Related papers: Hyperfine spectroscopy using co-propagating pump-p…
Optical pumping is fundamental to high-precision measurement using thermal alkali-metal atoms in vapor cells. In applications such as atomic magnetometry, buffer gases (e.g., $\mathrm{N}_2$ or $\mathrm{He}$) at specific pressures are…
In the present article we consider an accurate modeling of spectrograph with cascade of volume-phase holographic gratings. The proposed optical scheme allows to detect spectra in an extended wavelength range without gaps providing…
We have measured hyperfine structure in the first-excited $P$ state ($D$ lines) of all the naturally-occurring alkali atoms. We use high-resolution laser spectroscopy to resolve hyperfine transitions, and measure intervals by locking the…
Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…
We present an experimental technique enabling mechanical-noise free, cavity-enhanced frequency measurements of an atomic transition and its hyperfine structure. We employ the 532nm frequency doubled output from a Nd:YAG laser and an iodine…
We have developed a hyperspectral imaging scheme that involves a combination of dual-comb spectroscopy and Hadamard-transform-based single-pixel imaging. The scheme enables us to obtain 12,000 hyperspectral images of amplitude and phase at…
Optical spectroscopy of atoms and molecules is a field where one usually operates very far from thermal equilibrium conditions. A prominent example is spectroscopy of thin vapors, where the pump irradiation leads to a non equilibrium…
We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…
We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…
We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…
In this paper, ultra-broad band optical signal amplification are analyzed and demonstrated by utilizing supercontinuum generation propagating over the photonic crystal fiber. The coupled nonlinear Schroodinger equation containing parametric…
Photonic quantum technologies rely on the efficient generation and interference of indistinguishable photons. Exceptional achievements in this respect have been obtained by domain engineering of quasi-phase-matched parametric…
Currently, there is great interest in laser cooling of barium monofluoride (BaF) molecules for precision tests of fundamental symmetries. We use high-resolution absorption spectroscopy to characterize several as yet imprecisely known…
We present an experimental approach to detect the saturated absorption spectroscopy different from conventional scheme. Using this approach, crossovers are removed to avoid their overlap with other peaks in the spectrum and sensitivity of…
Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…
Detailed analysis of spectral line broadening and variations in relative intensities of hyperfine spectral components due to optical pumping is presented. Hyperfine levels of sodium $3p_{1/2}$ and $3p_{3/2}$ levels are selectively excited…
The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…
We report on the observation of enhanced four-wave mixing via crossover resonance in a Doppler broadened cesium vapor. Using a single laser frequency, a resonant parametric process in a double-$\Lambda$ level configuration is directly…
A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…
Vacuum birefringence is one of the most striking predictions of strong field quantum electrodynamics: Probe photons traversing a strong field region can indirectly sense the applied "pump" electromagnetic field via quantum fluctuations of…