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To shed light on the role of magnetism on the superconducting mechanism of the oxygen-free FeAs pnictides, we investigate the effect of magnetic ordering on phonon dynamics in the low-temperature orthorhombic parent compounds, which present…

Linear and non-linear couplings of magnetic and lattice excitations are at the heart of many fascinating magnetophononic phenomena observed in rare-earth orthoferrites, the distinctive feature of which is the tendency to spin-reorientation…

We present a Raman study of ZrAs_{2} single crystals, a nodal line semimetal with symmetry-enforced Dirac-like band crossings. We identified the symmetry of phonon modes by polarized light measurements and comparison with calculated phonon…

Materials Science · Physics 2024-05-16 R. Bacewicz , C. Jastrzębski , K. Zberecki , A. S. Wadge , D. Jastrzębski , A. Wiśniewski

We report the first observation of soft-x-ray scattering from spin fluctuations in a high-Tc parent compound. An antiferromagnetic charge transfer insulator, CaCuO2, was irradiated by Cu M-edge soft x-rays. Ultra-high resolution…

We investigate the electronic and magnetic properties as well as lattice dynamics and spin-phonon coupling of $\beta$-Na$_{0.33}$V$_2$O$_5$ using temperature-dependent Raman scattering, dc-magnetization and dc-resistivity, x-ray…

Materials Science · Physics 2022-11-23 Rishabh Shukla , Clemens Ulrich , R. S. Dhaka

We used polarization-resolved Raman scattering to study the magneto-elastic coupling in the parent compounds of several families of Fe-based superconductors (BaFe2As2, EuFe2As2, NaFeAs, LiFeAs, FeSe and LaFeAsO). We observe an emergent…

Spin-lattice relaxation is a key open problem to understand the spin dynamics of single-molecule magnets and molecular spin qubits. While modelling the coupling between spin states and local vibrations allows to determine the more relevant…

Atomic and Molecular Clusters · Physics 2021-11-08 Aman Ullah , José J. Baldoví , Alejandro Gaita-Ariño , Eugenio Coronado

We report low-temperature Raman signatures of the Heisenberg quantum magnet Ca$_{10}$Cr$_7$O$_{28}$, showing clear anomalies in phonon mode frequencies and linewidths below $\sim$100 K. This crossover temperature lies in between the…

Strongly Correlated Electrons · Physics 2023-12-12 Srishti Pal , Arnab Seth , Anzar Ali , Yogesh Singh , D. V. S. Muthu , Subhro Bhattacharjee , A. K. Sood

The mechanism of unconventional superconductivity, such as high-temperature-cuprate, Fe-based, and heavy-fermion superconductors, has been studied as a central issue in condensed-matter physics. Spin fluctuations, instead of phonons, are…

Superconductivity · Physics 2021-10-27 K. Ishida , S. Matsuzaki , M. Manago , T. Hattori , S. Kitagawa , M. Hirata , T. Sasaki , D. Aoki

We investigate theoretically the superconducting state of the undoped Fe-based superconductor ThFeAsN. Using input from $ab~initio$ calculations, we solve the Fermi-surface based, multichannel Eliashberg equations for Cooper-pair formation…

Superconductivity · Physics 2021-09-22 Fabian Schrodi , Fairoja Cheenicode Kabeer , Alex Aperis , Peter M. Oppeneer

We performed in-situ angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES (SARPES) experiments to investigate the relationship between electronic band structures and ferromagnetism in SrRuO$_3$ (SRO) thin films. Our…

Spin-phonon interactions are central to many interesting phenomena, ranging from superconductivity to magnetoelectric effects. Yet, they are believed to have a negligible influence on the structural behavior of most materials. For example,…

Materials Science · Physics 2016-12-14 Claudio Cazorla , Oswaldo Dieguez , Jorge Iniguez

The coupling between antiferromagnetic spins and infrared-active phonons in solids is responsible for many intriguing phenomena and is a field of intense research with extensive potential applications in the modern devices based on…

Lattice vibrations are highly sensitive to crystal symmetries and their changes across phase transitions. The latter can modify irreducible (co)representations and corresponding infrared and Raman selection rules of phonons. This concept is…

We present a theoretical study of the dynamical spin susceptibility for the intriguing Fe-based superconductor FeSe, based on a tight-binding model developed to account for the temperature-dependent band structure in this system. The model…

Superconductivity · Physics 2016-01-05 A. Kreisel , Shantanu Mukherjee , P. J. Hirschfeld , Brian M. Andersen

For more than a decade, the unusual distribution of electrons observed in ARPES (angle-resolved photoemission spectroscopy) data within the energy range of ~30meV to ~300meV below the Fermi level, known as the ARPES range, has remained a…

Superconductivity · Physics 2024-01-05 Chi Ho Wong , Rolf Lortz

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

Strongly Correlated Electrons · Physics 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

In recent years, the fundamental physics of spin-thermal (i.e., magnon-phonon) interaction has attracted significant experimental and theoretical interests given its potential paradigm-shifting impacts in areas like spin-thermoelectrics,…

Materials Science · Physics 2018-03-14 Xufei Wu , Zeyu Liu , Tengfei Luo

We report temperature-dependent Raman spectra of CeFeAsO0.9F0.1 from 4 K to 300 K in spectral range of 60 to 1800 cm-1 and interpret them using estimates of phonon frequencies obtained from first-principles density functional calculations.…

The lattice dynamics of the $\rm YMnO_3$ magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data…

Materials Science · Physics 2012-03-09 Julien Varignon , Sébastien Petit , Marie-Bernadette Lepetit
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