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We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…

Strongly Correlated Electrons · Physics 2016-08-31 H. Fukazawa , R. G. Melko , R. Higashinaka , Y. Maeno , M. J. P. Gingras

A spin-ice compound dysprosium titanate, Dy2Ti2O7, is studied by specific heat measurements in magnetic fields applied along the [110] direction of the cubic unit cell. Above a magnetic field of 0.4 T a relatively sharp peak at T = 1.1 K in…

Materials Science · Physics 2009-11-10 Zenji Hiroi , Kazuyuki Matsuhira , Masao Ogata

We present time-of-flight inelastic neutron scattering measurements at low temperature on powder samples of the magnetic pyrochlore oxides Tb2Ti2O7 and Tb2Sn2O7. These two materials possess related, but different ground states, with…

Strongly Correlated Electrons · Physics 2014-05-01 J. Zhang , K. Fritsch , Z. Hao , B. V. Bagheri , M. J. P. Gingras , G. E. Granroth , P. Jiramongkolchai , R. J. Cava , B. D. Gaulin

We present a first-principles investigation of the spin-ice state in Dy$_2$Ti$_2$O$_7$ using a magnetic source-free exchange and correlation functional, implemented in the Castep electronic-structure code. By comparing results from the…

Materials Science · Physics 2023-02-20 Z. Hawkhead , N. Gidopoulos , S. J. Blundell , S. J. Clark , T. Lancaster

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

Strongly Correlated Electrons · Physics 2018-10-03 S. K. Takahashi , A. Arsenault , C. Mauws , A. M. Hallas , C. Sarkis , K. A. Ross , C. R. Wiebe , M. Tachibana , G. M. Luke , T. Imai

We study quantum antiferromagnetism on the highly frustrated checkerboard lattice, also known as the square lattice with crossings. The quantum Heisenberg antiferromagnet on this lattice is of interest as a two-dimensional analog of the…

Statistical Mechanics · Physics 2015-06-24 R. Moessner , Oleg Tchernyshyov , S. L. Sondhi

Magnetization, magnetocaloric, calorimetric, neutron and X-ray diffraction and inelastic neutron scattering measurements are performed on single crystals of BaCdVO(PO$_4$)$_2$. The low-temperature crystal structure is found to be of a lower…

Strongly Correlated Electrons · Physics 2019-11-07 V. K. Bhartiya , K. Yu. Povarov , D. Blosser , S. Bettler , Z. Yan , S. Gvasaliya , S. Raymond , E. Ressouche , K. Beauvois , J. Xu , F. Yokaichiya , A. Zheludev

We identify the low energy effective Hamiltonian that is expected to describe the low temperature properties of the frustrated magnet $\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$. Motivated by the fact that this effective Hamiltonian…

Strongly Correlated Electrons · Physics 2018-03-07 Sounak Biswas , Kedar Damle

The recent discoveries of proximate quantum spin-liquid compounds and their potential application in quantum computing informs the search for new candidate materials for quantum spin-ice and spin-liquid physics. While the majority of such…

Strongly Correlated Electrons · Physics 2019-01-16 K. M. Taddei , L. Sanjeewa , J. W. Kolis , A. S. Sefat , C. de la Cruz , D. M. Pajerowski

We report vibrating coil magnetometry of the spin ice system Ho2Ti2O7 down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History dependent behavior emerges below T*_0 ~ 0.6 K near zero magnetic field, in…

Strongly Correlated Electrons · Physics 2012-06-25 C. Krey , S. Legl , S. R. Dunsiger , M. Meven , J. S. Gardner , J. M. Roper , C. Pfleiderer

The pyrochlore material Nd$_2$Zr$_2$O$_7$ with an "all-in-all-out" (AIAO) magnetic order shows novel quantum moment fragmentation with gapped flat dynamical spin ice modes. The parameterized spin Hamiltonian with a dominant frustrated…

Materials Science · Physics 2020-03-11 J. Xu , Owen Benton , A. T. M. N. Islam , T. Guidi , G. Ehlers , B. Lake

We have studied long range orders of electric quadrupole moments described by an effective pseudospin-$\frac{1}{2}$ Hamiltonian representing pyrochlore magnets with non-Kramers ions under [111] magnetic field, in relevance to…

Strongly Correlated Electrons · Physics 2021-07-06 Hiroaki Kadowaki , Hiroshi Takatsu , Mika Wakita

There are two discrepant experimental results on the magnetic ground state of Y$_{2}$Mn$_{2}$O$_{7}$, one study proposes a spin glass state, while another introduces the material as a ferromagnet. In this study, we attempt to resolve this…

Materials Science · Physics 2020-09-09 Mohammad Amirabbasi , Mojtaba Alaei

Geometric frustration usually arises in systems that comprise magnetic moments (spins) which reside on the sites of a lattice made up of elementary triangular or tetrahedral units and which interact via antiferromagnetic nearest-neighbor…

Statistical Mechanics · Physics 2009-03-17 Michel J. P. Gingras

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

We investigate theoretically the phase diagram of a classical Heisenberg antiferromagnet on the pyrochlore lattice perturbed by a weak second-neighbor interaction J_2. The huge ground state degeneracy of the nearest-neighbor Heisenberg…

Strongly Correlated Electrons · Physics 2009-07-17 Gia-Wei Chern , R. Moessner , O. Tchernyshyov

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

We study spin correlations for the highly frustrated classical pyrochlore lattice antiferromagnets with O(N) symmetry in the limit T->0. We conjecture that a local constraint obeyed by the extensively degenerate ground states dictates a…

Disordered Systems and Neural Networks · Physics 2016-08-31 S. V. Isakov , K. Gregor , R. Moessner , S. L. Sondhi

Spin ice, a peculiar thermal state of a frustrated ferromagnet on the pyrochlore lattice, has a finite entropy density and excitations carrying magnetic charge. By combining analytical arguments and Monte Carlo simulations, we show that…

Strongly Correlated Electrons · Physics 2011-05-24 Gia-Wei Chern , Paula Mellado , O. Tchernyshyov

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…