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We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared…

Atomic Physics · Physics 2015-06-24 Chen-Ting Liao , Arvinder Sandhu , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde

We present transient absorption spectra of an extreme ultraviolet attosecond pulse train in helium dressed by an 800 nm laser field with intensity ranging from $2\times10^{12}$ W/cm$^2$ to $2\times10^{14}$ W/cm$^2$. The energy range probed…

We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity,…

Atomic Physics · Physics 2016-03-09 Chen-Ting Liao , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde , Arvinder Sandhu

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

The extreme ultraviolet absorption spectrum of an atom is strongly modified in the presence of a synchronized intense infrared field. In this work we demonstrate control of the absorption properties of helium atoms dressed by an infrared…

We introduce a machine-learning-based approach to enhance the sensitivity of optical-extreme ultraviolet (XUV) transient absorption spectroscopy. A reference spectrum is used as input to a three-layer feed-forward neural network, allowing…

Optics · Physics 2023-05-04 Tobias Heinrich , Hung-Tzu Chang , Sergey Zayko , Murat Sivis , Claus Ropers

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We present a table-top extreme ultraviolet (XUV) beamline for measuring time- and frequency-resolved XUV excited optical luminescence (XEOL) with additional femtosecond-resolution XUV transient absorption spectroscopy functionality. XUV…

We study theoretically the photoabsorption spectra of an attosecond XUV pulse by a laserdressed atomic system. A weak XUV excites an autoionizing state which is strongly coupled to another autoionizing state by a laser. The theory was…

Atomic Physics · Physics 2012-05-23 Wei-Chun Chu , C. D. Lin

The ability to control absorption by modifying the polarization of light presents an exciting opportunity to experimentally determine the orbital alignment of absorption features. Here, attosecond extreme ultraviolet (XUV) transient…

X-ray refraction and absorption by neon atoms under the influence of an 800 nm laser with an intensity of 10^13 W/cm^2 is investigated. For this purpose, we use an ab initio theory suitable for optical strong-field problems. Its results are…

Atomic Physics · Physics 2013-03-25 Christian Buth , Robin Santra , Linda Young

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

Using ab-initio non-Born-Oppenheimer simulations, we demonstrate amplification of XUV radiation in a high-harmonic generation type process using the example of the hydrogen molecular ion. A small fraction of the molecules is pumped to a…

Atomic Physics · Physics 2016-03-23 Timm Bredtmann , Szczepan Chelkowski , Andre. D. Bandrauk , Misha Ivanov

We report on the experimental observation of strong-field dressing of an autoionizing two-electron state in helium with intense extreme-ultraviolet laser pulses from a free-electron laser. The asymmetric Fano line shape of this transition…

The free-free opacity in plasmas is fundamental to our understanding of energy transport in stellar interiors and for inertial confinement fusion research. However, theoretical predictions in the challenging dense plasma regime are…

We observe and control a molecular vibrational wave packet in an electronically excited state of the neutral hydrogen molecule. In an extreme-ultraviolet (XUV) transient-absorption experiment we launch a vibrational wave packet in the $D…

An extreme ultraviolet (EUV) single attosecond pulse passing through a laser-dressed dense gas is studied theoretically. The weak EUV pulse pumps the helium gas from the ground state to the 2s2p(1P) autoionizing state, which is coupled to…

Atomic Physics · Physics 2013-01-18 Wei-Chun Chu , C. D. Lin

Femtosecond carrier recombination in PbI2 is measured using tabletop high-harmonic extreme ultraviolet (XUV) transient absorption spectroscopy and ultrafast electron diffraction. XUV absorption from 45 eV to 62 eV measures transitions from…

The operation of a frequency comb at extreme ultraviolet (XUV) wavelengths based on pair-wise amplification and nonlinear upconversion to the 15th harmonic of pulses from a frequency comb laser in the near-infrared range is reported.…

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in…

Atomic Physics · Physics 2008-11-18 Christian Buth , Robin Santra
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