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Layered antiferromagnetic materials have emerged as a novel subset of the two-dimensional family providing a highly accessible regime with prospects for layer-number-dependent magnetism. Furthermore, transition metal phosphorous…

Materials Science · Physics 2024-01-09 Daniel J. Gillard , Daniel Wolverson , Oscar M. Hutchings , Alexander I. Tartakovskii

Polarized Raman-scattering spectra of superconducting, single-crystalline FeSe evidence pronounced phonon anomalies with temperature reduction. A large 6.5% hardening of the B_1g(Fe) phonon mode is attributed to the suppression of local…

Polarized Raman-scattering spectra of non-superconducting, single-crystalline FeTe are investigated as function of temperature. We have found a relation between the magnitude of ordered magnetic moments and the linewidth of A1g phonons at…

Strongly Correlated Electrons · Physics 2015-05-27 V. Gnezdilov , Yu. Pashkevich , P. Lemmens , A. Gusev , K. Lamonova , I. Vitebskiy , O. Afanasiev , S. Gnatchenko , V. Tsurkan , J. Deisenhofer , A. Loidl

Using Raman spectroscopy, we investigate the lattice phonons, magnetic excitations, and magneto-elastic coupling in the distorted triangular-lattice Heisenberg antiferromagnet alpha-SrCr2O4, which develops helical magnetic order below 43 K.…

We investigate the interplay of the electron-phonon and the spin fluctuation interaction for the superconducting state of YBa$_2$Cu$_3$O$_{7}$. The spin fluctuations are described within the nearly antiferromagnetic Fermi liquid theory,…

Superconductivity · Physics 2009-10-31 T. S. Nunner , J. Schmalian , K. H. Bennemann

We report plane-polarized Raman scattering spectra of iron oxypnictide superconductor NdFeAsO$_{1-x}$F$_x$ single crystals with varying fluorine $x$ content. The spectra exhibit sharp and symmetrical phonon lines with a weak dependence on…

Superconductivity · Physics 2009-11-13 Y. Gallais , A. Sacuto , M. Cazayous , P. Cheng , L. Fang , H. H. Wen

The interactions among lattice, charge, and spin degrees of freedom fundamentally shape material properties. In FeSe, symmetry-breaking perturbations serve as highly sensitive probes of these couplings. Previous work has shown that defects…

Raman scattering in the spin-crossover system [Fe(pmd)(H2O){Au(CN)2}2]*H2O reveals a complex three-phase spin-state transition in contrast to earlier observations in magnetization measurements. We observe different spin state phases as…

Strongly Correlated Electrons · Physics 2010-03-09 V. Gnezdilov , P. Lemmens , P. Scheib , M. Ghosh , Yu. G. Pashkevich , H. Paulsen , V. Schuenemann , J. A. Wolny , G. Agusti , J. A. Real

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

We report the direct observation of a "resonance" mode in the lowest-energy optic phonon very near the zone center around (111) in the multiferroic BiFeO$_3$ using neutron scattering methods. The phonon scattering intensity is enhanced when…

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

We investigate the effects of electron-phonon coupling, as well as of spin and charge fluctuations on the superconducting state in a single layer of FeSe on SrTiO$_3$ substrate. These three bosonic mediators of Cooper pairing are treated on…

Superconductivity · Physics 2020-11-11 Fabian Schrodi , Alex Aperis , Peter Oppeneer

We use inelastic neutron scattering to study acoustic phonons and spin excitations in single crystals of NaFeAs, a parent compound of iron pnictide superconductors. NaFeAs exhibits a tetragonal-to-orthorhombic structural transition at…

The magnetic moment in the parent phase of the iron-pnictide superconductors varies with composition even when the nominal charge of iron is unchanged. We propose the spin-lattice coupling due to the magneto-volume effect as the primary…

Superconductivity · Physics 2015-05-14 T. Egami , B. V. Fine , D. J. Singh , D. Parshall , C. de la Cruz , P. Dai

The lattice dynamics and the effect of pressure on superconducting LiFeAs in both nonmagnetic (NM) and striped antiferromagnetic (SAF) phases are investigated using the plane-wave pseudopotential, density-functional-based method. While the…

Superconductivity · Physics 2010-07-13 G. Q. Huang , Z. W. Xing , D. Y. Xing

Muon-spin rotation experiments were performed on the pnictide high temperature superconductor SmFeAsO$_{1-x}$F$_{x}$ with x=0.18 and 0.3. We observed an unusual enhancement of slow spin fluctuations in the vicinity of the superconducting…

In this letter we investigated the temperature-dependent Raman spectra of CaMn7O12 helimagnet from room temperature down to 10 K. The temperature dependence of the Raman mode parameters show remarkable anomalies for both antiferromagnetic…

Recent observation of a "kink" in single-particle dispersion in photoemission experiments on cuprate superconductors has initiated a heated debate over the issue of a boson that mediates the pairing in cuprates. If the "kink" is indeed…

Strongly Correlated Electrons · Physics 2009-11-11 Tonica Valla

Neutrons have played an important role in advancing our understanding of the pairing mechanism and the symmetry of the superconducting energy gap in the iron arsenide compounds. Neutron measurements of the phonon density-of-state are in…

Superconductivity · Physics 2014-07-15 R. Osborn , S. Rosenkranz , E. A. Goremychkin , A. D. Christianson

Magnetic inelastic neutron scattering (INS) studies of iron-based superconductors reveal a strongly temperature-dependent spin-fluctuation spectrum in the normal conducting state, which develops a prominent low-energy resonance feature when…

Superconductivity · Physics 2012-09-28 Andreas Heimes , Roland Grein , Matthias Eschrig
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