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A new pyrochlore ruthenium oxide, Hg2Ru2O7 was synthesized under a high pressure of 6 GPa. In contrast to the extensively studied Ru4+ oxides, this compound possesses a novel Ru5+ valence state, corresponding to a half-filled t_2g_3…

Muon spin relaxation measurements on the filled skutterudite compound SmRu4P12 have been carried out in zero- and longitudinal-fields. Temperature dependence of both initial asymmetry and muon-spin depolarization rate show the appearance of…

Strongly Correlated Electrons · Physics 2009-11-11 K. Hachitani , H. Fukazawa , Y. Kohori , I. Watanabe , C. Sekine , I. Shirotani

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Anomalous low temperature electronic and structural behaviour has been discovered in PbRuO3. The structure (space group Pnma, a = 5.56314(1), b = 7.86468(1), c = 5.61430(1) A) and metallic conductivity at 290 K are similar to those of…

Strongly Correlated Electrons · Physics 2009-11-13 S. A. J. Kimber , J. A. Rodgers , H. Wu , C. A. Murray , D. N. Argyriou , A. N. Fitch , D. I. Khomskii , J. P. Attfield

Muon-spin relaxation results on the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ are reported. Spontaneous coherent muon-spin precession below the metal-insulator transition (MIT) temperature of about 33 K is observed, indicating the appearance of…

Strongly Correlated Electrons · Physics 2013-09-03 Hanjie Guo , Kazuyuki Matsuhira , Ikuto Kawasaki , Makoto Wakeshima , Yukio Hinatsu , Isao Watanabe , Zhu-an Xu

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

We investigated the magnetoresistance (MR) effect of the pyrochlore oxide Nd2Ir2O7, which shows a metal-insulator transition at T_MI =33 K. A small positive MR effect was observed in the metallic state above T_MI, while a large negative MR…

Strongly Correlated Electrons · Physics 2013-01-18 Kazuyuki Matsuhira , Masashi Tokunaga , Makoto Wakeshima , Yukio Hinatsu , Seishi Takagi

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose electronic properties within a localized ion picture are characterized by non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical frustration, has…

Strongly Correlated Electrons · Physics 2015-03-17 M. Miyazaki , R. Kadono , K. H. Satoh , M. Hiraishi , S. Takeshita , A. Koda , A. Yamamoto , H. Takagi

We report the observation of metal-like to insulator transition (MTI) in the 3dpyrochlore oxide Tb2Ti2O7 at 603 K due to the interaction of empty 3d orbitals of Ti4+ with O2- ions, evidenced by the transition in resistivity. Magnetisation,…

Materials Science · Physics 2020-07-28 B. Santhosh Kumar , C. Venkateswaran

The consecutive magnetic ordering of the Ho and Ru ions in the pyrochlore Ho2Ru2O7 and their interplay are investigated by neutron scattering, magnetic and specific heat measurements. The Ru moments order at 95 K into a $\Gamma_5$…

We present measurements of the magnetic moment and specific heat of single crystals of the spin-chain insulator, Pr3RuO7. The susceptibility indicates that three-dimensional antiferromagnetic order sets in at TN = 54 K, with spin…

Strongly Correlated Electrons · Physics 2009-11-11 M. Freamat , X. N. Lin , V. Durairaj , S. Chikara , G. Cao , J. W. Brill

Neutron scattering measurements on the spin-ice candidate material Ho$_2$Ru$_2$O$_7$ have revealed two magnetic transitions at T $\sim$ 95 K and T $\sim$ 1.4 K to long-range ordered states involving the Ru and Ho sublattices, respectively.…

Statistical Mechanics · Physics 2009-11-10 C. R. Wiebe , J. S. Gardner , S. -J. Kim , G. M. Luke , A. S. Wills , B. D. Gaulin , J. E. Greedan , I. Swainson , Y. Qiu , C. Jones

We present magnetization and Hall effect measurements on the pyrochlore iridate Nd2Ir2O7. Previous muon spin rotation measurements have shown that the system undergoes an unusual transition at T$_M$ = 110 K into a magnetic phase lacking…

Strongly Correlated Electrons · Physics 2015-06-12 S. M. Disseler , S. R. Giblin , Chetan Dhital , K. C. Lukas , Stephen D. Wilson , M. J. Graf

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Our single crystal study of the magneto-thermal and transport properties of the pyrochlore iridate Eu2Ir2O7 reveals a continuous phase transition from a paramagnetic metal to an antiferromagnetic insulator for a sample with stoichiometry…

Strongly Correlated Electrons · Physics 2015-06-04 Jun J. Ishikawa , Eoin C. T. O'Farrell , Satoru Nakatsuji

R$_2$Mo$_2$O$_7$ compounds show a ferromagnetic metal-insulator spin glass transition tuned by the radius of the rare earth ion R$^{3+}$. We have studied Gd$_2$Mo$_2$O$_7$ located on the verge of the transition, by neutron diffraction on a…

Strongly Correlated Electrons · Physics 2007-05-23 I. Mirebeau , A. Apetrei , I. Goncharenko , D. Andreica , P. Bonville , J. P. Sanchez , A. Amato , E. Suard , W. A. Crichton

We investigate the metal-insulator transition in the layered Ruddelsden Popper series of strontium iridates Srn+1IrnO3n+1. Tight-binding models of t2g orbitals for n = 1, 2, and infinity are constructed, and changes in band dispersion due…

Strongly Correlated Electrons · Physics 2015-06-05 Jean-Michel Carter , V. Vijay Shankar , Hae-Young Kee

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim
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