English
Related papers

Related papers: Increasing the density melts ultrasoft colloidal g…

200 papers

We explore the relationship between a machine-learned structural quantity (softness) and excess entropy in simulations of supercooled liquids. Excess entropy is known to scale well the dynamical properties of liquids, but this…

Soft Condensed Matter · Physics 2023-06-07 Ian R. Graham , Paulo E. Arratia , Robert A. Riggleman

We introduce a new quantity to probe the glass transition. This quantity is a linear generalized compressibility which depends solely on the positions of the particles. We have performed a molecular dynamics simulation on a glass forming…

Disordered Systems and Neural Networks · Physics 2007-05-23 Herve M. Carruzzo , Clare C. Yu

In a preceding paper, Mukhopadhyay and I studied the diffusive motion of a tagged molecule in a heterogeneous glass-forming liquid at temperatures just above a glass transition. Among other features of this system, we postulated a relation…

Statistical Mechanics · Physics 2009-11-13 J. S. Langer

The penetrable-sphere model has been introduced in the literature to describe the peculiar thermodynamic behavior of some colloidal systems. In this model the interaction potential is $\phi(r)=\epsilon>0$ if the two spheres are overlapped…

Statistical Mechanics · Physics 2014-11-10 Andres Santos

Rapidly cooling a liquid may result in a glass transition, creating an amorphous solid whose shear and bulk moduli are finite. Even when done with constant density, these resulting moduli depend strongly on the rate of cooling.…

Materials Science · Physics 2013-05-03 Ashwin J. , Eran Bouchbinder , Itamar Procaccia

In this work, we study the nature of transitions between inherent structures of a two-dimensional model supercooled liquid. We demonstrate that these transitions occur predominately along a small number of directions on the energy…

Statistical Mechanics · Physics 2013-03-12 Glen M. Hocky , David R. Reichman

Using molecular dynamics calculations and the Voronoi tessellation, we study the evolution of the local structure of a soft-sphere glass versus temperature starting from the liquid phase at different quenching rates. This study is done for…

Disordered Systems and Neural Networks · Physics 2009-10-31 Philippe Jund , Remi Jullien

The understanding of thermodynamic glass transition has been hindered by the lack of proper models beyond mean-field theories. Here, we propose a three-dimensional lattice glass model on a simple cubic lattice that exhibits the typical…

Statistical Mechanics · Physics 2020-08-07 Yoshihiko Nishikawa , Koji Hukushima

We consider a microscopic model of a polymer blend that is prone to phase separation. Permanent crosslinks are introduced between randomly chosen pairs of monomers, drawn from the Deam-Edwards distribution. Thereby, not only density but…

Soft Condensed Matter · Physics 2009-11-11 Christian Wald , Paul M. Goldbart , Annette Zippelius

A simple model of dimerizing hard spheres with highly nontrivial fluid-solid phase behaviour is proposed. The model is studied using the recently proposed resummed thermodynamic perturbation theory for central force (RTPT-CF) associating…

Soft Condensed Matter · Physics 2016-07-26 Yurij V. Kalyuzhnyi , Peter T. Cummings

Dense or glassy active matter, as a result of its remarkable resemblance to passive glass-forming materials, is enjoying increasing scientific interest. To better grasp the subtle effect of active motion on the process of vitrification, a…

Soft Condensed Matter · Physics 2023-10-20 Vincent E. Debets , Liesbeth M. C. Janssen

The low-temperature quasi-universal behavior of amorphous solids has been attributed to the existence of spatially-localized tunneling defects found in the low-energy regions of the potential energy landscape. Computational models of…

Disordered Systems and Neural Networks · Physics 2023-01-05 Felix C. Mocanu , Ludovic Berthier , Simone Ciarella , Dmytro Khomenko , David R. Reichman , Camille Scalliet , Francesco Zamponi

We study model protein solutions and colloidal suspensions in the temperature range whereupon the nature of the system changes from a homogeneous fluid to a "cluster fluid". It is commonly assumed - as deduced by the behavior of the…

Statistical Mechanics · Physics 2011-09-02 Jean-Marc Bomont , Jean-Louis Bretonnet , Dino Costa

The study of the properties of glass-forming liquids is difficult for many reasons. Analytic solutions of mean field models are usually available only for systems embedded in a space with an unphysically high number of spatial dimensions;…

Disordered Systems and Neural Networks · Physics 2015-02-26 Manuel Sebastian Mariani , Giorgio Parisi , Corrado Rainone

We found a finite temperature glass transition in the absence of quenched disorder in frustrated Josephson junction arrays (JJA) on a square lattice with anisotropic Josephson couplings by numerical simulations. The vortexes develop zigzag…

Superconductivity · Physics 2009-07-23 Hajime Yoshino , Tomoaki Nogawa , Bongsoo Kim

We study the quantum version of a lattice model whose classical counterpart captures the physics of structural glasses. We discuss the role of quantum fluctuations in such systems and in particular their interplay with the amorphous order…

Disordered Systems and Neural Networks · Physics 2015-03-17 Laura Foini , Guilhem Semerjian , Francesco Zamponi

If quenched fast enough, a liquid is able to avoid crystallization and will remain in a metastable supercooled state down to the glass transition, with an important increase in viscosity upon further cooling. There are important differences…

Disordered Systems and Neural Networks · Physics 2016-06-01 C. Yildirim , J. -Y. Raty , M. Micoulaut

A fresh approach to the data from experiments with hard sphere colloids yields seminal insights into the glass transition. The precise determination of the fraction of particles caged by their neighbours is unprecedented and provides…

Soft Condensed Matter · Physics 2021-10-01 W. van Megen , H. J. Schöpe

We propose a new analytic approach to study the phase diagram of random heteropolymers, based on the cavity method. For copolymers we analyze the nature and phenomenology of the glass transition as a function of sequence correlations.…

Disordered Systems and Neural Networks · Physics 2009-11-10 A. Montanari , M. Mueller , M. Mezard

We report computer simulations of oscillatory athermal quasi-static shear deformation of dense amorphous samples of a three dimensional model glass former. A dynamical transition is observed as the amplitude of the deformation is varied:…

Disordered Systems and Neural Networks · Physics 2015-06-15 Davide Fiocco , Giuseppe Foffi , Srikanth Sastry