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Upon rapid quenching of temperature of a glass forming liquid, the system falls out of equilibrium due its finite relaxation time. Additionally, the relaxation becomes progressively slower with time. The created nonequilibrium state of the…

Statistical Mechanics · Physics 2025-12-16 Biman Bagchi

We present ac susceptibility and specific heat measurements taken on samples of LiHo$_x$Y$_{1-x}$F$_4$ in the dilute limit: x = 0.018, 0.045, 0.080 and 0.12. Susceptibility measurements show glassy behavior including wide absorption spectra…

Disordered Systems and Neural Networks · Physics 2015-06-05 J. A. Quilliam , S. Meng , J. B. Kycia

We propose a computational strategy to quantify the temperature evolution of the timescales and lengthscales over which dynamic facilitation affects the relaxation dynamics of glass-forming liquids at low temperatures, that requires no…

Soft Condensed Matter · Physics 2024-06-25 Cecilia Herrero , Ludovic Berthier

Sub-coercive field non-linearities in $0.5(\text{Ba}_{0.7}\text{Ca}_{0.3}\text{TiO}_{3})-0.5(\text{BaZr}_{0.2}\text{Ti}_{0.8}\text{O}_{3})$ (BCTZ 50/50) thin film elaborated using pulsed laser deposition are studied using permittivity and…

This work aims at reconsidering several interpretations coexisting in the recent literature concerning non-linear susceptibilities in supercooled liquids. We present experimental results on glycerol and propylene carbonate showing that the…

Disordered Systems and Neural Networks · Physics 2017-11-02 P. Gadige , S. Albert , M. Mich , Th. Bauer , P. Lunkenheimer , A. Loidl , R. Tourbot , C. Wiertel-Gasquet , G. Biroli , J. -P. Bouchaud , F. Ladieu

In order to point out the influence of thermal history (fictive temperature) and OH content on the elastic properties of silica glass, we have performed high resolution in situ Brillouin spectra of SiO2 glass from room temperature to the…

Materials Science · Physics 2007-05-23 R Le Parc , C Levelut , J Pelous , V. Martinez , B Champagnon

The glass transition temperature $T_g$ and the temperature $T_{\alpha}$ corresponding to the peak in the dielectric loss due to the $\alpha$-process have been simultaneously determined as functions of film thickness $d$ through dielectric…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

We report a computer simulation study of the glass transition for water. To mimic the difference between standard and hyperquenched glass, we generate glassy configurations with different cooling rates and calculate the $T$ dependence of…

Soft Condensed Matter · Physics 2016-08-31 Nicolas Giovambattista , C. Austen Angell , Francesco Sciortino , H. Eugene Stanley

The observation of coherent quantum transport phenomena in metals and semiconductors is limited by the eventual loss of phase coherence of the conducting electrons. We use the weak localization effect to measure the low-temperature…

Mesoscale and Nanoscale Physics · Physics 2010-08-27 M. Eshkol , E. Eisenberg , M. Karpovski , A. Palevski

We argue that for generic systems close to a critical point, an extended Fluctuation-Dissipation relation connects the low frequency non-linear (cubic) susceptibility to the four-point correlation function. In glassy systems, the latter…

Statistical Mechanics · Physics 2009-11-11 Jean-Philippe Bouchaud , Giulio Biroli

We propose a new simple way to evaluate the effect of anharmonicity on a system's thermodynamic functions such as heat capacity. In this approach, the contribution of all potentially complicated anharmonic effects to constant-volume heat…

Statistical Mechanics · Physics 2015-06-15 E. I. Andritsos , E. Zarkadoula , A. E. Phillips , M. T. Dove , C. J. Walker , V. V. Brazhkin , K. Trachenko

Self diffraction is a four-wave mixing process proportional to the square modulus of third-order nonlinearity susceptibility $\chi^{(3)}$, which is related to the material's electronic and thermal properties. In this study, we investigate…

A novel approach has been developed to calculate the temperature dependence of the optical response of a semiconductor. The dielectric function is averaged over several thermally perturbed configurations that are extracted from molecular…

Materials Science · Physics 2011-05-27 Z. A. Ibrahim , A. I. Shkrebtii , M. J. G. Lee , K. Vynck , T. Teatro , W. Richter , T. Trepk , T. Zettler

We present a simple method for fast and cheap thermal analysis on supercooled glass-forming liquids. This "Thermalization Calorimetry" technique is based on monitoring the temperature and its rate of change during heating or cooling of a…

We show that a viscous liquid confined between two low thermal conductive surfaces (Al2O3) emit a thermal response upon applying a low frequency (Hz) shear excitation. Hot and cold thermal waves are observed in situ at atmospheric pressure…

Soft Condensed Matter · Physics 2022-04-20 Eni Kume , Laurence Noirez

We report dynamical shear-modulus measurements for five glass-forming liquids (pentaphenyl trimethyl trisiloxane, diethyl phthalate, dibutyl phthalate, 1,2-propanediol, and m-touluidine). The shear-mechanical spectra are obtained by the…

Soft Condensed Matter · Physics 2013-05-14 Claudio Maggi , Bo Jakobsen , Tage Christensen , N. B. Olsen , Jeppe C. Dyre

We study the statistical mechanics of supercooled liquids when the system evolves at a temperature $T$ with a field $\epsilon$ linearly coupled to its overlap with a reference configuration of the same liquid sampled at a temperature $T_0$.…

Statistical Mechanics · Physics 2022-04-05 Benjamin Guiselin , Ludovic Berthier , Gilles Tarjus

We assess the relative importance of spatial congestion and lowered temperature in the slowing dynamics of supercooled glycerol near the glass transition. We independently vary both volume, V, and temperature, T, by applying high pressure…

Soft Condensed Matter · Physics 2007-05-23 Kyaw Zin Win , Narayanan Menon

We have conducted a thorough theoretical and numerical investigation of the electronic susceptibility, polarizability, plasmons, their damping rates, as well as the static screening in pseudospin-1 Dirac cone materials with a flat band, or…

We investigate the temperature dependence of thermodynamic (density, isobaric heat capacity), dynamical (self-diffusion coefficient, shear viscosity), and dielectric properties of several water models, the commonly employed TIP3P water…

Soft Condensed Matter · Physics 2022-04-13 Tatiana I. Morozova , Nicolas A. Garcia , Jean-Louis Barrat