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The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

Strongly Correlated Electrons · Physics 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

Specific heat, elastic neutron scattering, and muon spin rotation ($\mu$SR) experiments have been carried out on a well-characterized sample of "stuffed" (Pr-rich) Pr$_{2+x}$Ir$_{2-x}$O$_{7-\delta}$. Elastic neutron scattering shows the…

Spin ordering in TbBaCo2O5.5 and its temperature transformation is studied. Polymorphism due to the oxygen ordering with the average content close to 5.5 is investigated. One of ceramic samples (I), in addition to the main phase ap x 2ap x…

Ruthenium-based perovskite systems are attractive because their Structural, electronic and magnetic properties can be systematically engineered. SrRuO$_3$/SrTiO$_3$ superlattice, with its period consisting of one unit cell each, is very…

Strongly Correlated Electrons · Physics 2012-10-15 Mingqiang Gu , Qiyun Xie , Xuan Shen , Rubin Xie , Jianli Wang , Gang Tang , Di Wu , G. P. Zhang , X. S. Wu

We give a quantitative analysis of the previously published nuclear magnetic resonance (NMR) experiments in the k-(ET)2X family of organic charge transfer salts by using the phenomenological spin fluctuation model of Moriya, and Millis,…

Strongly Correlated Electrons · Physics 2009-11-13 Eddy Yusuf , B. J. Powell , Ross H. McKenzie

The magnetic structure and metal-insulator transition in antiferromagnetic (AFM) BaMn2As2 and Ba1-xKxMn2As2 single crystals have been investigated by 55Mn and 75As nuclear magnetic resonance (NMR) measurements. In the parent AFM insulator…

Strongly Correlated Electrons · Physics 2014-05-23 S. Yeninas , Abhishek Pandey , V. Ogloblichev , K. Mikhalev , D. C. Johnston , Y. Furukawa

Results of the nuclear resonance experiments for the planar Cu sites in PrBa2Cu4O8 are presented. The NMR spectrum at 1.5 K in zero magnetic field revealed an internal field of 6.1 T, providing evidence for an antiferromagnetic order of the…

Strongly Correlated Electrons · Physics 2009-11-07 S. Fujiyama , M. Takigawa , T. Suzuki , N. Yamada , S. Horii , Y. Yamada

We investigate a (semi-)metal to insulator transition (MIT) realized in geometrically frustrated electron systems on the basis of the Hubbard model on a three-dimensional pyrochlore lattice and a two-dimensional checkerboard lattice. Using…

Strongly Correlated Electrons · Physics 2009-11-10 Satoshi Fujimoto

Cd2Os2O7 shows a peculiar metal-insulator transition at 227 K with magnetic ordering in a frustrated pyrochlore lattice, but its magnetic structure in the ordered state and the transition origin are yet uncovered. We observed a commensurate…

Strongly Correlated Electrons · Physics 2012-06-20 J. Yamaura , K. Ohgushi , H. Ohsumi , T. Hasegawa , I. Yamauchi , K. Sugimoto , S. Takeshita , A. Tokuda , M. Takata , M. Udagawa , M. Takigawa , H. Harima , T. Arima , Z. Hiroi

We discuss the notions of spin-orbital polarization and ordering in paramagnetic materials, and address their consequences in transition metal oxides. Extending the combined density functional and dynamical mean field theory scheme to the…

Strongly Correlated Electrons · Physics 2014-12-16 Cyril Martins , Markus Aichhorn , Loig Vaugier , Silke Biermann

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

Combining density functional theory (DFT) and embedded dynamical mean-field theory (DMFT) methods, we study the metal-insulator transition in $R_2$Ir$_2$O$_7$ ($R$=Y, Eu, Sm, Nd, Pr, and Bi) and the topological nature of the insulating…

Strongly Correlated Electrons · Physics 2017-01-18 Hongbin Zhang , Kristjan Haule , David Vanderbilt

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

Materials Science · Physics 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition…

Strongly Correlated Electrons · Physics 2014-12-12 Hiroshi Takatsu , Kunihiko Watanabe , Kazuki Goto , Hiroaki Kadowaki

The electronic structures of the metallic and insulating phases of the alloy series Ca(2-x)Sr(x)RuO4 (0 <= x <= 2) are calculated using LDA, LDA+U and Dynamical Mean-Field Approximation methods. In the end members the groundstate…

Strongly Correlated Electrons · Physics 2009-09-25 V. I. Anisimov , I. A. Nekrasov , D. E. Kondakov , T. M. Rice , M. Sigrist

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

Strongly Correlated Electrons · Physics 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

The canting angles and fluctuation of the magnetic ion spins of spinel oxide MnCr${}_2$O${}_4$ were studied by nuclear magnetic resonance (NMR) at low temperatures, which has a collinear ferrimagnetic order below $T_C$ and a ferrimagnetic…

Strongly Correlated Electrons · Physics 2015-05-19 Dong Young Yoon , Soonchil Lee , Yoon Seok Oh , Kee Hoon Kim

Neutron diffraction studies have been carried out on a single crystal of oxygen-deficient perovskite TbBaCo2O5.5 in the temperature range of 7-370 K. There have been observed several magnetic or structural transitions. Among these, the…

Strongly Correlated Electrons · Physics 2009-11-10 Minoru Soda , Yukio Yasui , Toshiaki Fujita , Takeshi Miyashita , Masatoshi Sato , Kazuhisa Kakurai