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Using one-dimensional simulations analyzed through the lens of open quantum systems, we study the photoelectron's strong-field dynamics from an atom surrounded by a scattering environment stochastically structured. We theoretically…

Quantum Physics · Physics 2026-05-21 Simon His , Camille Lévêque , Jérémie Caillat , Richard Taïeb , Jonathan Dubois

The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…

Atomic Physics · Physics 2016-09-28 Xi Liu , Xiaosong Zhu , Liang Li , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We report theoretical calculations on the effect of the multiple orbital contribution in high-order harmonic generation (HHG) from aligned CO$_2$ with inclusion of macroscopic propagation of harmonic fields in the medium. Our results show…

Atomic Physics · Physics 2011-05-10 Cheng Jin , Anh-Thu Le , C. D. Lin

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We present a numerical study of the resonant high harmonic generation by tin ions in an elliptically-polarised laser field along with a simple analytical model revealing the mechanism and main features of this process. We show that the…

Optics · Physics 2021-04-22 M. A. Khokhlova , M. Yu. Emelin , M. Yu. Ryabikin , V. V. Strelkov

The total cross section of the top quark-antiquark pair production near threshold in $\gamma\gamma$ collision is computed analytically up to the next-to-leading order in perturbative and nonrelativistic expansion for general photon…

High Energy Physics - Phenomenology · Physics 2009-10-31 A. A. Penin , A. A. Pivovarov

We present a novel ab-initio single-electron approach to correlated electron dynamics in strong laser fields. By writing the electronic wavefunction as a product of a marginal one-electron wavefunction and a conditional wavefunction, we…

Atomic Physics · Physics 2016-02-02 Axel Schild , E. K. U. Gross

The interaction of matter with a quantized electromagnetic mode is considered. Representing a strong exciting field, the mode is assumed to contain a large number of photons. As a result, the material response is highly nonlinear: the…

Quantum Physics · Physics 2020-01-17 Ákos Gombkötő , Sándor Varró , Péter Mati , Péter Földi

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

High-harmonic generation (HHG) is one of the fundamental processes at the heart of attosecond physics. Traditionally viewed as an effective single-particle effect, recent advances have focused on contributions beyond this single-particle…

We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities…

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron

High-harmonic generation (HHG), a typical nonlinear optical effect, has been actively studied in electron systems such as semiconductors and superconductors. As a natural extension, we theoretically study HHG from electric polarization,…

Strongly Correlated Electrons · Physics 2020-03-10 Tatsuhiko N. Ikeda , Masahiro Sato

We present the experimental and theoretical details of our recent published letter [Phys. Rev. Lett. 115. 123002] on synchronized high-harmonic and terahertz-wave spectroscopy (HATS) from nonadiabatically aligned nitrogen molecules in…

Atomic Physics · Physics 2016-06-03 Yindong Huang , Chao Meng , Jing Zhao , Xiaowei Wang , Zhihui Lü , Dongwen Zhang , Jianmin Yuan , Zengxiu Zhao

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Xiao Zhang , Tao Zhu , Hongchuan Du , Hong-Gang Luo , Jeroen van den Brink , Rajyavardhan Ray

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…