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We present a new imaging method for pump-probe microscopy that explores non-collinear excitation. This method (crossed-beam pump-probe microscopy, or CBPM) can significantly improve the axial resolution when imaging through low-NA lenses,…

Optics · Physics 2020-04-22 Jun Jiang , Warren S. Warren , Martin C. Fischer

We present ultrahigh-resolution measurements of state-to-state inelastic differential cross sections for NO-Ne and NO-Ar collisions, obtained by combining the Stark deceleration and velocity map imaging techniques. We show that for…

Optical parametric amplifiers (OPAs) are promising to overcome the wavelength coverage and noise limitations in conventional optical amplifiers based on rare-earth doping and semiconductor gain. However, the high power requirement remains a…

Optics · Physics 2026-02-06 Yung-Cheng Kao , Jiaqi Huang , Ian Briggs , Pao-Kang Chen , Linran Fan

We introduce the concept of phase-synchronous undersampling in nonlinear spectroscopy. The respective theory is presented and validated experimentally in a phase-modulated quantum beat experiment by sampling high phase modulation…

Chemical Physics · Physics 2018-03-14 Lukas Bruder , Marcel Binz , Frank Stienkemeier

We demonstrate cantilever-enhanced photoacoustic spectroscopy in the mid-infrared using a supercontinuum source. The approach is broadband, compact, and allows for higher photoacoustic signal intensity and enhanced signal-to-noise ratio as…

Instrumentation and Detectors · Physics 2018-11-14 Tommi Mikkonen , Caroline Amiot , Antti Aalto , Kim Patokoski , Goëry Genty , Juha Toivonen

Pump-probe spectroscopy is a powerful tool to study ultrafast exciton dynamics, revealing the underlying complex interactions on the electronic scale. Despite significant advances in experimental techniques, developing a comprehensive and…

Materials Science · Physics 2025-09-10 Lu Qiao , Ronaldo Rodrigues Pela , Claudia Draxl

We present an effective linear response approach to pump-probe femtosecond coherence spectroscopy in the well separated pulse limit. The treatment presented here is based on a displaced and squeezed state representation for the…

Chemical Physics · Physics 2009-11-06 Anand T. N. Kumar , Florin Rosca , Allan Widom , Paul M. Champion

It is demonstrated that velocity selective optical pumping/saturation resonances of reduced absorption in a Rb vapor nanocell with thickness \textit{L=} $\lambda $, 2$\lambda $, and 3$\lambda $ (resonant wavelength $\lambda $ = 780 nm)…

Classical Physics · Physics 2009-11-13 A. Sargsyan , D. Sarkisyan , A. Papoyan , Y. Pashayan-Leroy , P. Moroshkin , A. Weis , A. Khanbekyan , E. Mariotti , L. Moi

Superconducting resonator parametric amplifiers achieve ultra-low-noise amplification through the nonlinear kinetic inductance of thin-film superconductors. One of the main challenges to the operation of these devices is the separation of…

Instrumentation and Detectors · Physics 2024-10-29 Songyuan Zhao , Stafford Withington , Christopher Niall Thomas

The conditions required for spontaneous parametric down-conversion in a waveguide with periodic nonlinearity in the presence of an unguided pump field are established. Control of the periodic nonlinearity and the physical properties of the…

Hyperspectral imaging is useful for applications ranging from medical diagnostics to agricultural crop monitoring; however, traditional scanning hyperspectral imagers are prohibitively slow and expensive for widespread adoption. Snapshot…

Image and Video Processing · Electrical Eng. & Systems 2020-09-30 Kristina Monakhova , Kyrollos Yanny , Neerja Aggarwal , Laura Waller

Point-spread function of the probe forming optics ($PSF_{optics} $) is reported for the first time in an uncorrected (without multipole correctors) scanning electron microscope (SEM). In an SEM, the electron probe information is lost as the…

Materials Science · Physics 2024-07-02 Surya Kamal , Richard K. Hailstone

We demonstrate how a narrowband pump and a broadband spectrum can be spatially multiplexed by selective coupling them in two distinct modes of a few-mode microstructure fiber. The first mode carries most of the input pump energy, and…

We investigate the propagation of a coherent probe light pulse through a three-level atomic medium (in the $\Lambda$--configuration) in the presence of a pump laser under the conditions for gain without inversion. When the carrier frequency…

Quantum Physics · Physics 2007-05-23 Filippo Caruso , Ivan Herrera , Saverio Bartalini , Francesco Cataliotti

We demonstrate an unseeded, multimode four-wave mixing process in hot $^{85}$Rb vapor, using two pump beams of the same frequency that cross at a small angle. This results in the simultaneous fulfillment of multiple phase-matching…

Quantum Physics · Physics 2018-08-01 Erin M. Knutson , Jon D. Swaim , Sara Wyllie , Ryan T. Glasser

Millimetre-wave observations represent an important tool for Cosmology studies. The Line Intensity Mapping (LIM) technique has been proposed to map in three dimensions the specific intensity due to line (e.g. [CII], CO) emission, for…

Instrumentation and Methods for Astrophysics · Physics 2023-08-29 Usasi Chowdhury , Florence Levy-Bertrand , Martino Calvo , Johannes Goupy , Alessandro Monfardini

Band-resolved frequency modulation spectroscopy is a common method to measure weak signals of radiative ensembles. When the optical depth of the medium is large, the signal drops exponentially and the technique becomes ineffective. In this…

Skimmed supersonic beams provide intense, cold, collision-free samples of atoms and molecules are one of the most widely used tools in atomic and molecular laser spectroscopy. High-resolution optical spectra are typically recorded in a…

In this paper, we demonstrate that it is possible to combine both Raman amplification and polarization attraction of a signal wave in a single optical fiber by means of a counterpropagating scheme. Experiments were performed near 1550 nm in…

Optics · Physics 2012-07-20 Philippe Morin , Stéphane Pitois , Julien Fatome

In pump-probe spectroscopy, one often needs to analyse the transmission or reflection of electromagnetic waves through optically pumped media. Here, it is common practice to approximate the analysis in order to extract non-equilibrium…

Optics · Physics 2019-02-26 Peter Karlsen , Euan Hendry