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We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…

Atomic Physics · Physics 2021-03-30 Hakon Volkmann , Vinay P. Majety , Armin Scrinzi

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

A new scheme for a double-slit experiment in the time domain is presented. Phase-stabilized few-cycle laser pulses open one to two windows (``slits'') of attosecond duration for photoionization. Fringes in the angle-resolved energy spectrum…

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

We investigate the carrier-envelope phase and intensity dependence of the longitudinal momentum distribution of photoelectrons resulting from above-threshold ionization of argon by few-cycle laser pulses. The intensity of the pulses with a…

Atomic Physics · Physics 2018-07-04 M. Kübel , M. Arbeiter , C. Burger , Nora G. Kling , T. Pischke , R. Moshammer , T. Fennel , M. F. Kling , B. Bergues

Light-induced states are commonly observed in the photoionization spectra of laser-dressed atoms. The properties of autoionizing polaritons, entangled states of light and Auger resonances, however, are largely unexplored. We employ…

Atomic Physics · Physics 2021-07-14 Nathan Harkema , Coleman Cariker , Eva Lindroth , Luca Argenti , Arvinder Sandhu

We present measurements of the second-order coherence function on emission from single GaN quantum dots. In some cases a large degree of photon antibunching is observed, demonstrating isolation of a single quantum system. For a selected…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Charles Santori , Stephan Gotzinger , Yoshihisa Yamamoto , Satoshi Kako , Katsuyuki Hoshino , Yasuhiko Arakawa

Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…

Accelerator Physics · Physics 2025-07-01 Andreas Seidel , Carola Zepter , Alexander Sävert , Stephan Kuschel , Matt Zepf

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

We demonstrate an optical method for detecting the mechanical oscillations of an atom with single-phonon sensitivity. The measurement signal results from the interference between the light scattered by a single trapped atomic ion and that…

Atomic Physics · Physics 2021-08-11 G. Cerchiari , G. Araneda , L. Podhora , L. Slodička , Y. Colombe , R. Blatt

A Kohn-Sham time-dependent local-density-functional scheme is utilized to predict attosecond time delays of xenon 4d photoionization that involves the 4d giant dipole resonance and Cooper minimum. The fundamental effect of electron…

Atomic Physics · Physics 2021-06-08 Maia Magrakvelidze , Mohamed El-Amine Madjet , Himadri S. Chakraborty

Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…

Optics · Physics 2023-02-22 H. Y. Kim , M. Garg , S. Mandal , L. Seiffert , T. Fennel , E. Goulielmakis

Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…

Optics · Physics 2020-05-20 Constantin Krüger , Jaco Fuchs , Laura Cattaneo , Ursula Keller

Experimental cross sections for $m$-fold photodetachment ($m=3-6$) of silicon anions via $K$-shell excitation and ionization were measured in the photon-energy range of 1830-1900 eV using the photon-ion merged-beams technique at a…

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…

Materials Science · Physics 2021-04-26 E. E. Krasovskii , R. O. Kuzian

Photoionization is a key step in many attosecond processes. Accurately determining the photoionization time delay is critical to understanding electron dynamics during and after ionization and can guide future efforts to manipulate electron…

Atomic Physics · Physics 2026-02-26 J. Aygun , D. Yaacoub , A. L. Harris

Gas phase C$_{70}$ molecules have been ionized with single photons of energies between 16 eV and 70 eV and the electron spectra measured with velocity map imaging in coincidence with the ions. The doubly ionized and unfragmented species was…