat. Our experimental results show that in Li$_2$Co(WO$_4$)$_2$ a…

Strongly Correlated Electrons · Physics 2014-11-25 I. Panneer Muthuselvam , R. Sankar , A. V. Ushakov , G. Narsinga Rao , Sergey V. Streltsov , F. C. Chou

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

Strongly Correlated Electrons · Physics 2010-07-13 Gia-Wei Chern , Natalia Perkins

In both spinel compounds GeCo$_2$O$_4$ and GeNi$_2$O$_4$ which order antiferromagnetically (at $T_N = 23.5 K$ and $T_{N_1} = 12.13 K$, $T_{N_2} = 11.46 K$) with different Curie Weiss temperatures ($T_{CW}$=80.5 K and -15 K), the usual…

Strongly Correlated Electrons · Physics 2009-11-11 Sébastien Diaz , Sophie De Brion , G. Chouteau , Benjamin Canals , Virginie Simonet , P. Strobel

The spin-1/2 Cu2+ ions of LiCuVO4 form one-dimensional chains along the b-direction, and the spin frustration in LiCuVO4 is described in terms of the nearest-neighbor ferromagnetic exchange J1 and the next-nearest-neighbor antiferromagnetic…

Strongly Correlated Electrons · Physics 2011-03-09 Hyun-Joo Koo , Changhoon Lee , Myung-Hwan Whangbo , Garry J. McIntyre , Reinhard K. Kremer

We have studied the structural, magnetic properties, and electronic structure of the compound InCuPO5 synthesized by solid state reaction method. The structure of InCuPO5 comprises of S = 1/2 uniform spin chains formed by corner-shared CuO4…

Strongly Correlated Electrons · Physics 2017-05-30 B. Koteswararao , Binoy K. Hazra , Dibyata Rout , P. V. Srinivasarao , S. Srinath , S. K. Panda

We develop a microscopic theory of finite-temperature spin-nematic orderings in three-dimensional spatially anisotropic magnets consisting of weakly-coupled frustrated spin-1/2 chains with nearest-neighbor and next-nearest-neighbor…

Strongly Correlated Electrons · Physics 2013-02-19 Masahiro Sato , Toshiya Hikihara , Tsutomu Momoi

We study the phase diagram of a frustrated spin-1/2 ferromagnetic chain with anisotropic exchange interactions in an external magnetic field, using the density matrix renormalization group method. We show that an easy-axis anisotropy…

Strongly Correlated Electrons · Physics 2009-10-29 F. Heidrich-Meisner , I. P. McCulloch , A. K. Kolezhuk

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…