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The effects of confinement resonances on photoelectron group delay (Wigner time delay) following ionization of an atom encapsulated inside a C$_{60}$ cage have been studied theoretically using both relativistic and non-relativistic random…

Atomic Physics · Physics 2014-06-11 P. C. Deshmukh , A. Mandal , S. Saha , A. S. Kheifets , V. K. Dolmatov , S T Manson

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

In a seminal article, Fano predicts that absorption of light occurs preferably with increase of angular momentum. Here we generalize Fano's propensity rule to laser-assisted photoionization, consisting of absorption of an…

The photoelectric effect has a sister process relevant in optoelectronics called internal photoemission. Here an electron is photoemitted from a metal into a semiconductor. While the photoelectric effect takes place within less than 100…

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

High harmonic spectroscopy can access structural and dynamical information on molecular systems encoded in amplitude and phase of high harmonic generation (HHG) signals4. However, measurement of the harmonic phase is a daunting task. Here…

Through examining the product of the mathematical variance of intensity with respect to time and frequency, we arrive at a temporal characterization of laser pulses through parameters for pulse duration, group delay dispersion and temporal…

Phase and time delays of atomic above-threshold ionization are usually experimentally explored by the reconstruction of attosecond harmonic beating by interference of two-photon transitions (RABBIT) technique. Theoretical studies of RABBIT…

Atomic Physics · Physics 2024-03-25 Sebastián D. López , Matias L. Ocello , Diego G. Arbó

We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of…

We present a combined theoretical and experimental work investigating the angle-resolved phases of the photoionization process driven by a two-color field consisting of an attosecond pulse train and an infrared pulse in an ensemble of…

We theoretically study the photoelectron angular distributions (PADs) from two-color two-photon near-threshold ionization of hydrogen and noble gas (He, Ne, and Ar) atoms by a combined action of femtosecond extreme ultraviolet (EUV) and…

Atomic Physics · Physics 2015-06-22 Kenichi L. Ishikawa , A. K. Kazansky , N. M. Kabachnik , Kiyoshi Ueda

We study ionization of aligned H$_2^+$ in strong elliptically-polarized laser fields numerically and analytically. The calculated offset angle in photoelectron momentum distribution is several degrees larger for the molecule than a model…

Atomic Physics · Physics 2023-01-03 J. Y. Che , Y. G. Peng , F. B. Zhang , X. J. Xie , G. G. Xin , Y. J. Chen

We present measurements of the pulse length of ultracold electron bunches generated by near-threshold two-photon photoionization of a laser-cooled gas. The pulse length has been measured using a resonant $3$ GHz deflecting cavity in…

Atomic Physics · Physics 2017-03-24 J. G. H. Franssen , T. L. I. Frankort , E. J. D. Vredenbregt , O. J. Luiten

We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the…

Atomic Physics · Physics 2020-08-26 Renata Della Picca , Ana Alicia Gramajo , Sebastián López , Diego G Arbó

Adiabatic passage techniques allow the generation of single photons which are very long compared to the typical detector time resolution. Therefore the detection time of a photon can be measured within the duration of the single-photon…

Quantum Physics · Physics 2011-09-06 T. Legero , T. Wilk , A. Kuhn , G. Rempe

Single, double, and triple ionization of the C+ ion by a single photon have been investigated in the energy range 286 to 326 eV around the K-shell single-ionization threshold at an unprecedented level of detail. At energy resolutions as low…

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

Time delays in photoemission are on the order of attoseconds and have been experimentally determined in atoms, molecules and solids. Their magnitude and energy dependence are expected to yield fundamental insights into the properties of the…

In this study, we investigate the potential of electronic interferometers for probing the quantum state of electromagnetic radiation on a chip at sub-nanosecond time scales. We propose to use single electron excitations propagating within…

Quantum Physics · Physics 2024-05-10 H. Souquet-Basiège , B. Roussel , G. Rebora , G. Ménard , I. Safi , G. Fève , P. Degiovanni