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Thermodynamic properties, $^{31}$P nuclear magnetic resonance (NMR) measurements, and density-functional band-structure calculations for $\varepsilon$-LiVOPO$_4$ are reported. This quantum magnet features a singlet ground state and…

Strongly Correlated Electrons · Physics 2020-06-03 Prashanta K. Mukharjee , K. M. Ranjith , M. Baenitz , Y. Skourski , A. A. Tsirlin , R. Nath

We report a 51V nuclear magnetic resonance investigation of the frustrated spin-1/2 chain compound LiCuVO4, performed in pulsed magnetic fields and focused on high-field phases up to 55 T. For the crystal orientations H // c and H // b we…

Isotropic and anisotropic magnetic behavior of the frustrated spin chain compound $\beta$-TeVO$_4$ is reported. Three magnetic transitions observed in zero magnetic field are tracked in fields applied along different crystallographic…

Magnetic excitations in an array of (VO)2P2O7 single crystals have been measured using inelastic neutron scattering. Until now, (VO)2P2O7 has been thought of as a two-leg antiferromagnetic Heisenberg spin ladder with chains running in the…

Statistical Mechanics · Physics 2008-02-03 Alan Tennant , Stephen Nagler , Ted Barnes , Andrew Garrett , Jose Riera , Brian Sales

Frustrated spin-1/2 chains, despite the apparent simplicity, exhibit remarkably rich phase diagram comprising vector-chiral (VC), spin-density-wave (SDW) and multipolar/spin-nematic phases as a function of the magnetic field. Here we report…

Strongly Correlated Electrons · Physics 2019-09-24 M. Pregelj , A. Zorko , M. Klanjšek , O. Zaharko , J. S. White , O. Prokhnenko , M. Bartkowiak , H. Nojiri , H. Berger , D. Arčon

We present here a study of the magnetic properties of the antiferromagnetic dimer material CuVOF$_4$(H$_2$O)$_6\cdot$H$_2$O, in which the dimer unit is composed of two different $S = 1/2$ species, Cu(II) and V(IV). An applied magnetic field…

We report on the microscopic magnetic model of a spin-1/2 magnet BaV$_3$O$_8$. In contrast to earlier phenomenological analysis, our density-functional band-structure calculations combined with quantum Monte-Carlo simulations establish a…

Materials Science · Physics 2014-01-09 Alexander A. Tsirlin

$\beta$-TeVO$_4$ is a frustrated spin 1/2 zig-zag chain system,where spin-density-wave (SDW), vector chiral (VC)and an exotic dynamic spin-stripe phase compete at low temperatures. Here we use torque magnetometry to study the anisotropy of…

Strongly Correlated Electrons · Physics 2020-07-16 M. Herak , N. Novosel , M. Dragičević , Thierry Guizouarn , Olivier Cador , Helmuth Berger , Matej Pregelj , Andrej Zorko , Denis Arčon

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

Materials Science · Physics 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

We investigate the spin-stripe mechanism responsible for the peculiar nanometer modulation of the incommensurate magnetic order that emerges between the vector-chiral and the spin-density-wave phase in the frustrated zigzag spin-1/2 chain…

Strongly Correlated Electrons · Physics 2016-08-31 M. Pregelj , O. Zaharko , M. Herak , M. Gomilsek , A. Zorko , L. C. Chapon , F. Bourdarot , H. Berger , D. Arčon

We report an investigation on structure and magnetic properties of the $S=3/2$ zigzag spin chain compound BaCoTe$_2$O$_7$. Neutron diffraction measurements reveal BaCoTe$_2$O$_7$ crystallizes in the noncentrosymmetric space group $Ama2$…

Strongly Correlated Electrons · Physics 2021-07-06 Lisi Li , Xunwu Hu , Zengjia Liu , Jia Yu , Benyuan Cheng , Sihao Deng , Lunhua He , Kun Cao , Dao-Xin Yao , Meng Wang

We report magnetic susceptibility, specific heat, and Raman scattering investigations of alpha-TeVO4 containing V-O edge-sharing chains. These chains promote a system of ferromagnetic/antiferromagnetic spin-1/2 Heisenberg alternating…

Strongly Correlated Electrons · Physics 2010-03-09 V. Gnezdilov , P. Lemmens , A. A. Zvyagin , V. O. Cheranovskii , K. Lamonova , Yu. G. Pashkevich , R. K. Kremer , H. Berger

Magnetization of the frustrated $S=1/2$ chain compound LiCuVO$_4$, focusing on high magnetic field phases, is reported. Besides a spin-flop transition and the transition from a planar spiral to a spin modulated structure observed recently,…

Strongly Correlated Electrons · Physics 2011-03-03 L. E. Svistov , T. Fujita , H. Yamaguchi , S. Kimura , K. Omura , A. Prokofiev , A. I. Smirnov , Z. Honda , M. Hagiwara

We report on the dynamics of the spin-1/2 quasi-one-dimensional frustrated magnet LiCuVO$\mathrm{_4}$ measured by nuclear spin relaxation in high magnetic fields 10--34 T, in which the ground state has spin-density-wave order. The spin…

Strongly Correlated Electrons · Physics 2017-11-27 Kazuhiro Nawa , Masashi Takigawa , Steffen Krämer , Mladen Horvatić , Claude Berthier , Makoto Yoshida , Kazuyoshi Yoshimura

A microscopic magnetic model for the spin-1/2 Heisenberg chain compound CuSe2O5 is developed based on the results of a joint experimental and theoretical study. Magnetic susceptibility and specific heat data give evidence for quasi-1D…

Strongly Correlated Electrons · Physics 2009-11-20 O. Janson , W. Schnelle , M. Schmidt , Yu. Prots , S. -L. Drechsler , S. K. Filatov , H. Rosner

Competing magnetic interactions in low-dimensional quantum magnets can lead to the exotic ground state with fractionalized excitations. Herein, we present our results on an S = 5/2 quasi-one-dimensional spin system Bi3FeMo2O12. The…

We consider the spin-1/2 Heisenberg chain with alternating spin exchange %on even and odd sites in the presence of additional modulation of exchange on odd bonds with period three. We study the ground state magnetic phase diagram of this…

Strongly Correlated Electrons · Physics 2015-05-30 M. Shahri Naseri , G. I. Japaridze , S. Mahdavifar , S. Farjami Shayesteh

We study electronic and magnetic properties of the quasi-one-dimensional spin-1/2 magnet Ba3Cu3Sc4O12 with a distinct orthogonal connectivity of CuO4 plaquettes. An effective low-energy model taking into account spin-orbit coupling was…

Strongly Correlated Electrons · Physics 2016-09-14 D. I. Badrtdinov , O. S. Volkova , A. A. Tsirlin , I. V. Solovyev , A. N. Vasiliev , V. V. Mazurenko

Employing first-principles modelling and many-body methods, the magnetic properties of spin-1/2 chain compound NaVOPO$_4$ are explored. The extensive first-principles calculations establish an intricate three-dimensionally coupled model…

Strongly Correlated Electrons · Physics 2024-08-30 Manoj Gupta , Manodip Routh , Manoranjan Kumar , Tanusri Saha Dasgupta

Magnetic excitations in an array of (VO)_2P_2O_7 single crystals have been measured using inelastic neutron scattering. Until now, (VO)_2P_2O_7 has been thought of as a two-leg antiferromagnetic Heisenberg spin ladder with chains running in…

Condensed Matter · Physics 2016-08-31 A. W. Garrett , S. E. Nagler , D. A. Tennant , B. C. Sales , T. Barnes