English

Dimensional change of quadrupole orders in pseudospin-$\frac{1}{2}$ pyrochlore magnets under [111] field

Strongly Correlated Electrons 2021-07-06 v3

Abstract

We have studied long range orders of electric quadrupole moments described by an effective pseudospin-12\frac{1}{2} Hamiltonian representing pyrochlore magnets with non-Kramers ions under [111] magnetic field, in relevance to Tb2_{2}Ti2_{2}O7_{7}. Order parameters and phase transitions of this frustrated system are investigated using classical Monte-Carlo simulations. In zero field, the model undergoes a first-order phase transition from a paramagnetic state to an ordered state with an antiparallel arrangement of pseudospins. This pseudospin order is characterized by the wavevector k=0\boldsymbol{k}=0 and is selected by an energetic or an order-by-disorder mechanism from degenerate k=(h,h,h)\boldsymbol{k}=(h,h,h) mean-field orders. Under [111] magnetic field this three-dimensional quadrupole order is transformed to a quasi two-dimensional quadrupole order on each kagom\'{e} lattice separated by field-induced ferromagnetic triangular lattices. We discuss implication of the simulation results with respect to experimental data of Tb2_{2}Ti2_{2}O7_{7}.

Keywords

Cite

@article{arxiv.1807.07722,
  title  = {Dimensional change of quadrupole orders in pseudospin-$\frac{1}{2}$ pyrochlore magnets under [111] field},
  author = {Hiroaki Kadowaki and Hiroshi Takatsu and Mika Wakita},
  journal= {arXiv preprint arXiv:1807.07722},
  year   = {2021}
}

Comments

11 pages, 10 figures; Fig. 1 and Eqs. (A1), (A2), (A3) are corrected (v3)