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The microscopic dynamics of spontaneously aged and rejuvenated glassy Laponite is investigated through X-ray photon correlation spectroscopy. Two different behaviours of the intensity autocorrelation functions are observed depending on the…

Soft Condensed Matter · Physics 2023-09-06 Roberta Angelini , Barbara Ruzicka

We show numerically that a three-dimensional model for structural glass displays aging, rejuvenation and memory effects when submitted to a temperature cycle. These effects indicate that the free energy landscape of structural glasses may…

Soft Condensed Matter · Physics 2019-07-03 Camille Scalliet , Ludovic Berthier

The structural relaxation, potential energy states, and mechanical properties of a model glass subjected to thermal cycling are investigated using molecular dynamics simulations. We study a non-additive binary mixture which is annealed with…

Soft Condensed Matter · Physics 2018-12-05 Nikolai V. Priezjev

Using molecular simulations, we identify microscopic relaxation events of individual particles in ageing structural glasses, and determine the full distribution of relaxation times. We find that the memory of the waiting time $t_w$ elapsed…

Soft Condensed Matter · Physics 2015-05-13 Mya Warren , Joerg Rottler

The competing effects of slow structural relaxations (aging) and deformation at constant strain rate on the shear yield stress $\tau^y$ of simple model glasses are examined using molecular simulations. At long times, aging leads to a…

Soft Condensed Matter · Physics 2009-11-11 Joerg Rottler , Mark O. Robbins

Molecular dynamics simulations are used to study a unique expanded jammed state. Tension transforms many glassy polymers from a dense glass to a network of fibrils and voids called a craze. Entanglements between polymers and interchain…

Soft Condensed Matter · Physics 2009-11-07 Jörg Rottler , Mark O. Robbins

We study the effect of shear on the aging dynamics of a colloidal suspension of synthetic clay particles. We find that a shear of amplitude $\gamma$ reduces the relaxation time measured just after the cessation of shear by a factor…

Soft Condensed Matter · Physics 2009-11-07 F. Ozon , T. Narita , A. Knaebel , G. Debrégeas , P. Hébraud , J. -P. Munch

The evolution of porous structure, potential energy and local density in binary glasses under oscillatory shear deformation is investigated using molecular dynamics simulations. The porous glasses were initially prepared via a rapid thermal…

Soft Condensed Matter · Physics 2022-10-25 Nikolai V. Priezjev , Maxim A. Makeev

With molecular dynamics simulations of a fluid mixture of classical particles interacting with pair-wise additive Weeks-Chandler-Andersen potentials, we consider the time series of particle displacements and thereby determine distributions…

Statistical Mechanics · Physics 2011-11-10 Lester O. Hedges , Lutz Maibaum , David Chandler , Juan P. Garrahan

The history dependence of the glasses formed from flow-melted steady states by a sudden cessation of the shear rate $\dot\gamma$ is studied in colloidal suspensions, by molecular dynamics simulations, and mode-coupling theory. In an ideal…

We study shear yielding and steady state flow of glassy materials with molecular dynamics simulations of two standard models: amorphous polymers and bidisperse Lennard-Jones glasses. For a fixed strain rate, the maximum shear yield stress…

Soft Condensed Matter · Physics 2009-11-10 Joerg Rottler , Mark O. Robbins

The dynamic fragmentation of residually stressed solids involves a complex interplay between stored elastic energy, stress wave propagation, and crack instabilities. In this work, we investigate the fracture mechanics of chemically…

Soft Condensed Matter · Physics 2026-02-25 Vineet Dawara , Koushik Viswanathan

Solids subjected to repeated cycles of stress or deformation can fail after several cycles, a phenomenon termed fatigue failure. Although intensely investigated for a wide range of materials owing to its obvious practical importance, a…

Soft Condensed Matter · Physics 2024-09-27 Swarnendu Maity , Himangsu Bhaumik , Shivakumar Athani , Srikanth Sastry

Motivated by recent experimental studies probing i) the existence of a mobile layer at the free surface of glasses, and ii) the capillary leveling of polymer nanofilms, we study the evolution of square-wave patterns at the free surface of a…

Soft Condensed Matter · Physics 2019-09-18 Ioannis Tanis , Kostas Karatasos , Thomas Salez

We propose a computational strategy to quantify the temperature evolution of the timescales and lengthscales over which dynamic facilitation affects the relaxation dynamics of glass-forming liquids at low temperatures, that requires no…

Soft Condensed Matter · Physics 2024-06-25 Cecilia Herrero , Ludovic Berthier

Glassy systems are ubiquitous in nature, and are characterized by slow relaxations to equilibrium without a typical timescale, aging and memory effects. Understanding these is a long-standing problem in physics. We study the aging of the…

Disordered Systems and Neural Networks · Physics 2009-11-30 Ariel Amir , Yuval Oreg , Yoseph Imry

Experiments performed on a wide range of glassy materials display many interesting phenomena, such as aging behavior. In recent years, a large body of experiments probed this nonequilibrium glassy dynamics through elaborate protocols, in…

Statistical Mechanics · Physics 2007-05-23 Ludovic Berthier , Virgile Viasnoff , Olivia White , Vladimir Orlyanchik , Florent Krzakala

Using molecular dynamics simulations, we investigate the effect of uniaxial elastostatic compression on the potential energy, structural relaxation, and mechanical properties of binary glasses. We consider the three-dimensional Kob-Andersen…

Soft Condensed Matter · Physics 2019-06-12 Nikolai V. Priezjev

The yielding transition, structural relaxation, and mechanical properties of metallic glasses subjected to repeated loading are examined using molecular dynamics simulations. We consider a poorly-annealed Cu-Zr amorphous alloy periodically…

Soft Condensed Matter · Physics 2024-08-30 Nikolai V. Priezjev

Elastic and dissipative properties of granular assemblies under uniaxial compression are studied both experimentally and by numerical simulations. Following a novel compaction procedure at varying oscillatory pressures, the stress response…

Soft Condensed Matter · Physics 2009-11-11 Jasna Brujic , Ping Wang , Chaoming Song , David L. Johnson , Olivier Sindt , Hernan A. Makse