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The transport properties of a large-spin molecule strongly coupled to ferromagnetic leads in the presence of transverse magnetic anisotropy are studied theoretically. The relevant spectral functions, linear-response conductance and the…

Mesoscale and Nanoscale Physics · Physics 2015-11-13 Maciej Misiorny , Ireneusz Weymann

The oxidation and spin state of a metal-organic molecule determine its chemical reactivity and magnetic properties. Here, we demonstrate the reversible control of the oxidation and spin state in a single Fe-porphyrin molecule in the force…

Mesoscale and Nanoscale Physics · Physics 2018-04-09 Benjamin W. Heinrich , Christopher Ehlert , Nino Hatter , Lukas Braun , Christian Lotze , Peter Saalfrank , Katharina J. Franke

We report the electronic structure and magnetic ordering of the single molecule magnet [Mn$_{10}$O$_{4}$(2,2'-biphenoxide)$_{4}$Br$_{12}$]$^{4-}$ based on first-principles all-electron density-functional calculations. We find that two of…

Materials Science · Physics 2009-11-07 Jens Kortus , Tunna Baruah , N. Bernstein , Mark R. Pederson

We demonstrate that the interplay of in-plane biaxial and uniaxial anisotropy fields in (Ga,Mn)As results in a magnetization reorientation transition and an anisotropic AC susceptibility which is fully consistent with a simple single domain…

Materials Science · Physics 2007-05-23 K-Y. Wang , M. Sawicki , K. W. Edmonds , R. P. Campion , S. Maat , C. T. Foxon , B. L. Gallagher , T. Dietl

Electrically manipulating the quantum properties of nano-objects, such as atoms or molecules, is typically done using scanning tunnelling microscopes and lateral junctions. The resulting nanotransport path is well established in these model…

We report on the charge carrier dynamics in single lateral quantum dot molecules and the effect of an applied electric field on the molecular states. Controllable electron tunneling manifests itself in a deviation from the typical excitonic…

Mesoscale and Nanoscale Physics · Physics 2012-02-29 C. Hermannstädter , G. J. Beirne , M. Witzany , M. Heldmaier , J. Peng , G. Bester , L. Wang , A. Rastelli , O. G. Schmidt , P. Michler

We theoretically investigate quantum transport through single-molecule magnet (SMM) junctions with ferromagnetic and normal-metal leads in the sequential regime. The current obtained by means of the rate-equation gives rise to the tunneling…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Haiqing Xie , Qiang Wang , Hujun Jiao , J. -Q. Liang

We present a new family of exchange biased Single Molecule Magnets in which antiferromagnetic coupling between the two components results in quantum behaviour different from that of the individual SMMs. Our experimental observations and…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 W. Wernsdorfer , N. Aliaga-Alcalde , R. Tiron , D. N. Hendrickson , G. Christou

The external controllability of the magnetic properties in topological insulators would be important both for fundamental and practical interests. Here we predict the electric-field control of ferromagnetism in a thin film of insulating…

Mesoscale and Nanoscale Physics · Physics 2015-07-15 Jing Wang , Biao Lian , Shou-Cheng Zhang

Electric-field control of magnetism via inverse magnetostrictive effect is an efficient path towards improving energy-efficient storage and sensing devices based on giant magnetoresistance effect. In this letter, we report on lateral…

Materials Science · Physics 2023-02-16 Vadym Iurchuk , Julien Bran , Manuel Acosta , Bohdan Kundys

We study electronic transport through a magnetic molecule with an intrinsic spin $S$ coupled to two magnetic electrodes, in the incoherent regime. The molecule is modeled as a single resonant level with large Coulomb repulsion (no double…

Mesoscale and Nanoscale Physics · Physics 2010-11-19 Thibaut Jonckheere , Ken-Ichiro Imura , Thierry Martin

We report the precise control of tunneling magnetoresistance (TMR) in devices of self-assembled core/shell Fe$_3$O$_4$/Co$_{1-x}$Zn$_x$Fe$_2$O$_4$ nanoparticles ($0\leq x\leq 1$). Adjusting the magnetic anisotropy through the content of…

We study gate field effects on the Mn$_{12}$O$_{12}$(COOH)$_{16}$(H$_2$O)$_4$ | graphene | GaAs heterostructure via first-principles calculations. We find that under moderate doping levels electrons can be added to but not taken from the…

Materials Science · Physics 2022-01-05 Shuanglong Liu , Maher Yazback , James N. Fry , Xiao-Guang Zhang , Hai-Ping Cheng

Search for single-molecule magnets (SMMs) with high blocking temperature (TB) is urgent for practical applications in magnetic recording, molecular spintronics and quantum computing. Based on the First-principles calculations, magnetic…

Materials Science · Physics 2014-02-04 Jun Hu , Ruqian Wu

Shuttling of electrons in single-molecule transistors with magnetic leads in the presence of an external magnetic field is considered theoretically. For a current of partially spin-polarized electrons a shuttle instability is predicted to…

Mesoscale and Nanoscale Physics · Physics 2015-07-22 O. A. Ilinskaya , S. I. Kulinich , I. V. Krive , R. I. Shekhter , Y. W. Park , M. Jonson

The electric field effect on magnetic anisotropy was studied in an ultrathin Fe(001) monocrystalline layer sandwiched between Cr buffer and MgO tunnel barrier layers, mainly through post-annealing temperature and measurement temperature…

The magnetic anisotropy of low-dimensional Mott systems exhibits unexpected magnetotransport behavior useful for spin-based quantum electronics. Yet, the anisotropy of natural materials is inherently determined by the crystal structure,…

We have investigated crystalline magnetic anisotropy in the electric field (EF) for the Fe-Pt surface which have a large perpendicular anisotropy, by means of the first-principles approach. The anisotropy is reduced linearly with respect to…

Materials Science · Physics 2015-05-13 Masahito Tsujikawa , Tatsuki Oda

The main objective of this work is to investigate theoretically how tilting of an easy axis of a single-molecule magnet (SMM) from the orientation collinear with magnetic moments of the leads affects the switching process induced by current…

Mesoscale and Nanoscale Physics · Physics 2016-08-14 Maciej Misiorny , Józef Barnas

Motivated in part by experiments performed by M.H. Pan et al. (nanoletters, v.5, p 83, 2005), we have undertaken a theoretical study of the the magnetic properties of two-monolayer thick Co nanoplatelets with an equilateral triangular…

Other Condensed Matter · Physics 2009-11-11 T. O. Strandberg , C. M. Canali , A. H. MacDonald
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